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Noisy propagation of coherent states in a lossy Kerr medium

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Abstract

We identify and discuss nonlinear phase noise arising in Kerr self-phase modulation of a coherent light pulse propagating through an attenuating medium with third-order nonlinearity in a dispersion-free setting. This phenomenon, accompanying the standard unitary Kerr transformation of the optical field, is described with high accuracy as Gaussian phase diffusion with parameters given by closed expressions in terms of system properties. We show that the irreversibility of the nonlinear phase noise ultimately limits the ability to transmit classical information in the phase variable over a lossy single-mode bosonic channel with Kerr-type nonlinearity. Our model can be also used to estimate the amount of squeezing attainable through self-phase modulation in a Kerr medium with distributed attenuation.

© 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

1. INTRODUCTION

Third-order nonlinearity in optical media makes the effective refractive index dependent on light intensity. One of the consequences of this phenomenon, known as the Kerr effect, is self-phase modulation, which consists of an intensity-dependent contribution to the phase shift acquired by a light beam propagating trough the medium. In the single-mode description, such propagation can be described by a nonlinear oscillator with 1 degree of freedom [13]. The quantum version of this model exhibits a wealth of nonclassical effects, such as squeezing [4] and generation of Schrödinger cat states [5]. However, their experimental realization requires suppression of the accompanying decoherence mechanisms with a prominent role played by photon loss. While it is feasible to experimentally produce squeezed states using third-order nonlinearity in optical fibers [68], Schrödinger cat states turn out to be much more elusive owing to higher nonlinearities necessary for generation and greater susceptibility to losses [9].

In parallel, optical nonlinearities have been recognized as a key factor limiting the information capacity of fiber optical communication links [1013]. To date, most studies in this area have used the classical description of electromagnetic fields in terms of complex amplitudes governed by deterministic equations of motion. In this approach, noise appears as a result of signal amplification, averaging over signals transmitted through other channels in a multiplexed system or the functioning of the detection stage. The performance of conventional optical detection is limited by the shot noise, which is a manifestation of quantum fluctuations in measured electromagnetic fields [14]. However, if the propagation of electromagnetic fields is both nonlinear and lossy, quantum fluctuations in the optical medium undergo a nonunitary transformation, which may result in additional noise that would not emerge in a classical description. This eventuality motivates a full quantum mechanical study of nonlinear effects in optical signal propagation.

The purpose of the present paper is to analyze a single-mode model for self-phase modulation of a coherent light pulse propagating through a lossy nonlinear dispersion-free medium. Our central objective will be to identify and characterize quantitatively excess noise, which occurs as a result of nonlinear transformation of quantum fluctuations in the course of lossy propagation and cannot be compensated at the output with the help of a reversible unitary transformation. Specifically, we show that lossy Kerr propagation can be mathematically decomposed into a sequence of three distinct processes that are formally applied to the input coherent state one after another. This decomposition is represented pictorially in Fig. 1. The first process is standard attenuation, which lowers the complex amplitude of the input coherent state. The last one is unitary Kerr evolution, which would have occurred in the absence of loss. The intermediary process we will focus our attention on arises solely as a result of a nontrivial interplay between the Kerr nonlinearity and the optical loss. We demonstrate that it has the form of nonlinear phase noise, which can be approximated with high accuracy by a Gaussian distribution for the additive random phase. We provide closed analytical expressions for parameters that characterize the properties of this decoherence mechanism.

 figure: Fig. 1.

Fig. 1. Decomposition of noisy propagation of a coherent light pulse in a lossy Kerr medium into a sequence of three processes. Process 1 is linear attenuation of the input complex amplitude ζ0 by a factor τ, where τ is the power transmission of the medium. Process 2 is nonlinear phase noise, which shifts the phase by ϕ0 and introduces Gaussian phase diffusion characterized by variance σ2. Finally, process 3 is unitary Kerr evolution, which would have occurred in the absence of attenuation, applied to the output of process 2.

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The derived effective description of the nonlinear phase noise is employed to discuss its impact on the transmission of classical information in the phase variable. We choose continuous phase modulation with constant intensity as the encoding format [15] and characterize accessible information using the Holevo quantity [1618], which takes into account the most general quantum mechanical measurement strategies at the channel output, including compensation of reversible nonlinear effects. It is shown that, for the propagation over a lossy Kerr medium, the Holevo quantity exhibits a maximum in the signal intensity, and that the nonlinear phase noise renders the phase variable useless for information encoding at high signal powers. Consequently, this effect can be expected to substantially alter the ultimate communication capacity of an optical channel compared with the linear case, which has been analyzed rigorously in recent years [19]. As another application of the presented description, we study generation of squeezing using the Kerr effect and derive a simple estimate for the impact of distributed loss in the squeezing medium on the output quadrature variance.

This paper is organized as follows. In Section 2, we introduce the theoretical model for the nonlinear propagation. In Section 3, we derive the effective description for the excess noise generated in the model. Based on this description, we demonstrate in Section 4 how the excess noise has an impact on the accessible information for the phase variable. In Section 5, we discuss the generation of squeezed states using a lossy Kerr medium and derive a simple estimate for the attainable reduction of quadrature noise in the case of distributed attenuation. Finally, Section 6 closes the paper with some concluding remarks.

2. LOSSY NONLINEAR PROPAGATION

In a single-mode model describing dispersion-free propagation of an optical pulse in a lossy Kerr medium along a direction z, the evolution of the system is given by the master equation

dϱ^dz=iμ[n^2,ϱ^(z)]+α2(2a^ϱ^(z)a^n^ϱ^(z)ϱ^(z)n^),
with the mode creation and annihilation operators a^ and a^, respectively, the photon number operator n^=a^a^, the nonlinearity strength μ, and the parameter α characterizing linear losses. The form of Eq. (1) follows the approach used in previous works to analyze the spatial propagation of light in nonlinear media [20,21], which can also include loss and decoherence mechanisms [22] analogously to the standard time-domain description. A more complete model should include other effects occurring in nonlinear media, such as guided acoustic wave Brillouin scattering and Raman scattering. Beyond the single-mode description considered here, one would need to take into account, e.g., modulation instability and cross-phase modulation, which severely affects the performance of wavelength-division multiplexed systems.

In order to separate reversible phenomena, we will carry out the analysis in the interaction picture defined by the nonlinear Hamiltonian μn^2 of the Kerr interaction and represent the field density operator ϱ^(z) as

ϱ^(z)=exp(iμzn^2)ϱ^(z)exp(iμzn^2).
One should note the opposite sign in the exponent of the evolution operator compared with the standard Heisenberg picture in the time domain, as the formalism is now applied to propagation along a spatial dimension. The master equation for the transformed density operator ϱ^(z) reads
dϱ^dz=α2(2a^(z)ϱ^(z)[a^(z)]n^ϱ^(z)ϱ^(z)n^),
with the distance-dependent annihilation operator in the interaction picture a^(z)=exp(iμzn^2)a^exp(iμzn^2) and the photon number operator n^ invariant with respect to the transformation. We assume that the input state is a coherent state with a complex amplitude ζ0, ϱ^(0)=|ζ0ζ0|, given in the Fock basis by a superposition:
|ζ0=en¯/2n=0ζ0nn!|n.
We will use n¯=|ζ0|2 to denote the mean photon number in the input coherent state. The propagation equations for the above model can be solved analytically [2,3]. In order to determine the elements of the field density matrix after a propagation distance z in the Fock basis ϱ^mn(z)=m|ϱ^(z)|n, one can use an ansatz:
ϱmn(z)=ζ0m(ζ0*)nm!n!e(m+n)αz/2cmn(z).
The factor cj(z) depends only on the difference j=mn between the matrix element indices. It is easy to verify that the above ansatz, after inserting into Eq. (3), yields a closed first-order differential equation for cj(z), which can be solved by standard means. For completeness, we present the detailed derivation in Appendix A.

It will be convenient to characterize the medium with two dimensionless parameters. The first one is the transmission τ=exp(αz), which specifies the fraction of optical energy τn¯ retained in the field at the channel output. The second one is the ratio ϰ=μ/α describing the strength of the nonlinear interaction with respect to attenuation. Note that ϰ is an intensive parameter characterizing the bulk medium itself, while τ depends on the channel length. Using this parameterization, the solution of the master equation can be written compactly as

ϱmn(z)=m|τζ0τζ0|nexp[n¯fτ((mn)ϰ)].
The product of the first two terms m|τζ0τζ0|n describes a coherent state with an attenuated amplitude τζ0. Because unitary Kerr evolution has been included in the transformation to the interaction picture in Eq. (2), the last factor exp[n¯fτ((mn)ϰ)] appearing on the right-hand side of Eq. (6) only contains effects arising from the combination of the Kerr nonlinearity and loss. The complex function in the exponent is given explicitly by
fτ(ϰ)=1τ1τ12iϰ12iϰ.
In Fig. 2 we depict the Husimi Q function for the state ϱ^(z) with an increasing mean photon number. The dimensionless nonlinearity for the example had been chosen as ϰ=5×106. It can be related to parameters of actual fiber optic links as ϰ=γNLω0/(αT), where γNL is the fiber third-order nonlinearity, ω0 is the energy of a single photon at the carrier frequency ω0, and T is the pulse duration. Combinations of these parameters that give the exemplary value of ϰ for two common types of optical fiber have been collected in Table 1. The channel transmission has taken τ=108, which corresponds to 400 km of a standard SMF-28 fiber. Two effects are clearly seen: the overall phase of the state is shifted, and the state becomes spread on a circle. The spreading becomes stronger with increasing pulse intensity. It should be emphasized that this spreading does not arise from the reversible deformation of quadrature fluctuations by the unitary Kerr self-modulation. These effects are excluded in the density matrix in the interaction picture ϱ^(z); furthermore, they can be estimated to be negligible in the presented numerical examples: for a nonlinear strength of ϰ=5×106, a channel transmission of τ=108 and a mean photon number at the output of τn¯=60 at the input, the relative change in quadrature fluctuations calculated using the approach presented in Section 5 can be characterized using the squeezing parameter r to remain below 2r2.2×102.

 figure: Fig. 2.

Fig. 2. Husimi Q function of the output state emerging from a lossy nonlinear medium with transmission τ=108 and nonlinearity ϰ=5×106, shown for the output mean photon number (a) τn¯=1, (b) τn¯=3, (c) τn¯=15, and (d) τn¯=60. A coherent state with a real amplitude n¯ has been assumed at the input. Nonlinear phase noise is clearly seen to increase with the pulse intensity.

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Tables Icon

Table 1. Exemplary Combinations of Optical Fiber and Pulse Parameters that Give the Value of the Dimensionless Nonlinearity Parameter ϰ=5×106

3. NONLINEAR PHASE NOISE

Let us now derive effective parameters that describe features seen in Fig. 2. The starting point will be the inspection of the real and imaginary parts of the function fτ(ϰ) defined in Eq. (7), shown in Fig. 3 for transmissions τ=108 and τ=0.8 as a function of the dimensionless nonlinearity ϰ. As seen in Fig. 3(a), for τ1 the real part Refτ(ϰ) has the form of a dip centered around ϰ=0. Using Eq. (7), this dip can be modelled by an inverted Lorentzian proportional to 1/(1+4ϰ2), whose width is of the order of 1. The relevant range of the argument of fτ in Eq. (6) is defined by the range of the Fock basis indices m and n for which the product of the scalar products m|τζ0τζ0|n substantially differs from zero. Because |m|τζ0|2 is a Poissonian distribution in the integer variable m with an average τn¯ and hence standard deviation τn¯, this condition will be met for |mn|τn¯. Consequently, the argument of the function fτ has the order of magnitude ϰ|mn|ϰτn¯. If the product ϰτn¯1, which is the case for the numerical example shown in the preceding section, it is justified to expand the function fτ(ϰ) up to the second order in ϰ, which gives

fτ(ϰ)2i(1τ+τlogτ)ϰ+[42τ2τ(1logτ)2]ϰ2.

After the above approximation, the exponent multiplying Fock basis elements of the coherent state density matrix in Eq. (6) contains terms linear and quadratic in mn with, respectively, imaginary and real multiplicative constants. It is easily verified by a direct calculation that such a density operator can be equivalently written as a statistical mixture of coherent states with a fixed mean photon number and the phase averaged using a Gaussian distribution with a mean ϕ0 and a standard deviation σ:

m,n=0|mn|m|ζζ|nexp[i(mn)ϕ0(mn)2σ22]=dϕ12πσ2e(ϕϕ0)2/2σ2|eiϕζeiϕζ|.
For clarity, we have denoted here ζ=τζ0. Using the explicit expression for the Fock state density matrix elements from Eq. (6) with the approximation given in Eq. (8) enables us to identify the parameters of the Gaussian distribution as
ϕ0=2ϰn¯(1τ+τlogτ),
σ2=4ϰ2n¯[2ττ(1logτ)2].
It is seen that the linear term in the expansion shown in Eq. (8) generates a phase shift ϕ0, and the quadratic term is responsible for the phase noise characterized by the variance σ2. While the phase shift ϕ0 can be pre-compensated at the channel input, the phase noise clearly affects the ability to encode information in the phase variable. We will discuss quantitatively this phenomenon in Section 4.

 figure: Fig. 3.

Fig. 3. Real and the imaginary parts of the function fτ(ϰ) defined in Eq. (7) for a transmission of (a) τ=108 and (b) τ=0.8.

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As a side remark, let us note that the validity of the expansion in Eq. (8) can be extended beyond the regime discussed above. This is because the function fτ(ϰ) appears in the exponent in Eq. (6) multiplied by the input intensity n¯. If this product is large compared with 1, the exponential factor effectively suppresses the respective off-diagonal elements of the density matrix regardless of its specific form. In Fig. 3(b) we plot the real and imaginary parts of fτ(ϰ) for τ=0.8 compared with the corresponding quadratic expansion. Because the asymptotic value for |ϰ|1 is fτ(ϰ)1τ, the rule of thumb for the quadratic expansion to hold using the above reasoning is (1τ)n¯1. The accuracy of this approximation can be assessed by comparing the infidelity 1F=1Trϱ^ϱ^Gϱ^ between the actual density matrix ϱ^ and its approximation ϱ^G introduced in Eq. (9) with parameters of the Gaussian phase noise given in Eqs. (10) and (11). The infidelity is shown in Fig. 4 for τ=0.8 as a function of the mean output photon number τn¯ and the strength of the nonlinear interaction ϰ. It is seen that the departure from the Gaussian approximation in the parameter space is localized in the region of high ϰ and moderate output mean photon numbers τn¯ and works very well for higher pulse intensities. Note that the upper limit for the range of ϰ in Fig. 4 has been taken well above realistic values for optical fibers. Notice also the small values of the infidelity 1F, ensuring that the physical properties of the phase diffused state are close to those of the state subject to lossy nonlinear propagation [2325].

 figure: Fig. 4.

Fig. 4. Infidelity 1F between the actual density matrix ϱ^ and its approximation ϱ^G based on the Gaussian phase diffusion model for the transmission τ=0.8 as a function of the output mean photon number τn¯ and the dimensionless nonlinearity ϰ.

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4. PHASE SHIFT KEYING

Nonlinear phase noise analyzed in the preceding section is a nondeterministic phenomenon that cannot be compensated at the channel output in contrast with unitary Kerr transformation. This affects the ability to transmit classical information in the phase variable, which is routinely used in keying constellations for fiber optic communication, such as quadriphase shift keying [26]. Without phase noise, the amount of information that can be transmitted by modulating the phase of a light pulse grows with its intensity. Fixing intensity defines a ring in the complex amplitude plane, which, with increasing radius, can accommodate more coherent states whose distinguishability is limited by the shot noise. This picture changes dramatically when channel nonlinearities induce phase noise. As seen in Eq. (11), the variance of the phase noise grows linearly with the input field intensity, which may actually obliterate information keyed in the phase.

We will analyze quantitatively the above phenomenon by considering a keying constellation, which consists of coherent states |eiϕζ0 continuously distributed on a circle with a uniform distribution pϕ=1/2π [15], as shown in Fig. 5(a). As a measure of accessible information, we will take the Holevo quantity χ, which takes into account the most general measurement strategies permitted in quantum mechanics [1618]. The Holevo quantity is given as a difference between the von Neumann entropy S(ϱ^)=Tr(ϱ^logϱ^) of the average state emerging from the channel and the average entropy of individual states, and it is given in our case by

χ=S(02πdϕpϕϱ^ϕ)02πdϕpϕS(ϱ^ϕ).
Because the von Neumann entropy is invariant with respect to unitary transformations, we can exclude from our calculations the unitary Kerr process and take as ϱ^ϕ phase-diffused states given by Eq. (9) for ζ=τeiϕζ0. The phase-averaged state appearing in the first term of Eq. (12) as the argument of the von Neumann entropy is a statistical mixture of Fock states with a Poissonian distribution characterized by the mean τn¯. Consequently, the classical Shannon entropy of this distribution yields the value of the first term in Eq. (12) irrespectively of the phase noise. The second term in Eq. (12) is simply given by the von Neumann entropy of any individual output state S(ϱ^ϕ), which does not depend on the specific value of ϕ.

 figure: Fig. 5.

Fig. 5. (a) Continuous phase shift keying. Information is encoded in the phase ϕ of a constellation of coherent states with constant intensity uniformly distributed on a circle. (b) Holevo quantity for the continuous phase shift keying constellation as a function of the output mean photon number τn¯ for several values of the nonlinearity ϰ.

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In Fig. 5(b), we depict the Holevo quantity as a function of the mean photon number in the output pulse for several values of the dimensionless nonlinearity parameter ϰ. In the case of a linear channel, when ϰ=0, the Holevo quantity grows monotonically with the signal intensity. However, in the nonlinear case, the Holevo quantity exhibits a maximum, which can be understood as an interplay between two effects. For low intensities, the nonlinear phase noise has minute impact, and increasing the mean photon number allows us to encode more information in the phase variable thanks to the lower extent of the shot noise relative to the circumference of the ring. For high intensities, the nonlinear phase noise makes coherent states diffused on the ring, as seen in Figs. 2(c) and 2(d), which effectively scrambles any information encoded in the phase variable. In general, one can consider an input ensemble of coherent states, which modulated both the intensity and the phase parameters. The quantification of the attainable transmission rate needs to take into account the nontrivial dependence of the information capacity of the phase variable on the signal intensity.

Let us stress that the nonlinear phase noise is irreversible, and it cannot be compensated at the channel output. Its origin can be understood intuitively as follows. The amplitude of the coherent pulse entering the nonlinear medium exhibits vacuum-level fluctuations. The nonlinearity deforms these fluctuations in a nontrivial manner, which for short distances can be visualized as squeezing one field quadrature at the cost of expanding the conjugate one [27]. In the lossless case, variances of these quadratures saturate the Heisenberg uncertainty relation, which indicates that the state remains pure, and the transformation is reversible. However, in the case of distributed attenuation, the propagating field exchanges fluctuations with the environment. The contribution to field fluctuations acquired that way is given at the vacuum level, which introduces excess noise [2830] that makes the state no longer Heisenberg-limited. Because the effect of losses is to lower the mean photon number of the Poissonian statistics of the pulse, and the Kerr nonlinearity affects only the off-diagonal elements of the density matrix in the Fock basis that characterize phase coherence, this mixedness occurs for the phase variable.

5. KERR SQUEEZING IN A LOSSY MEDIUM

The Kerr effect in optical fibers can be used to generate squeezed states of light, which exhibit quadrature fluctuations reduced below the shot noise level [4,68]. We will now use the effective description of self-phase modulation in a lossy nonlinear medium developed in preceding sections to analyze the attainable degree of squeezing in the presence of distributed attenuation.

In order to describe the output field emerging from the medium, we will take the phase diffused state evaluated using the Gaussian phase noise profile derived in Eq. (9):

ϱ^G=dϕ12πσ2eϕ2/2σ2|eiϕζeiϕζ|.
For notational simplicity, we have chosen the phase distribution to be centered at ϕ=0. We will also assume that the coherent amplitude ζ is real and positive, ζ=|ζ|. These two conditions can be satisfied by an appropriate choice of the input coherent state ζ0. The actual output state is obtained from ϱ^G via the unitary Kerr transformation, which yields exp(iμzn^2)ϱ^Gexp(iμzn^2). It will be most convenient to treat the unitary Kerr process exp(iμzn^2) in the Heisenberg picture, in which the propagation equation for the annihilation operator reads
da^dz=iμ[n^2,a^(z)]=iμ[2a^(z)a^(z)+1]a^(z).
Solving this equation allows us to express a^(z) and a^(z) in terms of a^(0) and a^(0). Expectation values involving the latter pair of operators should be taken over the ensemble of coherent states given in Eq. (13). For each individual pure state |eiϕζ in the ensemble, it will be convenient to use a substitution,
a^(z)=eiμz(2ζ2+1)eiϕ[ζ+b^(z)],
which shifts the reference frame to a location in which the initial mean field amplitude at z=0 is zeroed. This displacement maps the coherent state |eiϕζ onto the vacuum state |0, which should be used to calculate expectation values of expressions involving operators b^(0) and b^(0). The overall phase factor eiμz(2ζ2+1) has been introduced to simplify subsequent formulas. The resulting propagation equation for the operator b^(z) reads
db^dz=2iμζ2[b^(z)+b^(z)],
where on the right-hand side we retained only terms linear in b^(z) and b^(z). This is justified because b^(z) and b^(z) describe only small fluctuations around the field amplitude, which has been subtracted by the substitution in Eq. (15). The solution of the linearized differential equation for b^(z) is given by
b^(z)=(1+2iμzζ2)b^(0)+2iμzζ2b^(0).
We will now introduce operators for two orthogonal quadratures of the output field defined as
q^=eiμz(2ζ2+1)a^(z)+h.c.=eiϕ[ζ+b^(z)]+h.c.,
p^=ieiμz(2ζ2+1)a^(z)+h.c.=ieiϕ[ζ+b^(z)]+h.c.,
where h.c. denotes Hermitian conjugated terms. Calculating statistical properties of output field quadratures involves performing two averages. The first one is the quantum mechanical expectation value for expressions involving b^(z) and b^(z). These operators can be expressed using Eq. (17) by b^(0) and b^(0), which should be taken acting on the vacuum state. The results are
q^=2ζcosϕ,p^=2ζsinϕ
in the first order and
q^2=1+4ζ2cos2ϕ4μzζ2sin2ϕ+(4μzζ2)2sin2ϕ,
p^2=1+4ζ2sin2ϕ+4μzζ2sin2ϕ+(4μzζ2)2cos2ϕ
in the second order. The expectation value of the symmetrically ordered product of the quadratures q^ and p^ reads
12(q^p^+p^q^)=2ζ2sin2ϕ+4μzζ2cos2ϕ8(μtζ2)2sin2ϕ.
The second average is over the random phase shift ϕ with a probability distribution exp[ϕ2/(2σ2)]/2πσ2. Because the distribution function is even, we have sinϕ=sin2ϕ=0, and the remaining averages can be determined from the expectation values
cosϕ=eσ2/2,cos2ϕ=e2σ2.
It will be convenient to use in subsequent formulas a squeezing parameter r defined through a relation sinhr=2μzζ2. Let us now consider quadrature fluctuations around the mean value given by Δq^=q^q^ and Δp^=p^p^. Their variances are explicitly given by
(Δq^)2=1+2(1eσ2)2ζ2+2(1e2σ2)sinh2r,
(Δp^)2=1+2(1e2σ2)ζ2+2(1+e2σ2)sinh2r,
and the symmetrically ordered covariance reads
12(Δq^Δp^+Δp^Δq^)=2e2σ2sinhr.
Let us now identify the angle θ for which a general quadrature given by x^θ=q^cosθ+p^sinθ exhibits the strongest squeezing. It easy to verify that, in the absence of phase noise, when σ=0, the minimum quadrature variance is obtained for tanθ0=er and equals (Δx^θ0)2=e2r. When phase noise is included in the calculation, the optimal quadrature angle is given by
tan2θ=sinhrsinh2r+ζ2(eσ21),
and the corresponding variance reads
(Δx^θ)2=1+2ζ2(1eσ2)+2sinh2r2e2σ2sinh2r+[sinh2r+ζ2(eσ21)]2.
Let us recall that, in our representation of lossy Kerr self-phase modulation, the input coherent amplitude ζ0 enters the above expression through ζ2=τn¯ and hence sinhr=2μzτn¯, while σ2 is given by Eq. (11). In Fig. 6 we depict attainable squeezing for several values of the transmission τ assuming n¯=108. The abscissa is parameterized with the nonlinear interaction strength μ defining the actual value of sinhr. It is seen that, for strong nonlinearity, the squeezing is limited by the phase noise induced by the interplay between the self-phase modulation and losses.

 figure: Fig. 6.

Fig. 6. Attainable squeezing (Δx^θ)2 for the input mean photon number n¯=108 and several different values of the transmission τ as a function of the dimensionless nonlinear coefficient ϰ. For convenience, the abscissa is parameterized with sinhr=2ϰ(logτ)τn¯. Dashed horizontal lines correspond to the estimate (1τ)/3.

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The effective limit on attainable squeezing can be estimated using the following simple calculation. When exponents eσ2 and e2σ2 in Eqs. (25)–(27) are expanded up to the first order in σ2, the dominant effect of phase noise is the addition of an excess noise term (Δp)exc2=4σ2ζ2 to the variance of p^. All other terms including σ2 can be neglected, as they involve factors sinhr or sinh2r that are small compared to ζ2. This excess noise can be written as (Δp)exc2=4g(τ)sinh2r, where

g(τ)=2ττ(1logτ)2τ(logτ)213(1τ),
and the second approximate form is valid for the transmission τ close to one. For low attenuation, the optimal quadrature angle stays close to θ0; hence, the minimum quadrature variance can be approximated by
(Δx^θ0)2=e2r+(Δp)exc2sin2θ0=e2r+g(τ)(1e2r)tanhr.
For substantial squeezing, when r1, we have (1e2r)tanhr1; consequently, the second term simplifies to g(τ)(1τ)/3. This value defines the minimum quadrature variance in the presence of loss. It is noteworthy that it differs by a simple factor 1/3 compared with the scenario when attenuation physically occurs after the squeezing transformation. In realistic nonlinear media, one needs to include other effects, such as guided acoustic wave Brillouin scattering and Raman scattering, which have a more severe effect on the attainable squeezing [31].

6. CONCLUSIONS

We have presented a theoretical model for the propagation of coherent states in a lossy medium with third-order nonlinearity in a dispersion-free setting. Within this model, we have identified nonlinear phase noise emerging from the interplay between optical loss and the Kerr nonlinearity. This excess noise is nonunitary and cannot be compensated at the output. It has been shown that, for a broad range of system parameters, an effective description of this excess noise is given by a Gaussian distribution introducing also a nonlinear phase shift for the input state. While the phase shift can be taken into account at the preparation stage, the Gaussian phase diffusion process is nonunitary and cannot be compensated. Identification of the nonlinear phase noise allows us to formally decompose the description of propagation in a lossy nonlinear medium into a sequence of three distinct processes, namely, standard attenuation followed by Gaussian phase diffusion and then unitary Kerr evolution. The presented decomposition is valid for coherent states. It can be generalized to arbitrary states of the electromagnetic field using the Glauber–Sudarshan P quasiprobability distribution for the density operator [32,33], but it should be kept in mind that the effective transformation of individual coherent states in this representation depends in a nontrivial manner on their amplitudes through the parameters of the Gaussian phase diffusion process. As a side note, the quadratic approximation used in the derivation of the nonlinear phase noise parameters is reminiscent of certain simplified models of decoherence in quantum mechanics [34], which can be tested also in spatial propagation of optical fields through dense, multiple-scattering, random media [35].

We also demonstrated that the nonlinear phase noise severely impairs the ability to encode classical information in the phase variable. Specifically, we considered phase shift keying using a continuous constellation of coherent states distributed on a ring with a fixed intensity. In the case of nonzero nonlinearity, the Holevo quantity, used as a measure of accessible information, exhibits a maximum for a finite input mean photon number. This is because, for input coherent states with a sufficiently high mean photon number, the phase becomes completely scrambled due to increasing diffusion. Consequently, when designing an optimal input ensemble of coherent states in both phase and intensity variables for transmission of classical information, the contribution from the high intensity region should approach that of a Poisson channel [36]. It would be also interesting to investigate the ultimate quantum limit on the classical capacity of an optical channel with nonlinear phase noise, generalizing recently results obtained for linear Gaussian models [19]. Finally, we investigated the interplay between nonlinearity and losses in the generation of squeezed states utilizing a Kerr medium. We showed that the nonlinear phase noise can be used to estimate the attainable squeezing in the presence of distributed attenuation.

One should note that, in the context of optical communication, nonlinear transformation of spontaneous emission contributed by signal amplification is known to introduce excess phase noise [37,38]. This effect arises in the classical propagation model of electromagnetic fields. Our analysis incorporates fully quantum fluctuations contributed by both the input field and the loss mechanism, which are not taken into account in classical propagation equations. Hence, nonlinear phase noise discussed here appears even without signal amplification built into the optical link. Furthermore, when considering accessible information, we assumed that the reversible effects of the nonlinear propagation have been compensated by applying an appropriate unitary transformation at the channel output. Our quantum mechanical model can be extended to include amplifier noise using methods developed in [2].

APPENDIX A: SOLUTION OF THE MASTER EQUATION

In this appendix, we present a detailed calculation of the factor cj(z) used in the ansatz in Eq. (5). With the transformed operator a^(z)=exp(iμzn^2)a^exp(iμzn^2) and the number operator n^ the master equation,

dϱ^dz=α2(2a^(z)ϱ^(z)[a^(z)]n^ϱ^(z)ϱ^(z)n^),
can be reduced to a differential equation for the matrix elements of the density matrix, which then reads
dϱm,ndz=α2[2ρm+1,n+1(z)(m+1)(n+1)e2iμz(mn)ρm,n(z)(m+n)].

Inserting the ansatz given in Eq. (5) into Eq. (A2) yields a differential equation for the factor cj(z) with j=mn, which can be written as

dcjdz=αn¯eαze2iμzjcj(z).
This first-order differential equation is solved by standard separation of variables, which yields
cj(z)=exp(n¯αα2iμjeαze2iμzj+A0)=exp(n¯τ12iϰjτ2iϰj+A0),
where A0 is the integration constant and in the last step we used τ=eαz, ϰ=μ/α and e2iμzj=e2iϰjlogτ=τ2iϰj. Inserting this solution into the ansatz in Eq. (5) yields
ϱmn(z)=(τζ0)m(τζ0*)nm!n!exp(n¯τ12iϰ(mn)12iϰ(mn)+A0).
The constant A0 can be obtained from the initial condition ϱmn(0)=en¯ζ0m(ζ0*)n/m!n!, which yields Eq. (6) with the function fτ(ϰ) given by Eq. (7).

Funding

Fundacja na rzecz Nauki Polskiej (FNP); European Regional Development Fund (ERDF).

Acknowledgment

We acknowledge insightful discussions with Ivan H. Deutsch, R. García-Patrón, and Ch. Marquardt. This work is part of the project “Quantum Optical Communication Systems” carried out within the TEAM program of the Foundation for Polish Science co-financed by the European Union under the ERDF.

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Figures (6)

Fig. 1.
Fig. 1. Decomposition of noisy propagation of a coherent light pulse in a lossy Kerr medium into a sequence of three processes. Process 1 is linear attenuation of the input complex amplitude ζ 0 by a factor τ , where τ is the power transmission of the medium. Process 2 is nonlinear phase noise, which shifts the phase by ϕ 0 and introduces Gaussian phase diffusion characterized by variance σ 2 . Finally, process 3 is unitary Kerr evolution, which would have occurred in the absence of attenuation, applied to the output of process 2.
Fig. 2.
Fig. 2. Husimi Q function of the output state emerging from a lossy nonlinear medium with transmission τ = 10 8 and nonlinearity ϰ = 5 × 10 6 , shown for the output mean photon number (a)  τ n ¯ = 1 , (b)  τ n ¯ = 3 , (c)  τ n ¯ = 15 , and (d)  τ n ¯ = 60 . A coherent state with a real amplitude n ¯ has been assumed at the input. Nonlinear phase noise is clearly seen to increase with the pulse intensity.
Fig. 3.
Fig. 3. Real and the imaginary parts of the function f τ ( ϰ ) defined in Eq. (7) for a transmission of (a)  τ = 10 8 and (b)  τ = 0.8 .
Fig. 4.
Fig. 4. Infidelity 1 F between the actual density matrix ϱ ^ and its approximation ϱ ^ G based on the Gaussian phase diffusion model for the transmission τ = 0.8 as a function of the output mean photon number τ n ¯ and the dimensionless nonlinearity ϰ .
Fig. 5.
Fig. 5. (a) Continuous phase shift keying. Information is encoded in the phase ϕ of a constellation of coherent states with constant intensity uniformly distributed on a circle. (b) Holevo quantity for the continuous phase shift keying constellation as a function of the output mean photon number τ n ¯ for several values of the nonlinearity ϰ .
Fig. 6.
Fig. 6. Attainable squeezing ( Δ x ^ θ ) 2 for the input mean photon number n ¯ = 10 8 and several different values of the transmission τ as a function of the dimensionless nonlinear coefficient ϰ . For convenience, the abscissa is parameterized with sinh r = 2 ϰ ( log τ ) τ n ¯ . Dashed horizontal lines correspond to the estimate ( 1 τ ) / 3 .

Tables (1)

Tables Icon

Table 1. Exemplary Combinations of Optical Fiber and Pulse Parameters that Give the Value of the Dimensionless Nonlinearity Parameter ϰ = 5 × 10 6

Equations (36)

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d ϱ ^ d z = i μ [ n ^ 2 , ϱ ^ ( z ) ] + α 2 ( 2 a ^ ϱ ^ ( z ) a ^ n ^ ϱ ^ ( z ) ϱ ^ ( z ) n ^ ) ,
ϱ ^ ( z ) = exp ( i μ z n ^ 2 ) ϱ ^ ( z ) exp ( i μ z n ^ 2 ) .
d ϱ ^ d z = α 2 ( 2 a ^ ( z ) ϱ ^ ( z ) [ a ^ ( z ) ] n ^ ϱ ^ ( z ) ϱ ^ ( z ) n ^ ) ,
| ζ 0 = e n ¯ / 2 n = 0 ζ 0 n n ! | n .
ϱ mn ( z ) = ζ 0 m ( ζ 0 * ) n m ! n ! e ( m + n ) α z / 2 c m n ( z ) .
ϱ m n ( z ) = m | τ ζ 0 τ ζ 0 | n exp [ n ¯ f τ ( ( m n ) ϰ ) ] .
f τ ( ϰ ) = 1 τ 1 τ 1 2 i ϰ 1 2 i ϰ .
f τ ( ϰ ) 2 i ( 1 τ + τ log τ ) ϰ + [ 4 2 τ 2 τ ( 1 log τ ) 2 ] ϰ 2 .
m , n = 0 | m n | m | ζ ζ | n exp [ i ( m n ) ϕ 0 ( m n ) 2 σ 2 2 ] = d ϕ 1 2 π σ 2 e ( ϕ ϕ 0 ) 2 / 2 σ 2 | e i ϕ ζ e i ϕ ζ | .
ϕ 0 = 2 ϰ n ¯ ( 1 τ + τ log τ ) ,
σ 2 = 4 ϰ 2 n ¯ [ 2 τ τ ( 1 log τ ) 2 ] .
χ = S ( 0 2 π d ϕ p ϕ ϱ ^ ϕ ) 0 2 π d ϕ p ϕ S ( ϱ ^ ϕ ) .
ϱ ^ G = d ϕ 1 2 π σ 2 e ϕ 2 / 2 σ 2 | e i ϕ ζ e i ϕ ζ | .
d a ^ d z = i μ [ n ^ 2 , a ^ ( z ) ] = i μ [ 2 a ^ ( z ) a ^ ( z ) + 1 ] a ^ ( z ) .
a ^ ( z ) = e i μ z ( 2 ζ 2 + 1 ) e i ϕ [ ζ + b ^ ( z ) ] ,
d b ^ d z = 2 i μ ζ 2 [ b ^ ( z ) + b ^ ( z ) ] ,
b ^ ( z ) = ( 1 + 2 i μ z ζ 2 ) b ^ ( 0 ) + 2 i μ z ζ 2 b ^ ( 0 ) .
q ^ = e i μ z ( 2 ζ 2 + 1 ) a ^ ( z ) + h.c. = e i ϕ [ ζ + b ^ ( z ) ] + h.c. ,
p ^ = i e i μ z ( 2 ζ 2 + 1 ) a ^ ( z ) + h.c. = i e i ϕ [ ζ + b ^ ( z ) ] + h.c. ,
q ^ = 2 ζ cos ϕ , p ^ = 2 ζ sin ϕ
q ^ 2 = 1 + 4 ζ 2 cos 2 ϕ 4 μ z ζ 2 sin 2 ϕ + ( 4 μ z ζ 2 ) 2 sin 2 ϕ ,
p ^ 2 = 1 + 4 ζ 2 sin 2 ϕ + 4 μ z ζ 2 sin 2 ϕ + ( 4 μ z ζ 2 ) 2 cos 2 ϕ
1 2 ( q ^ p ^ + p ^ q ^ ) = 2 ζ 2 sin 2 ϕ + 4 μ z ζ 2 cos 2 ϕ 8 ( μ t ζ 2 ) 2 sin 2 ϕ .
cos ϕ = e σ 2 / 2 , cos 2 ϕ = e 2 σ 2 .
( Δ q ^ ) 2 = 1 + 2 ( 1 e σ 2 ) 2 ζ 2 + 2 ( 1 e 2 σ 2 ) sinh 2 r ,
( Δ p ^ ) 2 = 1 + 2 ( 1 e 2 σ 2 ) ζ 2 + 2 ( 1 + e 2 σ 2 ) sinh 2 r ,
1 2 ( Δ q ^ Δ p ^ + Δ p ^ Δ q ^ ) = 2 e 2 σ 2 sinh r .
tan 2 θ = sinh r sinh 2 r + ζ 2 ( e σ 2 1 ) ,
( Δ x ^ θ ) 2 = 1 + 2 ζ 2 ( 1 e σ 2 ) + 2 sinh 2 r 2 e 2 σ 2 sinh 2 r + [ sinh 2 r + ζ 2 ( e σ 2 1 ) ] 2 .
g ( τ ) = 2 τ τ ( 1 log τ ) 2 τ ( log τ ) 2 1 3 ( 1 τ ) ,
( Δ x ^ θ 0 ) 2 = e 2 r + ( Δ p ) exc 2 sin 2 θ 0 = e 2 r + g ( τ ) ( 1 e 2 r ) tanh r .
d ϱ ^ d z = α 2 ( 2 a ^ ( z ) ϱ ^ ( z ) [ a ^ ( z ) ] n ^ ϱ ^ ( z ) ϱ ^ ( z ) n ^ ) ,
d ϱ m , n d z = α 2 [ 2 ρ m + 1 , n + 1 ( z ) ( m + 1 ) ( n + 1 ) e 2 i μ z ( m n ) ρ m , n ( z ) ( m + n ) ] .
d c j d z = α n ¯ e α z e 2 i μ z j c j ( z ) .
c j ( z ) = exp ( n ¯ α α 2 i μ j e α z e 2 i μ z j + A 0 ) = exp ( n ¯ τ 1 2 i ϰ j τ 2 i ϰ j + A 0 ) ,
ϱ m n ( z ) = ( τ ζ 0 ) m ( τ ζ 0 * ) n m ! n ! exp ( n ¯ τ 1 2 i ϰ ( m n ) 1 2 i ϰ ( m n ) + A 0 ) .
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