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Conferences > CLEO_QELS > 2015 > FM2B > FM2B.1

Femtosecond coherent nano-spectroscopy of coupled molecular dynamics

Joanna M. Atkin, Paul M. Sass, Honghua U. Yang, Paul Teichen, Joel Eaves, and Markus B. Raschke

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Abstract

We isolate the vibrational free-induction decay of a homogeneous molecular sub-ensemble using ultrafast infrared vibrational scattering-scanning near-field microscopy. The observed long-lived few picosecond vibrational coherences, intramolecular coherence transfer, and spatial variations in vibrational modes indicate non-ergodic behavior.

© 2015 Optical Society of America

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