Abstract
High-order harmonic generation (HHG) from nonadiabatically aligned molecules has been demonstrated to have new abilities to probe molecular dynamics and structures with femtosecond (fs) temporal resolutions [1-4]. In the recent study of HHG from coherently rotating molecules, the present authors have shown that HHG properties strongly depend on the degree of molecular alignment, and a low rotational temperature Trot and resulting high degree of alignment is strongly desired in the HHG experiment to retrieve the image of electronic distribution or orbital structure in a molecule [3].
© 2009 IEEE
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