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Rabi Oscillations in Disguise: Strong Exciton-Surface Plasmon Polariton Coupling Probed by Two-Dimensional Electronic Spectroscopy

Daniel Timmer, Jin-Hui Zhong, Moritz Gittinger, Thomas Quenzel, Sven Stephan, Jennifer Zablocki, Arne Lützen, Martin Silies, Antonietta De Sio, and Christoph Lienau

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Abstract

We explore dynamics of strong exciton-plasmon couplings using two-dimensional electronic spectra displaying pronounced Rabi oscillations of their cross-peaks. Radiative couplings govern the polariton nonlinearity and provide first access to the two-quantum-excitations of the coupled system.

© 2022 The Author(s)

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More Like This
Two-Dimensional Electronic Spectroscopy of Strong Exciton-Surface Plasmon Polariton Coupling

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IH_4_2 International Quantum Electronics Conference (IQEC) 2013

View More...
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