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Nonlinear photocarrier dynamics in multilayer ${{\rm WSe}_2}$ induced by intense terahertz pulses

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Abstract

Non-equilibrium photocarriers in multilayer ${{\rm WSe}_2}$ injected by femtosecond laser pulses exhibit extraordinary nonlinear dynamics in the presence of intense THz fields. The THz absorption in optically excited ${{\rm WSe}_2}$ rises rapidly in the low THz field regime and gradually ramps up at high intensities. The strong THz pulses drive the photocarriers into sidebands of higher mobility and release trapped charge carriers, which consequently enhance the transient conductivity of ${{\rm WSe}_2}$. The spectrally analyzed conductivity reveals distinctive features, indicating that the photocarriers undergo resonant interactions such as carrier-photon scattering.

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The data that support the findings of this study are available from the corresponding author upon reasonable request.

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