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Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in J-aggregate/metal hybrid nanostructures

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Abstract

We report the first real-time observation of ultrafast Rabi oscillations in J-aggregate/metal nanostructures, evidencing coherent energy transfer between excitonic quantum emitters and SPP fields. This presents a new approach towards coherent, all-optical ultrafast plasmonic devices.

© 2013 Optical Society of America

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