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Optica Publishing Group
  • Conference on Lasers and Electro-Optics/Pacific Rim 2007
  • (Optica Publishing Group, 2007),
  • paper WB3_4

The Hollow on the Excited-State Potential for Photo-induced ‘Jahn-Teller’ Distortion of Copper Complexes Revealed by Ultrafast Spectroscopy

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Abstract

Ultrafast dynamics of photo-induced structural change of [Cu(dmphen)2]+ was studied by femtosecond emission spectroscopy and 25-fs time-resolved pump-probe spectroscopy. It was found that the S1 state remains undistorted for 660 fs before structural change, being trapped in a shallow potential minimum at the perpendicular configuration on the S1 potential.

© 2007 IEEE

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