Abstract
High-dimensional maximally entangled orbital angular momentum (OAM) states are a promising resource for enhancing information capacity and robustness in quantum communication. However, it still lacks an effective method to increase the state dimensionality. Here, we theoretically propose an efficient scheme to generate maximally entangled OAM states of ultrahigh dimensionality by manipulating the radial components of a Laguerre-Gaussian (LG) pump beam. By optimizing the complex amplitudes of multiple radial modes of the LG pump light, one can feasibly achieve 101-dimensional OAM-based maximally entangled states. Our scheme has potential applications in high capacity quantum communication networks.
© 2022 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement
1. Introduction
High-dimensional maximally entangled states (MESs) of two photons have raised widespread interests because of their promising applications, such as closing the detection loophole in Bell test experiments, enhancing information capacity, and raising the resistance to noise in quantum communication [1–3]. In generating MESs, various degrees of freedom such as which-way paths, discretized time and frequency modes, and transverse-spatial modes can be used [4–9].
The entanglement of Laguerre-Gaussian (LG) modes has been extensively studied because these modes carry OAM quanta [10]. The discrete nature of OAM in infinite-dimensional Hilbert space is quite suitable for high-dimensional quantum information. To date, the OAM of light has become a workhorse for high-dimensional spatial-mode-based MESs, which can be generated and manipulated conveniently in nonlinear optical processes [7,11–15]. In a nonlinear crystal, an intense pump light produces two entangled photons (referred to as signal and idler) through a spontaneous parametric down-conversion (SPDC) process, which obeys the conservation laws of energy, momentum, and OAM [16]. The main methods to generate high-dimensional OAM-based MESs are entanglement concentration (i.e., Procrustean filtering) [7,17] and pump light shaping (which manipulates the spatial modes of the pump light) [18–20]. The entanglement concentration method requires a broad spiral bandwidth to realize high-dimensional entanglement, which is difficult to be satisfied by using a traditional Gaussian pump beam. By shaping the LG pump light, several groups have successfully broadened the spiral bandwidth and efficiently produced arbitrary three-dimensional OAM-based MESs. These works mainly manipulate the azimuthal components (i.e., OAM quantum number l) of the pump light. However, such pump light carrying multiple OAM components usually produce unwanted photon modes during SPDC, which requires extra diagonalization of the OAM detection bases [19,20]. The higher the dimensionality of the state is, the more cumbersome the manipulation is.
In this paper, we theoretically propose a scheme to generate executable ultrahigh-dimensional OAM-based MESs efficiently by manipulating the radial components p of LG pump light. The OAM spectrum of two-photon states is dependent on the spatial shape of the pump light [18–22]. In our scheme, the azimuthal component of the pump light is fixed to be $l = 0$, which well avoids the requirement of detection base diagonalization in previous works. Using gradient descent and simulated annealing algorithms [23], we numerically simulate the optimal complex amplitudes of the p components of LG pump light to produce high-dimensional OAM-based MESs. By constructing proper LG pump light with six p components [24], we obtain OAM-based MESs from three dimensions to twenty dimensions with high accuracies. Furthermore, with an LG pump light consisting of seventeen p modes, 101-dimensional OAM-based MESs can be achieved, which has potential applications in high-capacity robust quantum networks. Our scheme can also be applied in quantum state engineering such as the generation of two-photon states with symmetric OAM spectra.
2. Principle
In a SPDC, signal and idler photons are strongly OAM-correlated through the conservation law of OAM [16]. Moreover, the OAM coincidence probability of the entangled two-photon state, i.e., the spiral spectrum [25], is not uniform because the coincidence probability depends on the overlap between the spatial modes of the entangled photons and the pump light. Here, we consider an ideally-phase-matched collinear SPDC process. For completeness of the LG base, the entangled two-photon state of the spatial modes in a thin crystal is [26]
To produce high-dimensional OAM-based MESs, the spatial mode of the pump light is a coherent superposition state ${|\psi \rangle _p}$ consisting of LG modes with the same lp but different pp. ${|\psi \rangle _p}$ is given as
where ${C_{{p_p}}}$ denotes the complex amplitude. We calculate the distribution of the coincidence probability amplitude $C_{{p_s},{p_i}}^{{l_s},{l_i}}$ when the pump light is a single LG mode within ${p_p} = 0,\textrm{ }1,\textrm{ } \cdots ,\textrm{ }5$ [ Fig. 1(a)]. All the spectra of the coincidence probability amplitudes are symmetric and centered at ${l_s} = 0$. When ${p_p} \ne 0$, negative values of $C_{{p_s},{p_i}}^{{l_s},{l_i}}$ arise from the non-uniform phase of the pump light.From the data in Fig. 1(a), we construct the matrix A consisting of six spectra of the coincidence probability amplitudes [Fig. 1(b)], in which the columns and rows refer to the LG components of the pump light (${p_p} = 0,\textrm{ }1,\textrm{ } \cdots ,\textrm{ }5$) and the OAM numbers of the detected photon pairs (${l_s},\textrm{ }{l_i} ={-} 50,\textrm{ } - \textrm{49},\textrm{ } \cdots ,\textrm{ }50$), respectively. The complex amplitude vector of the LG pump light is defined as $C = {({{C_1},\textrm{ }{C_2},\textrm{ } \cdots ,\textrm{ }{C_6}} )^T}$, and the target state of the d-dimensional OAM MES is given as ${|\psi \rangle _T} = \frac{1}{{\sqrt d }}\sum\limits_l {|{l,\textrm{ } - l} \rangle }$. In Fig. 1(b), the amplitude of the target state is set as the vector $\tilde{T}$. For odd d, the spatial modes of the d-dimensional target state ${|\psi \rangle _T}$ are $l ={-} {{({d - 1} )} / 2},\textrm{ } - {{({d - 1} )} / 2} + 1,\textrm{ } \cdots ,{{\textrm{ }({d - 1} )} / 2}$. For even d, the spatial modes of the target state ${|\psi \rangle _T}$ are $l ={-} {d / 2},\textrm{ } \cdots , - 1,\textrm{ }1,\textrm{ } \cdots ,{{\textrm{ }d} / 2}$. From the product of A and C, we obtain the vector O which denotes the coincidence probability amplitude of the two-photon output state ${|\psi \rangle _O}$. By post-selecting the modes of ${|\psi \rangle _T}$ from ${|\psi \rangle _O}$, we obtain the desired state ${|{\tilde{\psi }} \rangle _O}$. $\tilde{O}$ denotes the amplitude of ${|{\tilde{\psi }} \rangle _O}$, which should be as close to $\tilde{T}$ as possible.
With the gradient descent and simulated annealing algorithms, we find the optimal amplitude vector C to produce ${|{\tilde{\psi }} \rangle _O}$ efficiently and accurately. We first create the evaluation function E, i.e.,
withHere, all ${\tilde{T}_i}$ are positive (i.e., all ${\tilde{T}_i}$ are in-phase). The function ${E_1}$ (${E_2}$) is used to evaluate the similarity between $\tilde{O}$ ($O$) and $\tilde{T}$. The smaller the value of the function ${E_1}$ (${E_2}$), the more accurate (efficient) the desired state ${|{\tilde{\psi }} \rangle _O}$ is. Then, at each iteration, the amplitude vector changes by a small amount of
3. Experimental scheme and simulation
We propose an experimental scheme for the generation of high-dimensional OAM-based MESs (Fig. 2). A phase-only spatial light modulator1 (SLM1) realizes a complex-field modulation of the pump light, which is then injected into a BBO crystal [24]. One can generate the complex field with high fidelity by use of phase-amplitude encoding [27–31]. In this nonlinear crystal, a 415-nm pump light produces two entangled photons with the same polarizations, corresponding to a type-I SPDC process. We use lenses and single-mode fibers (SMFs) to control ${\gamma _s}$ and ${\gamma _i}$. Moreover, SLM 2 and SLM 3 are used to project the photons into the detection base and convert the specific spatial component of the photons into a Gaussian mode. To further improve the detection accuracy, one should consider the filtering effect from SMF and correct the holograms by a Gaussian mode function [32–35]. Then, SMFs collect the photons in Gaussian modes, avalanche photodiodes detect the delivered photons and a coincidence count takes place. For d-dimensional OAM-based MESs, where $d = 3,4, \cdots ,20$, we calculate the complex amplitudes of the six LG modes of the pump light (Table 1). The corresponding OAM-based MESs are given in Fig. 3(a) marked with red bars. In Table 1, negative signs indicate a π phase delay.
For these OAM-based MESs, the mean square errors of the coincidence probability amplitudes between $\tilde{O}$ and $\tilde{T}$, i.e., $\frac{{{E_1}}}{d}$ are less than 10−6 [Fig. 3(b)]. The curves of the mean square error and fidelity confirm the high accuracy between $\tilde{O}$ and $\tilde{T}$. In the detection base, we calculate the angular Schmidt numbers of the output states ${|\psi \rangle _O}$ [Fig. 3(c)]. With the growing dimensionality of MESs, the spiral bandwidth becomes broader, and the angular Schmidt numbers are always larger than the corresponding d. To compare our method with entanglement concentration, we plot the curve of the coincidence rate ratio of our method to that of entanglement concentration [Fig. 3(c)]. Here, the coincidence rate of entanglement concentration is calculated with pump light settings ${l_p} = {p_p} = 0$ and $\gamma = 1$. Note that the entanglement concentration method is efficient when $d < 6$. For higher dimensions, the high-order modes of the pump light having wide spiral bandwidths are fully utilized and the coincidence rate improvement in our method becomes notable. To further increase the coincidence rate and accuracy of the generated state, one can increase the p mode number of the LG pump light, optimize parameters ${\gamma _s}$ and ${\gamma _i}$, or increase the iteration number of the algorithm.
It is known that the parameter $\gamma$ should be set as large as possible to produce high-dimensional OAM-based MESs by entanglement concentration. However, $\gamma \gg 1$ cannot be achieved in an experiment because one cannot unlimitedly increase the size of the pump beam (or unlimitedly decrease the sizes of the signal and idler beams). Moreover, for small ${w_s}$ and ${w_i}$, the pixelation effects of the SLMs cannot be neglected in the detection of the two-photon states. Under a typical experimental scenario with $\gamma \sim 1$ [22], entanglement concentration is inefficient to produce high-dimensional OAM-based MESs because of its narrow spiral bandwidth. In contrast, by shaping the radial components p of the pump light, we can considerably enhance the coincidence rate with $\gamma = 1$. Figure 4(a) compares the coincidence rates of above two methods under different value of $\gamma$ for 10D, 15D, and 20D OAM-based MESs. The fidelities of our method are given in Fig. 4(b). Here, the coincidence rate of the entanglement concentration method is calculated with a pump light of ${l_p} = {p_p} = 0$. Clearly, for small $\gamma$ and large d, the proposed pump shaping method is remarkably efficient.
When the pump light consists of seventeen p components of LG pump light, we can produce in theory a 101D OAM-based MES with a fidelity of 0.999996 [ Fig. 5(a)]. This result suggests that ultrahigh-dimensional OAM-based MESs can be produced by increasing the p components of the LG pump light. Interestingly, by utilizing the symmetry of the matrix A, we can produce specific entangled states featuring symmetric weight distributions. Figure 5(b) shows three states with their weight distributions having square, peaked, and funnel-shaped profiles, which demonstrate the versatility of our scheme for quantum state engineering.
Our method can also be applied to generate high-brightness high-dimensional MESs with OAM state being defined by $|\psi \rangle = \sum\limits_{{l_s},{l_i}} {{C_{{l_s},{l_i}}}|{{l_s}} \rangle } |{{l_i}} \rangle$. Here, ${C_{{l_s},{l_i}}} = \sum\limits_{{p_s},{p_i}} {C_{{p_s},{p_i}}^{_{{l_s},{l_i}}}}$. In the numerical calculations, we use LG components of the pump light having mode indices of ${p_p} = 0,\textrm{ }1,\textrm{ } \cdots ,\textrm{ }5$ and ${l_p} = 0$. The spatial modes of the coincidence detection base are ${\gamma _s} = {\gamma _i} = \gamma = 1$, ${l_s},\textrm{ }{l_i} ={-} 50,\textrm{ } - \textrm{49},\textrm{ } \cdots ,\textrm{ }50$ and ${p_s},\textrm{ }{p_i} = 0,\textrm{ }1,\textrm{ } \cdots ,\textrm{ 1}0$. Figure 6(a) shows the normalized spectra of the coincidence probability amplitudes with ${p_p} = 0,\textrm{ }1,\textrm{ } \cdots ,\textrm{ }5$. Figure 6(b) shows the corresponding d-dimensional OAM MESs. Here, $d = 3,4, \cdots ,20$. Figure 6(c) shows the calculated fidelity and coincidence rate. Clearly, the coincidence rate in this case can be significantly improved after optimizing the pump light through our method.
4. Conclusion
To date, the highest quantum number of an OAM entangled state is 10010 [36], which indicates its great potential for increasing the capacity of quantum information processing. Using OAM correlation, researchers have realized quantum spiral imaging and pattern recognition [37–39], precision measurements [40,41], and combining and converting different physical degrees of freedom [42,43]. High-dimensional OAM-based MESs could further improve the performance of quantum states in these applications. With properly shaping the LG radial components of pump light, we propose a theoretical scheme to generate efficiently high-dimensional OAM-based MESs for quantum communication networks. Our method is also capable to realize quantum state engineering such as generation of OAM-entangled states with specific symmetric weights.
Funding
National Key Research and Development Program of China (2017YFA0303703, 2019YFA0308704); National Natural Science Foundation of China (11874212, 11874213, 11904424, 91950206); Fundamental Research Funds for the Central Universities (021314380105, 021314380191).
Disclosures
The authors declare no conflicts of interest.
Data availability
Data underlying the results presented in this paper are not publicly available at this time but may be obtained from the authors upon reasonable request.
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