Nonlinear optical properties of oxygen-doped and photopolymerized C60

Steven R. Flom; R. G. S. Pong; F. J. Barloli; Z. H. Kafafi; A. M. Rao; A. M. Rao; P. C. Eklund; P. C. Eklund

International Quantum Electronics Conference
OSA Technical Digest (Optica Publishing Group, 1994),
paper QTuG4

Nonlinear optical properties of oxygen-doped and photopolymerized C₆₀

Steven R. Flom, R. G. S. Pong, F. J. Barloli, Z. H. Kafafi, A. M. Rao, and P. C. Eklund

International Quantum Electronics Conference 1994

Anaheim, California United States
8–13 May 1994
ISBN: 1-55752-342-8

From the session
Nonlinear Properties of Organics (QTuG)

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S. R. Flom, R. G. S. Pong, F. J. Barloli, Z. H. Kafafi, A. M. Rao, and P. C. Eklund, "Nonlinear optical properties of oxygen-doped and photopolymerized C60," in International Quantum Electronics Conference, J. Shah, C. Weiman, R. Freman, and J. Fujimoto, eds., Vol. 9 of OSA Technical Digest (Optica Publishing Group, 1994), paper QTuG4.

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Abstract

The interest in the nonlinear optical (NLO) properties of the fullerenes lies in their unique structure and symmetry. Our previous studies have focused on the NLO behavior of pristine films of the fullerenes in the near-infrared^1,2 and in the visible.³ Recently, C₆₀ has been polymerized by irradiation of oxygen-free films with visible and ultraviolet light.⁴ It was found that oxygen plays an important role in the photochemistry of C₆₀. In addition, we have recently reported on the photo-assisted diffusion of O₂ into solid C₆₀ as well as its photo-oxidation.^5,6 The present paper addresses the effect that altering the electronic and chemical structure of C₆₀ through photopolymerization or oxygen doping has on the NLO properties and the dynamics of the NLO response.

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