Abstract
We present a high-performance functional perfect absorber in a wide range of terahertz (THz) wave based on a hybrid structure of graphene and vanadium dioxide (VO2) resonators. Dynamically electrical and thermal tunable absorption is achieved due to the management on the resonant properties via the external surroundings. Multifunctional manipulations can be further realized within such absorber platform. For instance, a wide-frequency terahertz perfect absorber with the operation frequency range covering from 1.594 THz to 3.272 THz can be realized when the conductivity of VO2 is set to 100000 S/m (metal phase) and the Fermi level of graphene is 0.01 eV. The absorption can be dynamically changed from 0 to 99.98% and in verse by adjusting the conductivity of VO2. The impedance matching theory is introduced to analyze and elucidate the wideband absorption rate. In addition, the absorber can be changed from wideband absorption to dual-band absorption by adjusting the Fermi level of graphene from 0.01 eV to 0.7 eV when the conductivity of VO2 is fixed at 100000 S/m. Besides, the analysis of the chiral characteristics of the helical structure shows that the extinction cross-section has a circular dichroic response under the excitation of two different circularly polarized lights (CPL). Our study proposes approaches to manipulate the wide-band terahertz wave with multiple ways, paving the way for the development of technologies in the fields of switches, modulators, and imaging devices.
© 2022 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement
1. Introduction
Terahertz radiation is an electromagnetic wave between infrared and microwave, ranging from 0.1 THz to 10 THz. The artificial and effective manipulation of Terahertz radiation has wide application in biomedicine [1,2], detectors [3–5], terahertz switches [6], imaging [7–9] and wireless communications [10,11]. Due to the natural materials contributing little to THz technologies, which is not conducive to its development. Later, the emergence of metamaterials (MMs) provides researchers with a new approach. Metamaterials consist of periodic arrays of subwavelength metals or dielectric blocks which can produce electromagnetic responses that are not exist in natural materials. Therefore, metamaterials have found a wide range of applications in the field of optical, such as perfect lenses [12–14], polarization converter [15–17], negative refraction [18], vector light fields [19] and perfect metamaterial absorber [20]. Perfect metamaterial absorber is a significant branch of metamaterial application. Degeneracy critical coupling [21] and breaking parity-time (PT) symmetry [22] are used to break the 50% absorption limit of subwavelength thickness film. Coherent asymmetric absorbers can change the absorption from almost perfect to very small by changing the incident Angle of coherent waves [23]. Random metasurfaces are used to reduce light interactions and thus solve the light scattering problem [24]. Metal-insulator-metal (MIM) structured absorbers utilizing Fabry-Perot (FP) cavity resonances are classic approach to achieve near-unity absorption. The search for perfect metamaterial absorbers (PMA) has not quit since Landy et al. first introduced a single band perfect absorber in 2008 [25], and gradually developed into a full-spectrum range including ultraviolet [26], visible light [27], infrared [28], THz [29] and microwave [30,31]. In particular, PMA in THz band is often limited to very narrow bandwidth and constant intensity which cannot be adjusted once the structure design is completed. Therefore, achieving dynamic tunable PMA with high absorption intensity over a wide THz range is an arduous task.
Graphene is a 2D film composed of periodic arrays of carbon atoms in a hexagonal lattice, and its conductivity can be dynamically adjusted over a wide frequency range by adjusting chemical doping or gate voltages [32–34]. As a phase change material, VO2 is another excellent dynamic tunable material that differs from graphene in that it can change from an insulating state to a metallic state at about 340 K [35], and the transition is reversible. This transition can be triggered by externally excited light and thermal radiation and can achieve conductivity changes of multiple orders of magnitude in the picosecond range. Nonetheless, previous graphene and VO2-based PMA remained limited to narrow-band or multi-band dynamic tuning [36,37], while tuning with high modulation depths remained rare for perfect absorbers of broadband terahertz. The comparison of wideband THz absorbers based on graphene or VO2 that have emerged in the past year are shown in Table 1.
Here, a broadband perfect absorber was proposed with dynamical tunability, which combines graphene and VO2, consists of a golden mirror at the bottom, a layer of topas, and a helical VO2 located on a layer of graphene. By adjusting the conductivity of VO2 from 200 S/m to 200000 S/m, VO2 can transform from an insulating phase to a metallic phase, and obtain the best broadband perfect absorption at a conductivity of 100000 S/m. When the conductivity of VO2 is 100000 S/m (metallic phase), the absorption rate is greater than 90% in the range of 1.594 THz-3.272 THz (bandwidth 1.678 THz) and greater than 99% in the range of 1.834 THz-3.155 THz (bandwidth 1.321 THz), of which the absorption of 2.05 THz is 100%, and the absorption of 3.08 THz is 99.55%. When the conductivity of VO2 is 200 S/m (insulator phase), the absorption rate of the absorber as a whole is close to 0. The maximum modulation depth (MD) is 99.98% and the minimum extinction ratio (ER) is -36.5 dB. In addition, by adjusting the Fermi energy level of graphene from 0.01 eV to 0.7 eV, the absorber can be changed from a wide-band absorber to an absorber with two resonant absorption peaks. Finally, a supplementary analysis of the chiral characteristic of the helical structure reveals that there is a circular dichroism response under the excitation of left-circularly polarized (LCP) and right-circularly polarized (RCP). The results show that the designed absorber not only has simple structure, but also shows a good prospect in imaging, optical switches, modulators.
2. Design and method
Full-wave simulations were implemented by using the finite element method (FEM). A unit cell of the absorber is equipped with periodic boundary conditions in the X and Y directions to simulate infinite arrays, and a perfect matching layer is created in the Z direction. Periodic ports are set as excitation sources and monitor wave transmission and reflection. Graphene layer with single atom thickness can be regarded as 2D infinite-thin layer, and transition boundary condition is set for it to improve computation efficiency. Fine mesh is used to ensure the convergence of the results. A 3D, side and top view of the absorber is shown in Fig. 1.
The unit consists of a gold substrate, a waveguide layer of topas, a layer of graphene covered in the waveguide layer and a VO2 helix. The parameters of the structure are set as follow. The helical VO2 with a thickness of t1 = 1 µm, graphene layer with a thickness of t2 = 0.34 nm, topas layer with a thickness of t3 = 20 µm and gold mirror with a thickness of t4 = 0.5 µm as the substrate, respectively. In addition, the lattice constant is P = 65 µm, the minimum radius of the innermost turn of helical VO2 is r = 1 µm, the width d1 and interval d2 of each turn of the helical VO2 are 2 µm and 3 µm, respectively. Furthermore, the designed structure can be manufactured by chemical vapor deposition (CVD) in practical applications.
Regardless of material loss and dispersion, the dielectric permittivity of topas is 2.35. The dielectric permittivity of VO2 in the range of THz can be described by Drude model [47–49], which can be expressed as
According to the Pauli Exclusion Principle, the contribution of the σinter in the THz frequency is negligible at room temperature (T = 300 K) and for Fermi level of interest (Ef/2kBT>>1), the conductivity of graphene can be simplified to a Drude-like model [55]
Here, we set the initial Fermi energy of graphene as 0.01 eV, kB is Boltzman constant, e is electron charge, $\hbar $ is Planck constant, ω is incident light frequency and τ=1 ps is relaxation time. In practical applications, the Fermi level of graphene can be adjusted by the bias voltage according to the condition [56]
where Fermi speed Vf = 1 × 106 m/s, a0 is the capacitance of the structure, and Vbias is the bias voltage.3. Results and discussion
The absorption of the designed absorber can be expressed by the formula A(ω) = 1-R(ω)-T(ω) = 1−|S11|2−|S21|2, where R(ω) and T(ω) represent reflectance and transmittance respectively and the S-parameters can be obtained in the finite element method (FEM) simulation. Since the Au substrate with a thickness of 0.5 µm blocks the transmission of electromagnetic wave, T(ω) can be regarded as zero, the absorption can be simplified as A(ω) = 1-R(ω) = 1−|S11|2 [57].
As shown in Fig. 2(a), the absorptivity of proposed absorber can reach greater than 90% from 1.594 THz to 3.272 THz with bandwidth 1.678 THz when the fermi energy of graphene is 0.01 eV and the conductivity of VO2 is 100000 S/m. The relative absorption bandwidth of the absorber can be calculated as 69% according to the calculation formula RAB = 2 × (fh-fl)/(fh + fl), where fh and fl are the highest limit and lowest limit of frequencies with absorptivity above 90%, respectively [58]. In addition, a larger version of the spectrum with absorption greater than 90% are shown in Fig. 2(b), it can be seen that a high absorptivity of more than 99% is achieved in the range of 1.834 THz to 3.155 THz (bandwidth 1.321 THz). There are two resonance absorption peaks at 2.05 THz and 3.08 THz, which are 100% and 99.55%, respectively. In order to analyze the mechanism of broadband perfect absorption, we plotted the surface electric field distributions in the x-y plane of EZ and surface current distributions at 2.05 THz, 2.5 THz, 3.08 THz and 3.155 THz frequencies, respectively, as shown in Figs. 2(c)–2(f). It can be seen from Figs. 2(c) and 2(e) that the obvious electric dipole resonance occurs at the positions of the two formants supported by the helical rings. The electric field is mainly concentrated on the helical rings and the positive and negative charges are distributed on both sides of the x-direction. However, the direction of the surface current at the second resonant frequency is opposite to that at the first resonant frequency. Therefore, we selected the surface electric field and current distribution at the intermediate frequency of 2.5 THz to help the analysis as shown in Fig. 2(d). It can be seen that the distribution of positive and negative charge positions at 2.5 THz is opposite to that at 2.05 THz. The change of the positions of positive and negative charges in the resonator is the main reason for the change of the direction of the surface current. In addition, it can be seen from Fig. 2(f) that the distribution of positive and negative charges in the innermost turn at 3.155 THz has a slight counterclockwise shift compared with that at 3.08 THz. From this we can deduce that the positive and negative charges will migrate counterclockwise along the helix as the frequency increases in the whole broadband perfect absorption frequency range. The combination of multiple modes of electric dipole resonance ensures the broadband perfect absorption characteristics of the absorber.
Impedance matching theory is used to further explain the physical mechanism of broadband absorption [59,60], which can be expressed as
The influences of the insulator-to-metal transition (IMT) property of VO2 on broadband absorption are also discussed. Figure 4(a) shows that when the Fermi level of graphene is fixed at 0.01 eV and the conductivity of VO2 is adjusted from 200000 S/m (metal phase) to 200 S/m (insulator phase), the absorber can gradually change from broadband perfect absorption to perfect reflection. In this regard, we selected the x-y plane electric field diagram when the conductivities are 200S/m, 2000S/m, 20000S/m and 200000S/m as shown in Figs. 4(b)–4(e). It can be seen that the electric field in the whole helical region is weak when the conductivity of VO2 is 200 S/m and 2000 S/m.The strong electric field is concentrated at the tip of the innermost turn ofthe helix when the conductivity is increased to 20000 S/m, and there is a strong electric field in the whole helical region when the conductivity is set to 200000 S/m, which is consistent with the description in Fig. 4(a). In addition, the IMT property of VO2 can be achieved by changing temperature [61,62]. According to the relationship between dielectric function and conductivity of materials [63], the functional relationship between the conductivity of VO2 corresponding to different temperatures in the phase transformation process can be obtained as
where ɛ0 is the vacuum permittivity and ɛc is the temperature dependent permittivity.Figure 4(f) shows the curve of VO2 changing with temperature, and the change process is reversible. Nevertheless, there is obvious thermal hysteresis effect in the curve, and there is a certain temperature difference ΔT between the heating curve and the cooling curve. This dynamically adjustable property of the absorber can be applied to modulation techniques, the modulation depth (MD) and extinction ratio (ER) are important indicators of a modulator [64,65], which can be expressed as
Furthermore, the simulated absorption spectra of the absorber as a function of the Fermi energy are presented in Fig. 5(a), as the Fermi level of graphene changes from 0.01 eV to 0.7 eV, the absorber gradually evolves from broadband absorption to dual-band absorption. Formant λ1 and λ2 have blue shift as the Fermi energy level of graphene increases is shown in Fig. 5(b), and the maximum adjustment range of absorption of λ1 and λ2 ranges from 21.8%-67% and 24.8%-95.5%, respectively. In order to analyze the reasons for the formation of the two formants, the three-dimensional surface electric field diagram of the formants λ1 and λ2 were selected at the Fermi level of 0.6 eV. The electric field distribution of λ1 is mainly concentrated on the four diagonals of the graphene layer, and is strongly confined to the interface between the graphene layer and topas layer, indicating that localized surface plasmon-polaritons (LSPP) and propagating surface plasmon-polaritons (PSPP) are excited simultaneously. The resonance principle of λ2 is basically similar to that of λ1, but it has more resonance regions than that of λ1, which is also consistent with the fact that the absorption strength of λ2 is higher than that of λ1.
In addition, it is necessary to analyze the chiral characteristics of the designed absorber due to the asymmetry of the helical structure. Circular dichroism (CD) spectroscopy is a common method to characterize chirality by measuring the differential absorption of LCP light and RCP light. In this paper, the extinction cross-section of the structure was calculated to obtain the CD spectrum. The extinction cross-section excited by LCP and RCP is shown in Fig. 6(a), while the CD spectrum is defined as the difference between the extinction cross section excited by LCP and RCP, as shown in Fig. 6(b). Nevertheless, the extinction cross-section σext is composed of two parts, the first is absorption cross section σabs and the second is scattering cross section σsc [66], which can be expressed as
4. Conclusions
In conclusion, we present a high-performance broadband terahertz wave absorber platform with dynamically electrical and thermal tunable absorption due to the management on the resonant properties via the external surroundings. We then numerically demonstrate the realization of multifunctional manipulations on such absorber. A wide-frequency terahertz perfect absorber with the operation frequency ranges from 1.594 THz to 3.272 THz with absorption intensity over 90% is achieved. The spectral frequency bandwidth exceeding of 1.321 THz with the absorption over 99% is also obtained when the conductivity of VO2 is set to 100000 S/m (metal phase) and the Fermi level of graphene is 0.01 eV. Moreover, the absorption can be artificially changed from 0 to 99.98% and in verse by adjusting the conductivity of VO2. In addition, the spectral absorption is feasible to be changed from wideband absorption to dual-band absorption by adjusting the Fermi level of graphene. Besides, the analysis of the chiral characteristics of the helical structure suggests that the extinction cross-section has a circular dichroic response. During the study, the impedance matching theory is introduced to analyze and elucidate the wideband absorption rate. Our results may introduce approaches to manipulate the wide-band terahertz wave with multiple ways and pave the way towards the development of advanced technologies in the fields of switches, modulators, and imaging devices.
Funding
National Natural Science Foundation of China (11804134, 62065007, 62275112); Natural Science Foundation of Jiangxi Province (JXSQ2019201058).
Disclosures
The authors declare no conflicts of interest.
Data availability
The data that support the findings of this study are available from the corresponding authors upon reasonable request.
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