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Temperature dependence of the linear optical properties of organic thin films of dye-doped PMMA via surface plasmon spectroscopy

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Abstract

Interest in organic materials for electro-optic device fabrication is due to the large molecular nonlinearities[1], the relative ease of fabrication[2], the ability to tailor the molecular structure through organic synthesis[3] and the potential for very high-speed low power devices[4]. The observation of an electric-field-induced quasi-permanent ordering[5], which eliminates the inversion symmetry and allows second order processes, has led to much work on the parameters which determine the degree[6] and the stability of alignment. This alignment induces a birefringence in the film[7] which is observed as the index perpendicular to the surface of the film via the surface plasmon[8].

© 1992 Optical Society of America

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