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Time-Domain Raman Tracking of Ultrafast Flattening Distortion in Organometallic Complex

S. Takeuchi, M. Iwamura, H. Watanabe, and T. Tahara

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Abstract

We studied vibrational structures of the metal-to-ligand-charge-transfer state of Cu(I)-diimine complexes through wavepacket motions generated impulsively at various delay-times. The obtained “instantaneous” Raman data provided firm vibrational evidences for ultrafast nature of the flattening distortion.

© 2010 Optical Society of America

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