Abstract
Theoretical research on opto–mechanical interactions at sub–wavelength levels using surface waves (SWs) excitation has a great impact in both the academic knowledge and practical realm. In this letter we have revealed that the dynamic characteristics of the SWs excited along a metamaterial boundary, such as its forward or backward propagation nature, provide a direct demonstration about the direction of action of the optical force exerted on a dielectric nano–particle. In particular, by using a rigorous electromagnetic formalism based in the second Green identity, we have modeled the scattering problem of a Gaussian beam impinging on a metamaterial plane surface with a sub–wavelength localized defect. We have shown that depending on the nature of the excited SW, dielectric nano–particles placed near the surface can be pushed away or towards the localized defect. We believe that this work unveils the potential implementation of sub–wavelength defects as sources of pushing or pulling optical forces.
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1. Introduction
Due to the unique property of high confinement that allowed optics to develop at sub–wavelength level, excitation of surface waves (SWs) –electromagnetic waves propagating along the interface between media with opposite signs of their permittivities or permeabilitties– became a subject of great interest in science applications. The vast majority of research in the last century was focused on SWs with $p$ polarization, taking place in the visible range, that occurs at the interface separating a conventional dielectric medium, such as an insulator medium with positive permittivity, from a metallic medium, with negative permittivity [1].
Perhaps one of the most interesting applications of metallic SWs refers to the optical control of the movement of nano–particles by exchanging momentum with light. Since the propagation constant of the SW at the insulator–metal interface is grater than that of the photon in the insulator medium, where the nano–particle is placed (usually vacuum or water), the momentum imparted to the nano–particle by its interaction with SWs results in a huge kick when compared to that provided by the photon. Such is the case of the pulling force, a force that pull the particle in the opposite direction as that of the incident photons, exerted on dielectric nano–particles placed near a metallic interface arising from the excitation of metallic SWs [2,3].
Possibilities have been broadened with the advent of metamaterials, synthetic composite material exhibiting electromagnetic properties not usually found in natural materials, where new optomechanics effects, as light induced levitation or strong optical pulling forces achievement, have been demonstrated [4–6]. In particular, transparent metamaterials with negative index of refraction (NIR) at the low–frequency spectrum, i.e., both permittivity and permeability with a negative real part in the terahertz (THz) and infrared (IR) region, have expanded the possibilities of having SWs not only with $p$ but also with $s$ polarization at these frequency ranges. In particular, NIR materials have stimulated a revived interest in the electromagnetic properties of SWs, and novel characteristics that do not exist in conventional media, such as backward behavior, with a total energy flux parallel to the interface, that is opposed to the phase velocity, have been reported in several works [7,8]. This property has been recently harnessed for optical surface tractor beams employing NIR materials [9].
In the present work, we propose the theoretical idea of a single localized defect on a plane NIR interface working as a source that is able to provide optical pulling or pushing force on dielectric nano–particles placed near the NRI interface. Interestingly, in case of the pulling source, the mechanism for which the particles are moved in the source direction in the present work is different from that used in Refs. [2,10,11], where the pulling force arises from the interaction between the circularly polarized dipolar moment induced on the nano–particle and the surface modes on the surface which can be excited by the near field scattering [12]. On the contrary, here, the direction of the force towards the source results by the electromagnetic pressure exerted on the nano–particle placed into the dielectric medium (vacuum in our simulations) and the excitation of backward SWs on the surface.
2. Theory
In order to demonstrate the above, we consider a localized defect with translation symmetry along an axis (the $y$ axis in our coordinate system) which scatters the impinging light on the flat NRI surface containing the defect (Fig. 1). The medium above the surface, where the dielectric nano–particles are placed, is vacuum ($\varepsilon _1=\mu _1=1$) and the constitutive parameters of the NRI medium are $\varepsilon _2$ and $\mu _2$, both with negative real part. The illumination is fulfilled by a Gaussian beam which is pointing in the direction of the center of the surface defect, $x=z=0$ in our coordinate system, $\phi _i(x,z)=e^{-(x \cos \phi _0 + z \sin \phi _0)^2/w^2}e^{ik_0(x \sin \phi _0-z \cos \phi _0)}$, where $\phi _i(x,z)$ is the $y$–directed component of the total magnetic field ($p$ polarization) or the total electric field ($s$ polarization), $w$ is half of the beam width at the waist, $\phi _0$ is the angle of incidence of the beam defined with respect to the $z$ axis, $\omega$ is the angular frequency and $c$ is the speed of light in vacuum. The solution $\phi (x,z)$ of Maxwell’s equations in the region $z>h$ can be written as
The novelty of this work is the theoretical demonstration of a tractor source, for which the momentum and energy carried by the scattered light in vacuum points out towards the object. To achieve this situation, and in order to avoid an energy sink at the position of the object (the surface defect in this work), it is necessary to have another channel where the energy flows in the opposite direction, i.e., away from the object and such that the nano–particle cannot access to it. This is the scheme proposed in the present work.
In our calculations, we have considered two kind of metamaterial boundaries, one of them supporting $p$–polarized forward SWs and the other $p$–polarized backward SWs. For clarity, we have chosen the NRI constitutive parameters so that the phase velocity of forward and backward SWs aproximately match. In the first case (case I), $\varepsilon _2=-1.3+i 0.01$, $\mu _2=-0.35+i 0.01$, which leads to a normalized propagation constant $\kappa _{sw}=k_x/k_0=1.337+i 0.02$. In the second case (case II), $\varepsilon _2=-0.8+i 0.01$, $\mu _2=-1.6+i 0.01$, which leads to a normalized propagation constant $\kappa _{sw}=1.332-i 0.0379$. Note that in the first case the sign of the imaginary part of the propagation constant is equal to that of the real part, meaning that the SW phase velocity is in the same direction as the energy flow (forward SW). On the contrary, in the second case, the sign of $\Im \,\kappa _{sw}$ is opposed to that of the $\Re \,\kappa _{sw}$, meaning that the phase velocity is in the opposed direction as the energy flow (backward SW).
3. Results
In order to find the value of the force acting on the nano–particle along the $x$ axis, we assume that the radius $a$ of the particle is smaller than SW and photon wavelengths, $a \ll \lambda _{sw} = \lambda /\Re \,\kappa \approx \lambda /1.3$ (the photon wavelength in vacuum is $\lambda =2\pi c/\omega$). In this framework, the time average of the force acting on a single particle located at the position $\mathbf {r}$ is written as [14],
In all the examples presented here we have calculated the normalized force with respect to the electromagnetic pressure on the same nano–particle exerted by a plane wave propagating along the $x$ direction whose amplitude coincides with that of the Gaussian beam at the center of it, i.e., $f=F_x/F_{ph}$ where $F_{ph}=0.5 \, k_0\,\Im { \alpha _0}\,|\mathbf {E}_{ph}|^2$, $\mathbf {E}_{ph}=\sqrt {\frac {\mu _0}{\varepsilon _0} } \phi _{inc}(0,0) \, e^{i \, k_0 \, x}\, \hat {z}$ and $\varepsilon _0,\,\mu _0$ are the vacuum permittivity and permeability, respectively.
In Fig. 2 we have plotted the dependence on the $x$ axis of the normalized optical force $f$ exerted on a dielectric nano–particle (radius $a=0.01\lambda$ and dielectric permittivity $\varepsilon _p=2.25$) near the surface with a protuberance $g(x)=\mbox {rec}(x/d) \, h\,[1+\cos (2\pi \,x/d)]$ ($\mbox {rec}(u)$ is the rectangular function centered at the origin with unit width and height), which represent the pulling or pushing source, with $d=\lambda$ and height $h=0.125\lambda$. The vertical position of the particle has been set at $z'=0.125\lambda$ and $z'=0.250\lambda$. The illumination is accomplished by a Gaussian beam of width $w=5\lambda$. In case I, corresponding to the excitation of forward SWs, the force has the same sign as the $x$ axis, i.e., $F_x>0$ for $x>0$ and $F_x<0$ for $x<0$. This fact means that the protuberance behaves as a pushing source. We observe that the force curve has a periodic behavior along the $x$ axis with a period $\Lambda =0.77\lambda$ gradually attenuating with the increasing distance $|x|$, with a decay length $\delta \approx 8 \lambda$. The value of the period coincides with that of the SW wavelength $\lambda _{sw}=\lambda /\kappa _{sw} \approx 0.76 \lambda$, whereas the decay length coincides with that of the SW, $\delta =\lambda /(2\pi \,\Im \,\kappa ) \approx 7.95 \lambda$. These facts make clear that the main contribution to the optical force pushing the nano–particle away from the protuberance is due to the SW field.
On the other hand, from Fig. 2 we see that for case II, corresponding to backward SWs excitation, the optical calculation force values are negative (positive) for $x>0$ ($x<0$). This fact can be understood by taking into account the fact that in backward SWs the sign of the real part of the propagation constant is opposite to the corresponding imaginary part. As a consequence, the energy carried by the backward SW is opposite to its direction of propagation. As the energy must attenuate, the exponential SW decay is in the same direction as the total energy flow, that is, the imaginary part of the propagation constant must be positive for $x>0$ and negative for $x<0$. Therefore, for $x>0$ is $\Re \,\kappa _{sw}<0$ , and for $x<0$ is $\Re \,\kappa _{sw}>0$. From the above discussion it follows that the SW field pushes the nano–particle towards the protuberance behaving as a tractor source. The force curves also show a periodic spatial dependence along the $x$–direction, $\Lambda =\lambda /\Re \,\kappa _{sw} \approx 0.75\lambda$ gradually attenuating with the increase of $|x|$, with a decay length $\delta =\lambda /(2\pi \,\Im \kappa _{sw}) \approx 4.2 \lambda$ owing to losses arising from absorption in the NRI medium.
In addition, in Fig. 2 (inset at the right side) we have plotted the modulus of the complex reflection coefficient $|R|$ as a function of the normalized wave–vector $\kappa$. In the radiative zone, $|\kappa |<1$, the curves show a central peak at $\kappa =0$ representing the wave reflected by the planar interface (without the protuberance). The protuberance is manifested by the presence of the peaks outside the radiative zone, $|\kappa |>1$. These peaks are centered at $\kappa \approx \pm 1.3$ and represent the SWs excited by the scattering of the incident field with the protuberance.
To add a physical insight, one can estimate quantitatively the SW component of the optical force as follows. Since the main contribution to the integral (1) is provided by the SW excitation (see inset at the right in Fig. 2), it follows that the near field can be approached by their contributions. To do this, one should take into account the forward or backward character of the excited SW since physical causality requires the attenuation of the field as $|x| \longrightarrow \infty$. From the above discussion, it follows that for $x>0$, the SW field can be approximately by the following expression,
for forward SW excitation, whereas for backward SW excitation is, where $A(\kappa _{sw})$ can be calculated as $2\pi i$ times the residue of the complex amplitude $R$, $\lim _{\kappa \longrightarrow \kappa _{sw}} (\kappa -\kappa _{sw})\,R(\kappa )$, or by integrating Eq. (1) into a bandwidth $\Re \,\kappa$ that embraces the whole resonant peak, i.e., $A=\int _{\Re \,\kappa _{sw}-\Delta _{\kappa }/2}^{\Re \,\kappa _{sw}+\Delta _{\kappa }/2} \, R(\kappa ) \,d\kappa$ with $\Delta _{\kappa }$ embracing the resonant peak at $\pm \Re \kappa _{sw}$ [12,15]. From Eqs. (3), (4) and Maxwell–Ampere, we calculate the electric field $\mathbf {E}_{sw}$ and deduce an expression for the SW contribution to the optical force (2) for $x>0$,In Fig. 3 we have plotted the optical force (2) for various values of the half of the beam width, $w=5\lambda,2.5\lambda, \lambda$ together with the SW contribution calculated with Eq. (5). We observe that the spatial variations on these curves are appreciable in the interval defined from $-w$ to $w$. This fact is due to the interference process between the specular reflected beam and the SWs excited by the near field scattered by the protuberance. We also observe that the SW contribution curve falls in the middle of the oscillation of those corresponding to the total force calculated with our rigorous integral method. Similar results, not showed here, have been obtained for the forward SWs excitation.
Next, we study the dependence with the angle of incidence $\phi$. From Fig. 4(a) and 4(b) we see that for forward (backward) SWs excitation, the force values are increased for $x>0$ ($x<0$) as the angle of incidence is increased. In addition, the force values are remarkably reduced in the opposite side, i.e., on the $x<0$ region for forward SW excitation and on $x>0$ region for backward SW excitation. This fact can be understood by means of the reflectivity plots shown in Fig. 4(c) and 4(d), where we see that the amplitude $R(\Re \kappa _{sw})$ increases with the increment of $\phi$, whereas the amplitude $R(-\Re \kappa _{sw})$ decreases with $\phi$, thus, the excited SWs with propagation constant $+\kappa _{sw}$ are strongly excited with respect to that with $-\kappa _{sw}$. As a consequence, from Eqs. (3) and (4) we see that the near field, and thus the SW contribution to the optical force (5), are increased on the right side $x>0$ for forward SW excitation and on left side $x<0$ for backward SW excitation. We also observe an asymmetry, which is more noticeable as the angle of incidence increases, in the period of the optical force at both sides of the protuberance. The occurrence of this asymmetry arise in the interference between the incident (and reflected field) and the SWs excited in the process [8]. The period can be roughly estimated in the limit of planar wave incidence, i.e., by assuming an incident plane wave ($w=\infty$) with wave–vector component parallel to the interface $k_{inc}=k_0\,\sin \phi _0$. Therefore, since the angle of incidence is grater than zero, $\phi _0>0$, the periods of the near field at both sides of the protuberance, for forward SW excitation, are $d_>=2\pi /|k_{inc} - k_0\kappa _{sw}|=\lambda /|\sin \phi _0-\kappa _{sw}|$ for $x>0$ and $d_<=2\pi /|\sin \phi _0+\kappa _{sw}|$ for $x<0$. On the contrary, for backward SW excitation, the periods are: $d_>=2\pi /|\sin \phi _0+\kappa _{sw}|$ for $x>0$ and $d_<=2\pi /|\sin \phi _0-\kappa _{sw}|$ for $x<0$. For example, for backward SW excitation, from Fig. 4 we obtain $d_< \approx 0.772 \lambda,\,0.926\lambda,\,1.112\lambda$ for $\phi =5,\,15,\,30^\circ$, respectively, whereas the corresponding calculated values are: $d_< \approx 0.803 \lambda,\,0.9318\lambda,\,1.201\lambda$. We have verified, not shown here, that the calculated values using the plane wave incidence limit converge to those rigorously obtained for values large enough of half beam width $w$ ($w>10\lambda$).
4. Conclusion
In conclusion, we have analyzed the scattering process for which a metamaterial planar boundary including a sub–wavelength protuberance behaves like a pushing or pulling beam source. Our results shown that the main character in this phenomenon are the SWs existing on the metamaterial boundary and their dynamic characteristics that provide the pulling or pushing optical force. By modifying the angle and the width of the incidence Gaussian beam, one can handle the force level at both sides of the protuberance and the spatial length of the fluctuation due to the interference between the reflected field by the plane metamaterial boundary (without any defect) and the SW generated by the scattering of the near field with the protuberance. The knowledge developed in this work could be interesting towards the development of pulling beam sources based on surface waves excitation.
Funding
School of Engineering of Universidad Austral (O04-INV0 0 020).
Acknowledgments
We acknowledge the financial supports of Universidad Austral O04-INV0 0 020, Agencia Nacional de Promoción de la Investigación, el desarrollo Tecnológico y la Innovación PICT-2020-SERIEA-02978 and Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET).
Disclosures
The authors declare no conflicts of interest.
Data availability
Data underlying the results presented in this paper are not publicly available at this time but may be obtained from the authors upon reasonable request.
Supplemental document
See Supplement 1 for supporting content.
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