Abstract
We demonstrate the generation of high-quality tunable terahertz (THz) vortices in an eigenmode by employing soft-aperture difference frequency generation of vortex and Gaussian modes. The generated THz vortex output exhibits a high-quality orbital angular momentum (OAM) mode with a topological charge of ℓTHz = ±1 in a frequency range of 2-6 THz. The maximum average power of the THz vortex output obtained was ∼3.3 µW at 4 THz.
© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
1. Introduction
A terahertz (THz) wave with a low photon energy within the range of 1-30 meV enables the assignment of intermolecular vibrations or cluster-cluster interactions [1–7], and offers a variety of fundamental and applied sciences, so-called THz photonics, such as the morphological change of polymers [8], orientation control of orbital ordering planes in strongly correlated materials [9], and structural analysis of crystalline objects [10–14]. An optical vortex [15–20] possesses unique properties, such as an annular spatial profile and an orbital angular momentum (OAM), characterized by a topological charge ℓ, associated with its helical wavefront. Thus, it has been widely studied in many applications, including optical trapping and manipulation [21–26], ultrahigh density telecommunications [27–31], nonlinear spectroscopy [32–34], the fabrication of chiral materials [35–42], and super-resolution microscopy [43–47]. Going beyond conventional THz photonics, THz vortex modes will open doors towards entirely advanced technologies, for instance, 2-dimensional THz imaging systems for structural identification of biomaterials with an ultrahigh spatial resolution beyond the diffraction limit.
To date, several artificially designed devices to generate THz vortex modes have been proposed, such as a molded phase plate composed of V-shaped slit antennas [48], a circular array antenna [49], an achromatic polarization device [50], and a binary diffractive element [51]. However, their conversion efficiencies from an incident Gaussian beam to an optical vortex mode are typically limited to a few percent owing to their narrow spectral bandwidth and low transmittance. Also, liquid crystal q-plates enable us to generate broadband THz vortices [52,53]. However, they exhibit relatively low damage threshold, and severe transmission loss. Furthermore, their bandwidths are not still enough to develop tunable THz vortex sources.
In recent years, we have developed a spiral phase plate (SPP) formed of a polymeric material, dubbed Tsurupica, with an extremely low-frequency dispersion (dn/dν = –5.1×10−4 /THz) and high transmission (0.4–0.94 cm−1) in the THz frequency region (1–6 THz), and we have successfully generated monochromatic 2 and 4 THz vortex outputs with topological charges of ℓ = 1 and 2 at high conversion efficiencies of over 70% and 50%, respectively [54]. The generation of a monocycle THz vortex mode [55] with ultrahigh intensity has also been demonstrated by employing the SPP in combination with tilted-pulse-front optical rectification [56]. Such a SPP is typically designed for a specific frequency; therefore, it inherently constrains the wavelength tunability of the THz vortex modes. This also leads to undesired higher-order radial Laguerre-Gaussian (LGp,ℓ) components [57], described by a radial index p, which thus degrades the mode quality of the generated vortex modes associated to the index ℓ.
An alternative route to generate the THz vortex mode is to use optical vortex pumped difference frequency generation (DFG). We have successfully developed mid-infrared optical vortex sources based on 2 µm optical vortex laser-pumped DFG with a moderate (millijoule level) pulse energy [58,59] and an extremely wide tunability over the entire mid-infrared region (6–18 µm) [60]. However, there is little discussion of the mode purity in an eigenmode of the vortex output generated from the DFG.
Here, we extend our previous mid-infrared optical vortex work to generate a tunable THz vortex mode with high quality in an eigenmode. This is the first demonstration of tunable THz vortex generation with a frequency range of 2–6 THz, based on the optical vortex-pumped DFG from a 4’-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST) crystal. The generated vortex mode exhibits ultrahigh mode purity (estimated mode purity of >90%) by soft aperture effects for the removal of undesired higher-order radial modes due to the spatial overlap between the vortex and Gaussian pump beams in the soft-aperture DFG.
2. Experiments
2.1 Setup
Figure 1(a) shows the experimental setup of the tunable THz vortex source. An in-house-built picosecond laser (wavelength: 1064 nm, average output power: ∼5 W, pulse width: 8.3 ps, pulse repetition frequency (PRF): 1 MHz) was used as a pump laser, and its output was delivered to two injection-seeded optical parametric amplifiers (OPA1 & 2) formed of two periodically poled stoichiometric lithium tantalite (PPSLT) crystals with a fan-out grating (15×1×35 mm, Λ = 29–31 µm) [61]. The OPA1 output was converted into a first-order optical vortex (ℓ = 1) using an SPP (Fig. 1(b)), and the wavelength, λ1, was then fixed to be 1.56 µm.
The OPA2 output exhibited a Gaussian spatial form (Fig. 1(c)), and its wavelength, λ2, was tuned within the wavelength range of 1.50–1.64 µm by translating the PPSLT crystal with a fan-out grating along the x-axis (as shown in Fig. 1) and controlling the lasing wavelength of the seed laser, an external cavity diode laser (ECDL; Anritsu, MG9541A). Both OPA1 and OPA2 outputs were then spatially overlapped and focused onto the DAST crystal, obtaining a ∼170 µm diameter spot size thus facilitating the generation of a THz vortex beam by means of DFG type-0 geometry (all optical fields involved in the process have the same polarization). The frequency of the generated THz output with this system was seamlessly tuned within the frequency range of 2–6 THz. The pump beams used exhibited a linewidth of ∼60 GHz, thus, the resulting THz vortex should exhibit a linewidth of less than double of ∼ 120 GHz.
2.2 Results
A general relationship,
The generated vortex mode exhibited a single ringed (p = 0) intensity profile for both the near-field and far-field (focused plane), which indicates the high quality in an eigenmode, as shown in Fig. 3. The topological charge was also assigned to be ± 1, as evidenced by the left or right diagonal Hermite-Gaussian mode HG0,1, produced by the astigmatic focusing optics [64,65]. Such a high-quality vortex mode without undesired higher-order radial modes could be generated by the soft-aperture effects in the DFG. Figure 4 summarizes the spatial profiles of the focused vortex modes at various frequencies. Though it is difficult to identify the annular spatial form of 2 THz vortex output owing to the relatively low sensitivity of THz camera for 2 THz [66], the system does not impact the vortex output generation at a frequency below 2THz.
3. Discussion
A conventional SPP provides only an azimuthal phase shift of 2ℓπ to a fundamental Gaussian beam. Thus, the generated vortex output typically includes undesirable higher-order radial Laguerre-Gaussian (LGp,ℓ) modes with radial index p and topological charge ℓ [57]. The electric field uvortex(r, ϕ, ω), of the vortex output with a beam radius of ω is then given by:
In the present system, a vortex output with a wavelength of λ1 (OPA1 output) and a Gaussian beam with a wavelength of λ2 (OPA2 output) are focused and spatially overlapped on a nonlinear crystal, i.e. far-field, in which the individual radial modes with multiple rings (p + 1) in the vortex output (OPA1 output) are spatially separated, to generate the THz vortex mode via DFG (Fig. 5(a)). The resulting DFG vortex output is expressed as:
Figure 6(a) shows the simulated spatial profile of the focused vortex mode generated by the SPP. The individual high-order radial LG modes included in the optical vortex are spatially separated, thereby forming a thick ring. They are removed by the soft-aperture effect of DFG, so as to produce the high quality THz vortex output in an eigenmode. In fact, the undesired higher-order radial modes are fully suppressed in the experimental THz vortex due to the soft-aperture DFG effect, as shown in Fig. 6(b). It is still difficult to further discuss the mode purity of the vortex output, for instance, OAM decomposition approach [67], owing to the absence of a commercial spatial light modulator (SLM) in the THz region.
It should also be noted that strong focusing of the vortex and Gaussian beams degrades the spatial quality of the THz vortex output. When the focused beam radii, ω1 and ω2, were ∼60 µm (these values were smaller than the wavelength of the generated THz output), the resultant THz output showed a Gaussian profile, as shown in Fig. 7(b).
4. Conclusion
We have demonstrated, for the first time to the best of our knowledge, the generation of a widely tunable THz vortex output with high quality in an eigenmode by employing soft-aperture DFG of vortex and Gaussian beams. The system enabled the production of a high-quality THz vortex mode with ℓTHz = ±1 within the frequency range of 2‒6 THz. Such a tunable THz vortex source with high quality in an eigenmode will pave the way towards new advanced technologies, such as 2-dimensional identification of the crystallinity and polymorphism of organic crystals with high spatial resolution beyond the diffraction limit. This proposed method based on DFG should be easily extended to freely synthesize any THz wavefront, such as higher-order LG, Bessel, and Airy wavefronts, by freely modulating the wavefront of the pump beam using an SLM [68,69].
Our current system enables us to provide only one polarized state, however, it should be potentially extended to generate two orthogonally polarized eigen states by employing additional polarization elements or parallel DFGs with different polarization states. Thus, the generation of Poincaré modes, for instance a vector vortex mode, superimposed by two orthogonally polarized eigen states, will be possible as a future work.
Appendix
THz vortex output with topological charge ℓTHz = ±2
There is no theoretical limitation for the topological charge ℓ of generated vortex modes. In fact, high quality second-order THz vortex outputs with a single ring without any undesired multiple outer rings, were also obtained (Figs. 8(a), (b)). Their topological charges were also assigned to be ℓTHz = ±2 by the focusing method with the inclined lens (Figs. 8(c), (d)). These indicate that our proposed approach allows us to generate the higher-order THz vortex modes with high quality.
In general, the OPA1 output with a larger ℓ, created by using the SPP, exhibits a larger focal spot on the DAST crystal, thereby resulting in less spatial overlap with the OPA 2 output with the Gaussian profile. It is noteworthy that the DFG efficiency is expected to decrease as the increase of topological charge of ℓ. In fact, the optical-optical efficiency of the second-order vortex output was measured to be ∼2.3×10−4%.
Funding
Japan Society for the Promotion of Science (16H06507, 18H03884, 19K05299).
Disclosures
The authors declare no conflicts of interest.
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