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Probing Free Carrier and Exciton Dynamics in Bulk Gallium Selenide with Two-Dimensional Electronic Spectroscopy

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Abstract

Ultrafast two-dimensional electronic spectroscopy with phase-locked pump pulses provides a unique method to disentangle exciton and free carrier dynamics in the prototypical semiconductor gallium selenide with sub-10 fs temporal and 4 meV spectral resolution.

© 2022 The Author(s)

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