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Injection-seeded high-power Yb:YAG thin-disk laser stabilized by the Pound-Drever-Hall method

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Abstract

We demonstrate an injection-seeded thin-disk Yb:YAG laser at 1030 nm, stabilized by the Pound-Drever-Hall (PDH) method. We modified the PDH scheme to obtain an error signal free from Trojan locking points, which allowed robust re-locking of the laser and reliable long-term operation. The single-frequency pulses have 50 mJ energy (limited to avoid laser-induced damage) with a beam quality of M2 < 1.1 and an adjustable length of 55-110 ns. Heterodyne measurements confirmed a spectral linewidth of 3.7 MHz. The short pulse build-up time (850 ns) makes this laser suitable for laser spectroscopy of muonic hydrogen, pursued by the CREMA collaboration.

© 2023 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement

1. Introduction

Thin-disk lasers (TDL) are well known for their high power and energy output at very good beam quality. High average power systems with close to diffraction limited beam quality and pulse durations from nanoseconds to femtoseconds are commercially available and a large variety of high-energy and high-intensity systems have been demonstrated [17]. While high-energy single transverse mode operation in TDLs is well established, high-energy single axial mode operation (i.e., single-frequency operation) is rarely pursued. Some projects using Yb:YAG are worth noting [812] but the vibrations caused by the impingement cooling of the disk make stable single-frequency operation in these high-power systems challenging.

In this paper we present an injection-seeded, Q-switched 1030 nm Yb:YAG TDL. Prior to trigger, a narrow-bandwidth CW seed laser is resonantly coupled into the TDL resonator, so that only a single axial mode is initially populated by the seed laser. The resulting high-energy pulse building up in the TDL is thus also narrow-bandwidth ("single-frequency"). Resonant injection of the seed light was achieved by stabilizing the TDL resonator length with the Pound-Drever-Hall (PDH) method [13,14], and we achieved close to time-bandwidth limited pulses with energies over 50 mJ in $\text {TEM}_{00}$ mode, 55 ns pulse duration and < 5 MHz bandwidth. We reached pulse repetition rates up to 1 kHz at 14 mJ pulse energy. To the best of our knowledge, this is the first time a high-power TDL has been frequency-stabilized via the PDH-method, and the obtained single-frequency pulses have the highest energy to date.

In addition to delivering narrow bandwidth pulses, the here presented laser must fulfill a number of additional requirements, as it is part of the laser system used for the HyperMu experiment [15,16] currently pursued at the Paul Scherrer Institut in Villigen, Switzerland. In this experiment, the CREMA collaboration [1721] aims at the first laser spectroscopy measurement of the ground-state hyperfine splitting in muonic hydrogen. The laser system is based on a TDL delivering high-energy pulses at 1030 nm which are down-converted in a series of optical parametric oscillators (OPO) and optical parametric amplifiers (OPA) to the mid-IR region (around 6.8 µm) where the hyperfine transition (100 MHz linewidth at full width half maximum) is expected. For efficient and reliable multi-stage down-conversion, the TDL output beam must be diffraction limited, must have stable beam parameters (pointing and beam size), and must have small pulse-to-pule energy variation. Additionally, for the spectroscopy experiment, the bandwidth must be $\leq$ 10 MHz, calling for pulse lengths on the order of 50 ns, and the laser must deliver the pulse with a short latency after trigger (about 1 µs) owing to the muon lifetime of 2 µs.

The TDL technology was chosen mainly since it allows short pulse build-up times, large pulse energies and good beam quality, as shown in earlier work of our group [2225]. The design of our new TDL presented here is based on three key innovations: 1) A PDH-based injection-seeding process, modified so that the TDL resonator is locking correctly on resonance with the seed even after large perturbations [26]. This makes the injection-seeding process very robust. 2) Asymmetric closing and opening of the resonator to obtain Gaussian pulses. For this purpose the outcoupling of the TDL resonator is voltage controlled via a Pockels cell, of which we control both electrodes independently. 3) A feedback loop controlling the beam pointing to mitigate slow drifts, and a feed-forward system stabilizing the pulse energy on a pulse-to-pulse level by dynamically adjusting the pulse build-up time.

The paper is organized as follows: Section 2 describes the TDL resonator design. Section 3 describes the injection-seeding process and the Q-switching dynamics. Single-frequency operation is demonstrated in Section 4, and the overall laser performance is presented in Section 5.

2. Resonator design

The design of our TDL is based on the TDL that was employed in the laser spectroscopy of the muonic helium ion [20,24]. One of the main design criteria was to ensure output beam parameters insensitive to variations of the thermal lens of the thin-disk. Such stability can be achieved by setting up the resonator as a Fourier transform (FT) resonator, in which the mode undergoes an optical FT in one round-trip from disk to disk. Such a FT resonator has the round-trip ABCD matrix [27]

$$M_{\text{FT}}=\left(\begin{array}{cc} 0 & F\\ -\frac{1}{F} & 0 \end{array}\right),$$
where $F>0$ is the so-called Fourier parameter of the resonator. The resulting beam size of the $\text {TEM}_{00}$ eigenmode at the disk is given by [27]
$$w_0 = \sqrt{\frac{F\lambda}{\pi}},$$
with $\lambda$ being the laser wavelength (in our case $\lambda = 1030$ nm). For example, a resonator sustaining a mode with $w_0 = 2.1$ mm has $F=13.4$ m (it turns out that $F$ is precisely the Rayleigh length of the FT resonator eigenmode at the disk).

We realized the FT resonator as a telescopic resonator in a V shape with the disk at the tip of the V as shown in Fig. 1. This configuration reduces the pulse build-up time for two reasons: the Galilean telescope shortens the physical propagation length of the resonator while the V-shape doubles the number of passes over the disk per round-trip. The disk (thickness: 275 µm, Yb-doping: 7 at. %) is continuously pumped at 969 nm (zero-phonon line) with about 350 W and water-cooled from the back side. The pump spot diameter is set to $d_\text {P} = 5.8$ mm to ensure efficient energy transfer from the disk to the laser mode. A quarter-wave plate is placed in front of the disk to suppress spatial hole-burning as detailed in [28].

 figure: Fig. 1.

Fig. 1. Schematic of the injection-seeded thin-disk oscillator. HV: high-voltage, PC: Pockels cell, TFP: thin-film polarizer, FR: Faraday rotator, PD: photodiode, PDH lock: Pound-Drever-Hall locking scheme, $\updownarrow$: P-polarization, $\odot$: S-polarization, $\mathrm {\lambda }$/2: half-wave plate, $\mathrm {\lambda }$/4: quarter-wave plate. The resonator is spanning between end-mirrors $\text {M}_1$ and $\text {M}_2$. The PC-$\mathrm {\lambda }$/4-TFP system forms a HV controlled outcoupler steering the Q-switching dynamics of the oscillator. Through this TFP the seed laser output is injected into the resonator prior to trigger, and the pulses are extracted from the oscillator after pulse-buildup. Resonant coupling of the seed laser light into the oscillator is achieved through a PDH-locking scheme acting on the resonator length. The resonator alignment is stabilized via an autoalignment system including the quadrature photodiode $\text {PD}_\text {A}$ and two piezos steering the alignment of mirror "cav". The pulse energy is stabilized via a feed-forward system including the photodiode $\text {PD}_\text {E}$ and a delay box adjusting the pulse build-up time.

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In contrast to our earlier FT resonator [22,24], we used a quasi flat disk with focal length $f_\text {D} \approx 10$ m instead of a curved disk (which is often employed in telescopic thin-disk lasers). The disk is thus not part of the telescope, and an additional concave mirror must be introduced. A round-trip in the resonator follows the propagation (see Fig. 1 and Fig. 2)

$$\text{M}_{1}~\overset{d_{0}}{\text{ - }}\text{ disk }\overset{d_{1}}{\text{ - }}\text{ cav }\overset{d_{2}}{\text{ - }}\text{ vex }\overset{d_{3}}{\text{ - }}~\text{M}_{2}~\overset{d_{3}}{\text{ - }}\text{ vex }\overset{d_{2}}{\text{ - }}\text{ cav }\overset{d_{1}}{\text{ - }}\text{ disk}\overset{d_{0}}{\text{ - }}~\text{M}_{1},$$
where cav and vex stand for the concave and a convex mirror with focal lengths $f_\text {cav}$ and $f_\text {vex}$, respectively. The flat end-mirrors are denoted $\text {M}_{1}$ and $\text {M}_{2}$, and the mirror spacings are defined as $d_0$, $d_1$, $d_2$ and $d_3$.

 figure: Fig. 2.

Fig. 2. Beam radius (1/$\text {e}^2$) of the $\text {TEM}_{00}$ mode along the TDL resonator for variations of the disk dioptric power $\Delta V$. For simplicity the location of folding mirror $\text {M}_\text {fold}$ is not shown.

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Since the beam is large and collimated between end-mirror $\text {M}_1$ and the disk, $d_0$ can be chosen arbitrarily (as long as $d_0$ is much smaller than the Rayleigh length of the eigenmode in this part of the resonator) and thus does not enter the calculations. The distance $d_1$ between disk and concave mirror was chosen as a compromise between short propagation and small incidence angle on the concave mirror to mitigate astigmatism. Finally, the remaining degrees of freedom $d_2$ and $d_3$ are determined by matching the ABCD round-trip matrix of the resonator to the FT matrix (1). Solving the equations (see appendix A) leads to

$$d_2 = f_\text{vex} + \frac{F \left( f_\text{D} - d_1 \right) }{ F - f_\text{D} - \xi \left( F - f_\text{D}\right) + F f_\text{D}/f_\text{cav}} + d_1 \frac{f_{\text{D}}}{F -f_{\text{D}} - \xi \left( F - f_{\text{D}} \right) + F f_{\text{D}}/f_{\text{cav}}},$$
$$d_3 = f_{\text{vex}} + \frac{F f_\text{vex}^2}{2} \left[ \frac{1}{f_{\text{D}^2}} - \frac{1}{F^2} + \frac{1}{f_{\text{cav}}^2} \right] \left( 1-\xi \right)^2 + F \left( \frac{f_{\text{vex}}}{f_\text{cav}}\right)^2 \left[ \left( \xi + \frac{f_{\text{cav}}}{f_{\text{D}}} \right) \left( 1-\xi \right) + \frac{1}{2} \xi^2 \right],$$
where we defined the parameter $\xi = d_1/f_{\text {cav}}$.

If a sufficiently curved disk is used, the concave mirror is not required so that $f_\text {cav}\rightarrow \infty$ and $d_1\rightarrow 0$, with $\xi \rightarrow 0$. Thus, Eq. (4) & Eq. (5) simplify to

$$d_2 \rightarrow f_\text{vex} + \frac{f_\text{D} F}{F-f_\text{D}}$$
and
$$d_3 \rightarrow f_\text{vex} + \frac{F}{2}\left[ \left(\frac{f_\text{vex}}{f_{\text{D}}}\right)^2 - \left( \frac{f_{\text{vex}}}{F} \right) ^2 \right].$$

The chosen values for all focal lengths and propagation distances are given in Table 1. Figure 2 illustrates the simulated beam size in the TDL resonator for the nominal focal power of the disk (black solid line). It also depicts the sensitivity of the mode in case of thermal lensing where the disk picks up an additional focal power of $\Delta V = \pm 0.02 \ \text {m}^{-1}$ (blue and red curves, respectively).

Tables Icon

Table 1. Resonator parameters.

Both injection of the seed laser and pulse extraction are occuring through the thin-film polarizer (TFP) located between end-mirror $M_1$ and the disk where the influence of a varying thermal lens on the resonator mode is minimal. Indeed, in this region of the resonator, small variations $\Delta V$ lead to a relative change in mode size [27] of

$$\frac{w}{w_0} = 1 + \frac{1}{4} F^2 \Delta V^2 + \frac{5}{32}F^4 \Delta V^4 + \ldots,$$
where $w_0$ is the mode size for the nominal value of $f_\text {D}=f_\text {nom}$ and $w$ is the mode size for $1/f_\text {D} = 1/f_\text {nom} \pm \Delta V$. The quadratic dependence of $w$ on $\Delta V$ results in stability against small variation of $\Delta V$ for both the pulse extraction and the seed incoupling.

An additional advantage of incoupling the seed through the TFP is that the reflectivity of the TDL resonator can be adjusted to optimize the PDH error signal. This greatly simplifies the commissioning of the laser and optimization of the PDH locking-system.

The seed is protected from the intense laser pulses by two optical isolators consisting of TFPs and Faraday rotators (FR) as well as an internal isolator in the seed laser module. Q-switching of the TDL is performed by varying the resonator losses with the standard combination of a TFP, a quarter-wave plate and a Pockels cell (PC), denoted as TFP-$\lambda /4$-PC (see Subsec. 3.2).

3. Experimental setup

3.1 Pound-Drever-Hall stabilized resonator length

Prior to a laser trigger, the TDL resonator is populated with seed laser photons (i.e. injection-seeded) by stabilizing the resonator length to the seed laser (Toptica DLPro, wavelength: 1030 nm, linewidth: 50 kHz (5 µs), nominal power: 200 mW) frequency via PDH locking. We use a modified PDH-scheme that guarantees automatic locking on resonance even after large perturbations [26]. This is achieved by modulating the phase of the seed laser light at half the free spectral range (FSR) of the TDL resonator to obtain the error signal shown in Fig. 3. This error signal has only one zero crossing between two neighboring resonances and is thus free from "Trojan" lock points [26]. This allows the servo-controller to always re-lock the TDL resonator correctly on resonance. Since the frequency of the intra-resonator light is defined by the seed laser frequency, it does not matter on which resonance the TDL is stabilized.

 figure: Fig. 3.

Fig. 3. (a) Typical open-loop PDH-error-signal measured with photodiode $\text {PD}_\text {PDH}$ in Fig. 1 obtained by scanning the resonator length. The modulation frequency of the seed laser is 40 MHz, i.e., half the free spectral range of the resonator. (b) Corresponding $\text {TEM}_{00}$ intra-resonator intensity measured with $\text {PD}_\text {I}$. As the resonator length is scanned, the side bands are also visible at $\pm 40$ MHz.

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The seed laser is sinusoidally current-modulated at $f_\text {M} = 40$ MHz by using one channel of a function generator (Tektronix AFG1062). The second channel, a copy of the modulation signal, is used as reference (local oscillator) for demodulation in the PDH scheme. The phase delay between modulation signal and reference can be continuously tuned by adjusting the relative phase between the two channels directly on the function generator.

The reflected light used for the PDH-lock is detected as leakage light through a 45$^{\circ }$ high-reflective mirror by the fast photodiode denoted $\text {PD}_\text {PDH}$ in Fig. 1. During pulse extraction, $\text {PD}_\text {PDH}$ saturates so that the lock is not functional for ca. $40$ µs after pulse extraction [26]. Once the photodiode has recovered, the resonator always re-locks correctly on resonance to the seed frequency thanks to our modified PDH scheme and is immediately ready for the next trigger.

3.2 Q-Switching dynamics

The time-dependent effective (power) reflectivity $R_\text {out}(t)$ of the system TFP-$\lambda /4$-PC can be calculated via the Jones vector formalism (see appendix B) as

$$\begin{aligned} R_\text{out}(t) &= \left| \cos\left( 2\pi \frac{\Delta U(t)}{U_{\lambda/4}}\right)\cos\left( 2\alpha \right) -\frac{1}{2}\sin\left( 2\pi \frac{\Delta U(t)}{U_{\lambda/4}}\right)\sin\left( 4\alpha \right) \right.\\ &\quad \left. + i \cdot \sin\left( 2\pi \frac{\Delta U(t)}{U_{\lambda/4}}\right)\sin\left( 2\alpha \right) \right|^2 \end{aligned}$$
where $\alpha$ is the rotation angle of the quarter-wave plate, $\Delta U(t) = U_1(t) - U_2(t)$ is the voltage difference between the two electrodes holding the BBO crystal of the PC in place, and $U_{\lambda /4}$ is the quarter-wave voltage of the PC.

A typical switching sequence is illustrated in Fig. 4. Initially, $U_1=U_2=0$ V, and the $\lambda /4$-plate is rotated so that $R_\text {out}(t<0) \approx 50$ % to allow seed incoupling while keeping the losses high enough to prevent pulse build-up. The TDL is PDH-stabilized in this state, and the intra-resonator power amounts to ca. 0.5 W. At $t=0$ the HV-switch to electrode E1 is closed so that $U_1 = 8$ kV builds up in about 10 ns. This results in $\Delta U = 8$ kV and the resonator is closed with $R_\text {out} \approx 100$ %. The pulse builds up quickly from the axial mode populated by the seed laser. After a pre-defined pulse build-up time, electrode E2 is switched to $U_2 = 13$ kV, resulting in $\Delta U = -5$ kV and an outcoupling reflectivity of $R_\text {out} \approx 25$ %. After 2 µs the switches to E1 and E2 are opened and the electrodes discharge with a decay time $\tau \approx 500$ ns. Both electrodes are grounded so that $R_\text {out} \approx 50$ % is re-established. The TDL resonator length is stabilized again by the PDH lock and the laser is ready for the next trigger.

 figure: Fig. 4.

Fig. 4. (a) Effective reflectivity $R_\text {out}$ of the thin-disk laser resonator versus voltage difference $\Delta U$ across the BBO crystal in the Pockels cell. The dashed arrows indicate a switching sequence where the resonator is closed by switching the first electrode to $U_1=8$ kV and then opened by switching the second electrode to either $U_2=8$ kV (black, dashed) or $U_2=13$ kV (red, dashed). (b) Typical pulse shapes for the two switching sequences in a). The gray shaded area shows the envelope of 100 pulses and the solid lines their average. Both pulses have an energy of 25 mJ.

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By controlling $U_1$ and $U_2$ independently, a lower outcoupling reflectivity can be achieved compared to the case when both electrodes are switched with the same voltage. This results in pulses with shorter tails which are more suited for subsequent non-linear conversion. As shown in Fig. 4(b) the temporal pulse shape significantly varied with the opening voltage $U_{2}$. For lower values of $U_{2}$ (e.g. $U_{1}=U_{2}=8$ kV) the reflectivity of the resonator is higher during the outcoupling process, which leads to pulses with a longer tail. We were able to tune the FWHM pulse length between 55 ns and 110 ns by tuning $U_2$ from 13.5 kV to 8 kV. We limited $U_{2}$ to 13.5 kV to avoid damaging the HV switches.

3.3 Autoalignment and pulse energy stabilization

During operation slow drifts (over several hours) might misalign the TDL resonator. This not only reduces the pulse energy and beam quality, but also limits the pulse-to-pulse stability to around 2 % (RMS). We therefore installed an auto-alignment system controlling the horizontal and vertical tilt of the mirror "cav" in Fig. 1 via piezo-electric actuators. The error signal was obtained by monitoring the leakage light of the resonator-enhanced seed prior to a pulse through mirror $\text {M}_\text {fold}$ on a quadrant photodiode ($\text {PD}_\text {A}$) to stabilize the position of the laser beam at approximately the location of the disk.

The output pulse energy was further stabilized by monitoring the intra-resonator power during pulse build-up with a fast photodiode ($\text {PD}_{\text {E}}$ in Fig. 1). Once a pre-defined voltage level $V_{\text {max}}$ was reached, the PC was triggered to extract a pulse. To prevent laser-induced damage due to trigger failure, we set a maximal pulse build-up time after which the PC is switched regardless of the photodiode signal. The outcoupling time jitter introduced by this stabilization method is marginal since the pulse build-up time only changes logarithmically with the pulse energy (i.e. the intra-resonator signal).

4. Demonstration of injection-seeding and chirp measurement

4.1 Heterodyne measurement setup

We checked proper injection-seeding by performing heterodyne measurements from which the bandwidth of the TDL laser pulses could be determined, as well as their instantaneous frequency relative to the seed laser frequency. Following the scheme from [29] we extracted the relative frequency shift $\Delta \nu (t)$ between TDL laser pulses and seed via quadrature demodulation of a heterodyne signal.

For the sake of brevity, we only sketch the experimental setup (see Fig. 5) and present the result (for details see [25,30]). The seed laser is current-modulated at $\nu _\text {M}=40$ MHz to lock the TDL to the seed laser with our modified PDH scheme. A fraction of the seed (10 %) is additionally phase modulated at $\nu _\text {EOM}=0.87$ GHz by a fiber-coupled EOM. This part is used to stabilize the seed laser frequency via a standard PDH lock on a Fabry-Perot (FP) cavity so that the blue sideband (at $\nu _\text {blue}=\nu _\text {seed}+\nu _\text {EOM}$) is always resonantly transmitted through the FP cavity. The transmitted blue sideband is superposed with the pulse from the TDL on a fast photodiode ($\text {PD}_2$ in Fig. 5). The beat note signal between the two beams recorded on this photodiode is high-pass filtered and sent to a quadrature demodulator board (ADL5387).

 figure: Fig. 5.

Fig. 5. Sketch of the optical setup used to generated the heterodyne signal. The dashed red line represents the laser pulses. The seed laser output is split into two branches. One branch injection-seeds the thin-disk laser oscillator with photons at a frequency $\nu _{\text {seed}}$. The other branch contains an EOM imprinting sidebands at $\nu _\text {seed}\pm \nu _\text {EOM}$. The blue side band is kept resonant with the Fabry-Perot (FP) cavity, so that only the frequency $\nu _\text {seed}+\nu _\text {EOM}$ is transmitted through the FP cavity and combined with the oscillator pulses on a fast photodiode ($\text {PD}_2$). The detected beat note is quadrature demodulated, and the resulting $I(t)$ and $Q(t)$ signals are used to measure the spectral properties of the TDL pulses.

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4.2 Pulse bandwidth extraction

In this heterodyne measurement, the laser pulses had an exponential-like shape with a relatively long tail since the PC electronics were not yet modified to yield Gaussian-like pulses. The FWHM pulse length was $\tau = 35$ ns. Fourier transforming the square root of the high-pass filtered beat note signal and fitting its power spectral density around $\nu _\text {EOM}$ with a Lorentzian lineshape lead to a FWHM of $\Delta f = 3.7$ MHz as shown in Fig. 6(a). This is in good agreement with the expected 3.1 MHz obtained from the time bandwidth product of $\tau \Delta f = \ln (2)/2\pi \approx 0.11$ for exponential pulses. The injection-seeded pulses from our TDL are thus close to Fourier transform limited. Although we have not repeated the measurement with the Gaussian pulses yet, we expect transform limited pulses in this case too.

 figure: Fig. 6.

Fig. 6. (a) Power spectrum of the heterodyne beat note between the laser pulse and the frequency shifted seed laser for 10 mJ pulse energy. A Lorentzian profile with FWHM linewidth of 3.7 MHz was fit to the data. (b) Top: Measured laser pulse (black, solid) and reconstructed laser pulse (red, dashed) using quadrature demodulation techniques for a pulse of 10 mJ energy. (c) Instantaneous frequency shift between laser pulse and seed laser obtained from Eq. (12).

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4.3 Chirp measurement

The in-phase and quadrature signals $I(t)$ and $Q(t)$, obtained after quadrature demodulating the beat note signal, were used to reconstruct the pulse envelope via

$$\left|A(t)\right|^2 \propto Q^2(t) + I^2(t)$$
and to calculate the instantaneous phase
$$\phi(t)=\arctan\left(\frac{Q(t)}{I(t)}\right).$$

The latter allows extraction of the instantaneous frequency shift w.r.t. the seed light (i.e. the chirp of the pulse) through

$$\Delta\nu(t)=\frac{1}{2\pi}\frac{d\phi(t)}{dt}.$$

Figure 6(b) shows a comparison between the original pulse (solid, black) and the reconstructed pulse (dashed, red) using Eq. (10). The close similarity of both pulse shapes serves as a cross-check of the single-frequency character of the original pulse since such a good reconstruction of the pulse can only be achieved if the original pulse is single-frequency. The bump-like features visible in the pulse are a general phenomenon which appears if the resonator losses are mostly localized at a single element (in our case the TFP) [31]. The frequency of the resulting amplitude modulation lies inevitably at the TDL’s free spectral range, and leads to a frequency component in the power spectrum at $\nu _\text {EOM} \pm 80$ MHz. A possible beating between two adjacent axial modes is thus masked by the bump-like features in the pulse. Nevertheless, as can be seen in Fig. 6(a) the spectral purity of the injection seeded TDL is better than 99 %. As shown in Fig. 6(c), the frequency of the pulse was within $\pm 10$ MHz of the seed frequency at all times during the pulse. The increase of $\Delta \nu (t)$ towards the end of the pulse is due to noise since both $I$ and $Q$ signals are small. The wildly oscillating signal before the pulse is either related to the switching of the PC or a measurement artefact and requires more investigation. However, since it happens before the high intensity part of the pulse, it is not of practical relevance to the spectroscopy experiment.

5. Laser performance

Having demonstrated injection-seeding of the TDL, we characterized the laser performance in view of our muonic hydrogen spectroscopy experiment.

Figure 7(a) shows the exponential increase of the pulse energy versus pulse build-up time after trigger. We limited the pulse energy to around 50 mJ in order to avoid laser-induced damage of the TDL. The pulse energy is slightly higher at longer pulse duration (black, circular markers) since the tail of a longer pulse is also amplified during the outcoupling. Thanks to the cavity layout and the injection-seeding, the beam is close to diffraction limited with $M^2 \leq 1.1$ (Fig. 7(b)). As shown in Fig. 8, the pulse-to-pulse energy variation is below 2 % (RMS) without additional stabilization, but the pulse energy exhibits drifts on the order of 20 % over time scales of hours due to seed power fluctuations related to variations of the polarization in the fiber and mechanical drifts caused by air temperature and cooling water temperature fluctuations. The auto-alignment is able to suppress these longterm fluctuations and even allows us to operate the TDL immediately from a cold start. It also slightly reduces the short-term pulse-to-pulse energy variation. The pulse energy stabilization further improves the pulse-to-pulse energy stability to < $0.5$ % (RMS) while increasing the timing jitter only marginally (< $0.3$ ns), so that the TDL can run reliably for hours. The remaining energy fluctuations on the order of $<4$ % (peak-to-peak) are most probably due to temperature instabilities in the cooling water and the air conditioning and require further investigation. The sudden drops in pulse energy visible in Fig. 8(b) and (c) correspond to re-locking of the injection-seeded TDL. Manifestly, a re-lock does not affect the stability of the laser.

 figure: Fig. 7.

Fig. 7. (a) Pulse energy delivered by the injection-seeded thin-disk laser versus pulse build-up time for two opening voltages $U_2$ at the Pockels cell leading to different FWHM pulse lengths $\tau _\text {P}$. Each data point represents the average over 500 pulses. The pump spot has a diameter of $d_\text {P} = 5.8$ mm, the initial resonator reflectivity is $R_\text {out}=50$ % and the repetition rate is 30 Hz. (b) $\text {M}^2$ measurement of 35 mJ pulses delivered by the injection-seeded thin-disk laser at 30 Hz repetition rate. The beam diameter was obtained by calculating the second-order intensity moments of the beam from pictures taken by a movable camera. Inset: Near-field beam profile of a laser pulse with 1/$\text {e}^2$ radius of 2.1 mm.

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 figure: Fig. 8.

Fig. 8. Long-term measurement of the output pulse energy of the injection-seeded thin-disk oscillator (a) without stabilization, (b) with auto-alignment on, (c) with both auto-alignment and pulse energy stabilizer on. With full stabilization the peak-to-peak variation is 4 % over about 80 min of operation. The inset is a zoom on 2 minutes of operation in the fully stabilized case. On this time scale the pulse-to-pulse energy variation is around $0.4$ %. The sudden drops in pulse energy visible in (b) and (c) occur when the laser re-locks.

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For the muon spectroscopy experiment the minimal time between two pulses without significant reduction of the pulse energy is important. We thus tested the laser in double pulsed mode with variable time $\Delta t$ between two pulses at an overall repetition rate of $f_\text {rep} = 30$ Hz. The drop in pulse energy from the first pulse with energy $E_1$ to the second pulse with energy $E_2$ is shown in Fig. 9(a) as a function of the time $\Delta t$ between first and second pulse. With these operating conditions, the pulse energy stays roughly constant down to $\Delta t = 2$ ms, which corresponds to a maximal triggering rate of about 500 $\text {s}^{-1}$. For smaller $\Delta t$, which lead to smaller population inversion for the second pulse, the pulse energy stabilizer compensates the decreased gain by increasing the pulse build-up time as illustrated in Fig. 9(b). For example, at $\Delta t=1$ ms the added pulse build-up time is 24 ns. The drop in pulse energy can be avoided down to $\Delta t = 1$ ms if the pulse energy stabilization unit is switched on (black, triangular data points in Fig. 9(a). Hence, the pulse energy stabilizer can be used to significantly increase the average repetition rate of the laser system when stochastically triggered.

 figure: Fig. 9.

Fig. 9. (a) Energy drop of the second pulse relative to the first pulse $\left (E_2-E_1\right )/E_1$ versus time $\Delta t$ between the two pulses with (black, triangles) and without (red, circles) pulse energy stabilizer. The error bars are obtained from about 300 double-pulses recorded for each setting of $\Delta t$. In this data series $E_1 = 14$ mJ and the overall repetition rate was 30 Hz. (b) Additional pulse build-up time introduced by the pulse energy stabilizer for the measurements given in panel (a).

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The drop in pulse energy at $\Delta t = 0.5$ ms even with the energy stabilizer turned on is explained as follows: The energy stabilizer keeps the resonator closed for some time $t_\text {stab}$ until a certain value of intra-resonator intensity is detected. In reality, however, the resonator is only opened after a time $t_\text {stab} + \delta t$ where $\delta t$ is an additional fixed delay caused by the stabilizer electronics. For very short pulse separations $\Delta t$ the gain for the second pulse falls so much behind the gain of the fist pulse that the energy extracted in this additional time $\delta t$ is much smaller than for the first pulse.

6. Conclusion and outlook

We developed an injection-seeded, Q-switched, Yb:YAG thin-disk laser with the following properties:

  • $\text {TEM}_{00}$ output with $\text {M}^2 \leq 1.1$,
  • • Up to 50 mJ pulse energy (we limited the output energy to this value to avoid laser induced damage),
  • • Stable output pulse energy, independent of the delay between pulses up to 1 kHz (at 14 mJ),
  • • On demand pulse generation with latency of 850 ns from trigger to pulse delivery,
  • • Adjustable pulse length from 55 ns to 110 ns,
  • • Fourier limited pulses with $<5$ MHz linewidth,
  • • Pulse-to-pulse energy fluctuations of 0.4 % and peak-to-peak energy fluctuation $<4$ % over hours of operation.

Single axial mode operation was achieved by PDH-locking the thin-disk laser resonator to a master seed laser. By modulating the seed laser at half the free spectral range of the thin-disk laser resonator, the PDH-lock was guaranteed to re-lock correctly even after large disturbances. In the present setup, the pulse energy can be stabilized up to a repetition rate of about 1 kHz which is well beyond our required repetition rate. If needed, the pulse build-up time could be reduced by shortening the thin-disk laser resonator length, by increasing the pump power density (i.e. the gain in the disk) and by increasing the seed power. We plan to further increase the long-term stability of our system by improving its temperature stability. This single-frequency thin-disk laser will be used in the laser system for the measurement of the ground-state hyperfine-splitting in muonic hydrogen, currently being pursued at the Paul Scherrer Institute in Villigen, Switzerland.

Appendix

A. Calculation of the resonator layout

The resonator layout for the $\text {TEM}_{00}$ Gaussian beam is calculated using the ABCD matrix and the complex beam parameter formalism [32]. The complex beam parameter $q$ is defined as

$$\frac{1}{q} \equiv \frac{1}{R} - i \frac{\lambda}{\pi w^2},$$
where $R$ is the radius of curvature of the phase front, $\lambda$ is the laser wavelength and $w$ is the beam radius (1/$\text {e}^2$). The complex beam parameter $q_\text {out}$ at the output of an optical system can be calculated knowing the ABCD matrix of the system and the input complex beam parameter $q_\text {in}$ by using the relation [33]
$$q_\text{out} = \frac{A q_\text{in}+B}{C q_\text{in}+D}.$$

For a stable resonator $q_\text {out} = q_\text {in}$ must be fulfilled, which leads to

$$q_0 = \frac{B(A-D)}{2(AD-1)} \pm \frac{B}{2(AD-1)}\sqrt{(A+D)^2-4},$$
where $q_0$ is the complex beam parameter of the stable resonator mode at the reference plane used to compute the round-trip ABCD matrix. Definition (13) indicates that a finite beam size is only possible for $\text {Im}(q_0) \neq 0$, which is fulfilled when $\left | A+D \right |^2<4$ (this is the well-known stability criterion for laser resonators [32]). Equation (15) also indicates that a collimated stable resonator mode, i.e., a beam with $\text {Re}(q_0) = 0$ at the reference plane of the ABCD matrix, is only possible when $A=D$ (we neglect the case $B=0$ with $AD=1$, as such a system is only marginally stable).

With these definitions and observations at hand, we can proceed to calculate expression (4) and (5). For simplicity, the resonator round-trip ABCD matrix $M$ is calculated for the cold state (i.e., at zero pump power), without taking into account soft aperture effects and thermal lensing [27]. $M$ is obtained by calculating (see Fig. 2)

$$M \equiv \left(\begin{array}{cc} A & B\\ C & D \end{array}\right) = P_{d_0} L_{f_D} P_{d_1} L_{f_\text{cav}} P_{d_2} L_{f_\text{vex}} P_{2d_3} L_{f_\text{vex}} P_{d_2} L_{f_\text{cav}} P_{d_1} L_{f_D} P_{d_0},$$
where $P_x$ and $L_f$ are the ABCD matrices for a free propagation of length $x$ and for a thin lens with focal length $f$, given by
$$P_{x}=\left(\begin{array}{cc} 1 & x\\ 0 & 1 \end{array}\right) \text{ and } L_{f}=\left(\begin{array}{cc} 1 & 0\\ -\frac{1}{f} & 1 \end{array}\right),$$
respectively. The general expression for $M$ is cumbersome and best evaluated with the help of a computer algebra program like Mathematica. For example the A and B elements consists of 106 and 126 distinct summands, respectively.

Nevertheless, we know that $A=D$ (see above) since the circulating beam is collimated at the end-mirror $\text {M}_1$ (reference plane of $M$), and identifying $M$ with $M_\text {FT}$ leads to $A=0$. Furthermore, since $\text {det}(M)=AD-BC = -BC = 1$, we are actually left with only one more independent matching identity, namely $B=F$ (we could also have chosen $C=-1/F$ which results in the same equation). These two equations were solved for $d_2$ and $d_3$ using Mathematica (note that expressions (4) and (5) were only obtained after a substantial manual simplification of the expressions obtained by first calling the Solve[] and then applying the Simplify[] functions).

B. Jones matrix of the TFP-$\lambda /4$-PC system

The Jones matrices used in our calculations are given in Table 2. Without loss of generality we identify (1,0) with the vertical y-axis and (0,1) with the horizontal x-axis. Note that an element with Jones matrix $J$ which is rotated by an angle $\alpha$ w.r.t. the y-axis has the Jones matrix $J(\alpha )=\mathcal {R}_\alpha J \mathcal {R}_{-\alpha }$ (see Table 2).

Tables Icon

Table 2. Jones matrices used to calculate the effective reflectivity of the TFP-$\lambda /4$-PC system.

The round-trip Jones matrix of the $\lambda /4$-PC system is given by

$$J = \mathcal{R}_{\alpha} J_{\lambda/4} \mathcal{R}_{-\alpha} \mathcal{R}_{45^{{\circ}}} J_\text{PC} \mathcal{R}_{{-}45^{{\circ}}} \mathcal{R}_{45^{{\circ}}} J_\text{PC} \mathcal{R}_{{-}45^{{\circ}}}\mathcal{R}_{\alpha} J_{\lambda/4} \mathcal{R}_{-\alpha} = \left(\begin{array}{cc} J_{11} & J_{12}\\ J_{12} & J_{11}^* \end{array}\right)$$
where * denotes complex conjugation. Note that the $\lambda /4$ waveplate is rotated by some angle $\alpha$ and the optical axis of the PC is rotated by 45$^{\circ }$ w.r.t. the y-axis, respectively. Thanks to the symmetry of the round-trip the Jones matrix has a simple structure with entries
$$\begin{aligned}J_{11} &={-}\frac{1}{2} \left(1 + \cos(\pi \Delta U) + 2 \cos(4 \alpha) \sin^2\left(\frac{\pi \Delta U}{2}\right)\right.\\ &\quad - \left.i \left[ ( \cos(6 \alpha) - \frac{1}{2} \cos(2 \alpha)) \sin^2\left(\frac{\pi \Delta U}{2}\right) + \sin(4 \alpha) \sin(\pi \Delta U)\right]\right) \end{aligned}$$
$$J_{12} = i \sin^2\left(\frac{\pi \Delta U}{2}\right) \sin(2 \alpha) \left(1 + \cos(4 \alpha) + 2 \cot\left(\frac{\pi \Delta U}{2}\right) \sin(2 \alpha)\right).$$

The entries were obtained with the help of Mathematica. After calling the Simplify[] function, significant simplification had to be performed manually to reach expressions (20).

Finally, the effective intensity reflectivity of the TFP-$\lambda /4$-PC system given by (9) is obtained by taking into account that the TFP is reflecting only the vertical polarization, yielding

$$R_\text{out}(\Delta U) = \left| \left[\begin{array}{c} 1\\ 0 \end{array}\right]\cdot J\left[\begin{array}{c} 1\\ 0 \end{array}\right]\right|^2 = \left| J_{11} \right|^2,$$
where $\cdot$ denotes the scalar product.

Funding

Agence Nationale de la Recherche (ANR-18-CE92-0030-02); Deutsche Forschungsgemeinschaft (DFG/ANR Project LASIMUS (407008443), EXC 1098 PRISMA (194673446), EXC PRISMA+ (390831469), Excellence Initiative EXC 1098 PRISMA (194673446), Excellence Strategy EXC PRISMA+ (390831469), LASIMUS (407008443)); Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung (SNF 200020_197052, SNF 200021_165854); European Research Council (CoG. #725039).

Acknowledgments

We gratefully acknowledge the support of the ETH Zürich electronics workshop. In particular, we thank Diogo Di Calafiori and Dr. Werner Lustermann. We also thank Dr. Marcos Gaspar, Dr. Carlo Vicario, Dr. Cezary Sidle and Stefan Mair from PSI.

Disclosures

The authors declare that there are no conflicts of interest related to this article.

Data availability

Data that support the findings of this study are available from the corresponding author upon reasonable request.

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Data availability

Data that support the findings of this study are available from the corresponding author upon reasonable request.

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Figures (9)

Fig. 1.
Fig. 1. Schematic of the injection-seeded thin-disk oscillator. HV: high-voltage, PC: Pockels cell, TFP: thin-film polarizer, FR: Faraday rotator, PD: photodiode, PDH lock: Pound-Drever-Hall locking scheme, $\updownarrow$: P-polarization, $\odot$: S-polarization, $\mathrm {\lambda }$/2: half-wave plate, $\mathrm {\lambda }$/4: quarter-wave plate. The resonator is spanning between end-mirrors $\text {M}_1$ and $\text {M}_2$. The PC-$\mathrm {\lambda }$/4-TFP system forms a HV controlled outcoupler steering the Q-switching dynamics of the oscillator. Through this TFP the seed laser output is injected into the resonator prior to trigger, and the pulses are extracted from the oscillator after pulse-buildup. Resonant coupling of the seed laser light into the oscillator is achieved through a PDH-locking scheme acting on the resonator length. The resonator alignment is stabilized via an autoalignment system including the quadrature photodiode $\text {PD}_\text {A}$ and two piezos steering the alignment of mirror "cav". The pulse energy is stabilized via a feed-forward system including the photodiode $\text {PD}_\text {E}$ and a delay box adjusting the pulse build-up time.
Fig. 2.
Fig. 2. Beam radius (1/$\text {e}^2$) of the $\text {TEM}_{00}$ mode along the TDL resonator for variations of the disk dioptric power $\Delta V$. For simplicity the location of folding mirror $\text {M}_\text {fold}$ is not shown.
Fig. 3.
Fig. 3. (a) Typical open-loop PDH-error-signal measured with photodiode $\text {PD}_\text {PDH}$ in Fig. 1 obtained by scanning the resonator length. The modulation frequency of the seed laser is 40 MHz, i.e., half the free spectral range of the resonator. (b) Corresponding $\text {TEM}_{00}$ intra-resonator intensity measured with $\text {PD}_\text {I}$. As the resonator length is scanned, the side bands are also visible at $\pm 40$ MHz.
Fig. 4.
Fig. 4. (a) Effective reflectivity $R_\text {out}$ of the thin-disk laser resonator versus voltage difference $\Delta U$ across the BBO crystal in the Pockels cell. The dashed arrows indicate a switching sequence where the resonator is closed by switching the first electrode to $U_1=8$ kV and then opened by switching the second electrode to either $U_2=8$ kV (black, dashed) or $U_2=13$ kV (red, dashed). (b) Typical pulse shapes for the two switching sequences in a). The gray shaded area shows the envelope of 100 pulses and the solid lines their average. Both pulses have an energy of 25 mJ.
Fig. 5.
Fig. 5. Sketch of the optical setup used to generated the heterodyne signal. The dashed red line represents the laser pulses. The seed laser output is split into two branches. One branch injection-seeds the thin-disk laser oscillator with photons at a frequency $\nu _{\text {seed}}$. The other branch contains an EOM imprinting sidebands at $\nu _\text {seed}\pm \nu _\text {EOM}$. The blue side band is kept resonant with the Fabry-Perot (FP) cavity, so that only the frequency $\nu _\text {seed}+\nu _\text {EOM}$ is transmitted through the FP cavity and combined with the oscillator pulses on a fast photodiode ($\text {PD}_2$). The detected beat note is quadrature demodulated, and the resulting $I(t)$ and $Q(t)$ signals are used to measure the spectral properties of the TDL pulses.
Fig. 6.
Fig. 6. (a) Power spectrum of the heterodyne beat note between the laser pulse and the frequency shifted seed laser for 10 mJ pulse energy. A Lorentzian profile with FWHM linewidth of 3.7 MHz was fit to the data. (b) Top: Measured laser pulse (black, solid) and reconstructed laser pulse (red, dashed) using quadrature demodulation techniques for a pulse of 10 mJ energy. (c) Instantaneous frequency shift between laser pulse and seed laser obtained from Eq. (12).
Fig. 7.
Fig. 7. (a) Pulse energy delivered by the injection-seeded thin-disk laser versus pulse build-up time for two opening voltages $U_2$ at the Pockels cell leading to different FWHM pulse lengths $\tau _\text {P}$. Each data point represents the average over 500 pulses. The pump spot has a diameter of $d_\text {P} = 5.8$ mm, the initial resonator reflectivity is $R_\text {out}=50$ % and the repetition rate is 30 Hz. (b) $\text {M}^2$ measurement of 35 mJ pulses delivered by the injection-seeded thin-disk laser at 30 Hz repetition rate. The beam diameter was obtained by calculating the second-order intensity moments of the beam from pictures taken by a movable camera. Inset: Near-field beam profile of a laser pulse with 1/$\text {e}^2$ radius of 2.1 mm.
Fig. 8.
Fig. 8. Long-term measurement of the output pulse energy of the injection-seeded thin-disk oscillator (a) without stabilization, (b) with auto-alignment on, (c) with both auto-alignment and pulse energy stabilizer on. With full stabilization the peak-to-peak variation is 4 % over about 80 min of operation. The inset is a zoom on 2 minutes of operation in the fully stabilized case. On this time scale the pulse-to-pulse energy variation is around $0.4$ %. The sudden drops in pulse energy visible in (b) and (c) occur when the laser re-locks.
Fig. 9.
Fig. 9. (a) Energy drop of the second pulse relative to the first pulse $\left (E_2-E_1\right )/E_1$ versus time $\Delta t$ between the two pulses with (black, triangles) and without (red, circles) pulse energy stabilizer. The error bars are obtained from about 300 double-pulses recorded for each setting of $\Delta t$. In this data series $E_1 = 14$ mJ and the overall repetition rate was 30 Hz. (b) Additional pulse build-up time introduced by the pulse energy stabilizer for the measurements given in panel (a).

Tables (2)

Tables Icon

Table 1. Resonator parameters.

Tables Icon

Table 2. Jones matrices used to calculate the effective reflectivity of the TFP- λ / 4 -PC system.

Equations (21)

Equations on this page are rendered with MathJax. Learn more.

M FT = ( 0 F 1 F 0 ) ,
w 0 = F λ π ,
M 1    -  d 0  disk   -  d 1  cav   -  d 2  vex   -  d 3   M 2    -  d 3  vex   -  d 2  cav   -  d 1  disk  -  d 0   M 1 ,
d 2 = f vex + F ( f D d 1 ) F f D ξ ( F f D ) + F f D / f cav + d 1 f D F f D ξ ( F f D ) + F f D / f cav ,
d 3 = f vex + F f vex 2 2 [ 1 f D 2 1 F 2 + 1 f cav 2 ] ( 1 ξ ) 2 + F ( f vex f cav ) 2 [ ( ξ + f cav f D ) ( 1 ξ ) + 1 2 ξ 2 ] ,
d 2 f vex + f D F F f D
d 3 f vex + F 2 [ ( f vex f D ) 2 ( f vex F ) 2 ] .
w w 0 = 1 + 1 4 F 2 Δ V 2 + 5 32 F 4 Δ V 4 + ,
R out ( t ) = | cos ( 2 π Δ U ( t ) U λ / 4 ) cos ( 2 α ) 1 2 sin ( 2 π Δ U ( t ) U λ / 4 ) sin ( 4 α ) + i sin ( 2 π Δ U ( t ) U λ / 4 ) sin ( 2 α ) | 2
| A ( t ) | 2 Q 2 ( t ) + I 2 ( t )
ϕ ( t ) = arctan ( Q ( t ) I ( t ) ) .
Δ ν ( t ) = 1 2 π d ϕ ( t ) d t .
1 q 1 R i λ π w 2 ,
q out = A q in + B C q in + D .
q 0 = B ( A D ) 2 ( A D 1 ) ± B 2 ( A D 1 ) ( A + D ) 2 4 ,
M ( A B C D ) = P d 0 L f D P d 1 L f cav P d 2 L f vex P 2 d 3 L f vex P d 2 L f cav P d 1 L f D P d 0 ,
P x = ( 1 x 0 1 )  and  L f = ( 1 0 1 f 1 ) ,
J = R α J λ / 4 R α R 45 J PC R 45 R 45 J PC R 45 R α J λ / 4 R α = ( J 11 J 12 J 12 J 11 )
J 11 = 1 2 ( 1 + cos ( π Δ U ) + 2 cos ( 4 α ) sin 2 ( π Δ U 2 ) i [ ( cos ( 6 α ) 1 2 cos ( 2 α ) ) sin 2 ( π Δ U 2 ) + sin ( 4 α ) sin ( π Δ U ) ] )
J 12 = i sin 2 ( π Δ U 2 ) sin ( 2 α ) ( 1 + cos ( 4 α ) + 2 cot ( π Δ U 2 ) sin ( 2 α ) ) .
R out ( Δ U ) = | [ 1 0 ] J [ 1 0 ] | 2 = | J 11 | 2 ,
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