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Broadband Electronic Two-Dimensional Spectroscopy in the Deep UV

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Abstract

We developed an all-reflective fully-noncollinear setup for two-dimensional electronic spectroscopy in the broadband UV (2DUV) with great phase stability (Λ/150) and applied it to the UV-chromophores dissolved in ethanol using 8-fs UV-pulses, generated in the 245-300 nm range. We are able to resolve 2D-spectra in the ~6000 cm−1 spectral window.

© 2014 Optical Society of America

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