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Conferences > CLEO_QELS > 2013 > QTu1B > QTu1B.3

Ultrafast infrared near-field vibrational nano-spectroscopy

Xiaoji G. Xu and Markus B. Raschke

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Abstract

We demonstrate femtosecond infrared vibrational free-induction decay spectroscopy on the nano-scale. The near-field coupling between the transient molecular polarization and optical antenna properties of the metallic scanning probe tip can enhance the vibrational dephasing.

© 2013 Optical Society of America

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