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Optica Publishing Group
  • European Quantum Electronics Conference
  • Technical Digest Series (Optica Publishing Group, 1994),
  • paper QThI6

Stimulated Raman adiabatic passage with pulsed lasers for coherent high-resolution ion dip spectroscopy of molecules

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Abstract

The coherent interaction of narrowband Fourier-transform limited nanosecond laser pulses with gas phase molecular systems has attracted increasing interest during the last years. It can lead to a nearly 100% population transfer efficiency from an initial to a final state in a lambda-type three-level system using the Stimulated Raman Rapid Adiabatic Passage (STIRAP) method.1 This high transfer efficiency cannot be explained by a rate equation approach often used in incoherent Stimulated Emission Pumping (SEP) experiments.

© 1994 IEEE

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