Local-Field Effects in Langmuir-Blodgett Monolayers Studied with Second-Harmonic Generation

G. Cnossen; K. E. Drabe; D. A. Wiersma

XVIII International Quantum Electronics Conference
Technical Digest Series (Optica Publishing Group, 1992),
paper TuO3

Local-Field Effects in Langmuir-Blodgett Monolayers Studied with Second-Harmonic Generation

G. Cnossen, K. E. Drabe, and D. A. Wiersma

International Quantum Electronics Conference 1992

Vienna Austria
14–19 June 1992
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NLO of Organic Materials (TuO)

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G. Cnossen, K. E. Drabe, and D. A. Wiersma, "Local-Field Effects in Langmuir-Blodgett Monolayers Studied with Second-Harmonic Generation," in XVIII International Quantum Electronics Conference, Technical Digest Series (Optica Publishing Group, 1992), paper TuO3.

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Abstract

We investigated the dependence of the second-order nonlinear susceptibility χ⁽²⁾ (2ω, ω, ω) of Langmuir-Blodgett monolayers as a function of surface density. A nonlinear dependence of χ⁽²⁾ on surface density N_s was observed, which could be attributed to the microscopic local-field.

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