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Two-Dimensional Electronic Spectroscopy of Strong Exciton-Surface Plasmon Polariton Coupling

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Abstract

Strong exciton-plasmon-couplings are investigated using two-dimensional electronic spectroscopy, revealing Rabi oscillations of polariton cross-peaks and accessing two-quantum excitations. Coherent population oscillations between excitons that are strongly and weakly coupled to the plasmonic field are demonstrated.

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