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Optica Publishing Group
  • Conference on Lasers and Electro-Optics/Pacific Rim 2007
  • (Optica Publishing Group, 2007),
  • paper TuB3_1

A theory of molecular high harmonic generation from coherently rotating molecules and interpretation of recent pump-probe experiments

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Abstract

A general theory of molecular high harmonic generation in intense femtosecond pump-probe experiments is presented. It provides explicit analytical expressions correlating the harmonic signals with the dynamical alignment of linear molecules. Recent experimental data from pump-probe experiments are analyzed and a unified interpretation of the diverse observations is given.

© 2007 IEEE

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