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Active phase-nulling of the self-mixing phase in a terahertz frequency quantum cascade laser

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Abstract

We demonstrate an active phase-nulling scheme for terahertz (THz) frequency quantum cascade lasers (QCLs) under optical feedback, by active electronic feedback control of the emission frequency. Using this scheme, the frequency tuning rate of a THz QCL is characterized, with significantly reduced experimental complexity compared to alternative approaches. Furthermore, we demonstrate real-time displacement sensing of targets, overcoming the resolution limits imposed by quantization in previously implemented fringe-counting methods. Our approach is readily applicable to high-frequency vibrometry and surface profiling of targets, as well as frequency-stabilization schemes for THz QCLs.

© 2015 Optical Society of America

Self-mixing (SM) interferometry [1] using quantum cascade lasers (QCLs) [2] has recently emerged as a powerful sensing technique in the terahertz (THz) frequency range. The SM scheme is based on the optical feedback (OF) of radiation coupled back into the laser cavity, where it mixes with the intracavity field causing measurable perturbations to the laser operating parameters [3]. Amongst the principal benefits of the SM scheme is the ability to probe the electric field reflected from remote targets coherently through the laser compliance voltage, thereby removing the need for an external detector and enabling the development of compact sensing systems. This is particularly beneficial at THz frequencies owing to a lack of mature technologies that provide fast, sensitive, and compact coherent detection capability. These benefits, in addition to the noninvasive nature of the SM scheme, have recently stimulated its application to displacement sensing [4], velocimetry [5], two- and three-dimensional imaging [69], and materials analysis [10] at THz frequencies. In addition, SM has been applied to study the fundamental properties of THz QCLs, including measurement of the linewidth enhancement factor [4,11] and investigation of the intrinsic stability of QCLs under optical reinjection [12]. In all SM studies to date, however, the QCL has been operated under free-running conditions without any electronic feedback control. In contrast, feedback control schemes for near-infrared lasers under OF have been demonstrated as powerful tools for applications including sub-wavelength displacement sensing of targets [13], and noncontact vibrometry of vehicles [14].

In this work, we develop an active phase-nulling scheme for THz QCLs under OF, through electronic feedback control of the emission frequency. We first apply this method to measurement of the frequency tuning of a laser as a function of drive current. Such characterization is essential for many applications, including gas spectroscopy, and frequency-modulated approaches to imaging and materials analysis using THz QCLs. In addition to offering real-time capability, our measurement approach provides a greatly reduced experimental complexity compared to previously reported schemes for characterizing frequency tuning in QCLs—these typically require detection of the high-frequency beat note generated by mixing the QCL field with that derived from a local oscillator source (either a second QCL [15,16] or an optically pumped gas laser [17,18]) on a diode mixer. In contrast to these approaches, which are restricted to the operating frequency range of the mixer, our technique can be applied across the full 1.2–5.2 THz spectral coverage range of THz QCLs. We also demonstrate that our phase-nulling scheme can be applied to real-time displacement sensing of targets. This scheme achieves all of the advantages of previous SM-based displacement sensors whilst overcoming the resolution limits imposed by the quantization associated with fringe counting methods [19,20] and simultaneously avoiding the need for parametric fitting to an OF model in post-processing [4].

A schematic diagram of our system is shown in Fig. 1. The THz QCL consisted of a 10-μm-thick bound-to-continuum active region [21], which was processed into a semi-insulating surface-plasmon ridge waveguide with dimensions 3mm×140μm. Measurements of the emission spectrum of the isolated laser, performed using a Fourier-transform infrared spectrometer with a spectral resolution of 7.5 GHz, revealed emission in a single longitudinal mode at a frequency, ν02.62THz (λ114μm) for all driving currents, at a heat sink temperature of 25 K. Radiation from the laser was focused onto a gold planar mirror using a pair of f/2 off-axis parabolic reflectors and coupled back into the QCL facet along the same optical path as the emitted beam. The planar mirror was mounted on a computer-controlled translation stage to enable mechanical modulation of the external cavity length around its mean value L0=0.41m. The mirror position was recorded in real-time at a sampling rate of 10 kS/s through the analogue output of the stage encoder. An externally modulated current source was used to drive the laser with an electronically conditioned dynamic feedback current Δi superimposed on a quiescent current of i0=1080mA (=1.08ith). The SM signal (VSM) was monitored using the QCL terminal voltage, which was amplified using a 15-dB dc-coupled voltage amplifier following subtraction of a dc voltage offset.

 figure: Fig. 1.

Fig. 1. Schematic diagram of the experimental system. A control signal Vout is generated by a PI loop filter (transfer function ALF) acting on the self-mixing voltage VSM. The current driver (transconductance G) causes a corresponding perturbation to the QCL driving current Δi, leading to active phase-nulling of VSM. The dashed box indicates the compensation loop used to cancel voltage modulation of the laser. LPF—low pass filter.

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Under constant current operation (i.e., without electronic feedback control), the laser under OF experiences a perturbation to the laser terminal voltage, producing a series of fringes described by the equation VSM=βcos(ϕ), in which β is the modulation index and ϕ is the external round-trip phase given by ϕ=4πLν/c, with ν being the emission frequency under OF and c the speed of light in vacuum [22]. It follows that the phase change Δϕ arising from a change in external cavity length ΔL can be compensated by an electronic feedback loop acting on the QCL emission frequency [13]. In this case, the condition Δϕ=0 holds, enabling an expression for the corresponding tuning of the emission frequency Δν to be obtained. For small perturbations this can be expressed as

Δνν0=ΔLL0.

In our active phase-nulling scheme, the amplified SM signal VSM was conditioned into an appropriate feedback control signal using an adjustable proportional−integral (PI) loop filter. A dc offset stage at the input to this filter enabled precision control of the fringe locking position VSM0, such that the error signal Verror=VSMVSM00 under appropriate feedback control. The local slope of the SM fringe around this locking position determines the optimum loop parameters for feedback control, with the fringe shape itself being dependent in particular upon the feedback parameter [3], which was determined to be C0.25 in our case. However, it is anticipated that this scheme would also operate under moderate feedback (C>1) [14]. The transfer function of the PI filter, ALF, was tuned empirically to provide 0 dB of proportional gain for frequencies f>1kHz, and integral gain with a slope 10 dB/decade below this corner frequency. The filter output, Vout, was fed into the modulation input of the current driver to control dynamically the driving current. The resulting current perturbation is given by Δi=GVout=GALFVerror, in which G=200mA/V is the transconductance of the current driver across its 65-kHz bandwidth. The corresponding change in emission frequency of the QCL under electronic feedback can therefore be expressed as

Δν=kΔi=kGVout,
where k is the frequency tuning rate of the QCL. In addition to this frequency tuning effect, the applied current perturbation also causes a direct modulation of the QCL terminal voltage through the differential resistance of the device, R. For small perturbations around the operating point of the laser, R can be approximated as being constant. This unwanted component of voltage modulation can therefore be subtracted from the input to the loop filter by use of an adjustable inverting amplifier stage acting on the filter output Vout, as shown by the dashed box in Fig. 1. This compensation loop was tuned to provide the necessary amplification, A=RG0.7, by applying a 30-mA ramp modulation to the driving current of the laser without OF, and adjusting the amplifier such that its output matched the resulting modulation of the QCL voltage.

Figure 2(b) shows the error signal Verror obtained in response to a modulation of the external cavity length, without feedback control of the QCL. In this example the cavity length was increased at a rate of 60μm/s with a peak mirror displacement ΔL25μm (corresponding to approximately half a fringe), as shown in Fig. 2(a). As expected, under open-loop operation, the SM signal VSM(and hence Verror) varies according to the external round-trip phase ϕ, as described above. By contrast Fig. 2(b) also shows Verror obtained in the closed-loop condition, along with the corresponding control signal Vout [Fig. 2(c)]. In this case, the SM voltage is maintained at a constant value as the feedback loop acts to compensate for the varying round-trip phase by dynamic control of the laser emission frequency. The resulting time-dependent frequency excursion of the laser can be deduced from the recorded mirror trajectory ΔL by use of Eq. (1). By correlating this with the measured control signal, the frequency tuning can be mapped as a function of current perturbation Δi, enabling the tuning rate k to be determined using Eq. (2). The relationship between Δi and Δν obtained in this way is shown in Fig. 3. From a linear fit to this data, a value k=8.2MHz/mA is found, consistent with the range of values reported for other THz QCLs [23].

 figure: Fig. 2.

Fig. 2. (a) Change in cavity length ΔL. (b) Corresponding error signal Verror measured without (red, dashed) and with (blue, solid) electronic feedback control of the QCL. (c) Corresponding feedback control signal generated by the PI filter.

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 figure: Fig. 3.

Fig. 3. Frequency tuning Δν of the QCL arising from a current perturbation Δi, as determined from the feedback control signal Vout measured in response to a modulation of the external cavity length. A linear fit to the data (red, dashed line) yields a tuning rate k=8.2MHz/mA. Inset: relationship between driving current and Δν determined using a swept-frequency interferometric measurement (blue circles). A linear fit to this data (red, solid line) yields a tuning rate k=8.5MHz/mA.

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To validate further our technique, the tuning rate was also measured using an alternative, nonreal-time method based on that described in Ref. [10]. Briefly, this swept-frequency interferometric method employs a linear frequency modulation of the QCL under OF, thereby generating a series of SM fringes on the terminal voltage. By tracking the phase of these fringes over a series of known cavity lengths, the relationship between driving current and the corresponding frequency tuning of the laser can be obtained in an analogous fashion to that reported here. The results of this analysis are shown in the inset to Fig. 3, for which a value k=8.5MHz/mA is obtained, in good agreement with the value measured using our real-time electronic feedback approach.

As a second demonstration of our scheme, we have applied it to the reciprocal modality, namely the real-time displacement sensing of targets. In this case, the filter output Vout generated in response to a moving target represents a replica of the target displacement, scaled by the responsivity factor R=ν0/kGL0=3.9V/mm according to Eqs. (1) and (2), and using the value k=8.2MHz/mA. Figure 4(a) shows the displacement measured over two oscillation cycles of a mirror vibrating at 2 Hz with a peak-to-peak displacement, D=22.5μm. This SM measurement yields a value of D=23.1μm, representing an error of only 2.5%. From Fourier analysis of the filter output signal, the noise equivalent displacement was found to be 0.2μm for a 1-Hz measurement bandwidth centered around the oscillation frequency of 2 Hz. In addition, the maximum displacement error recorded over the full range of displacement was determined to be 2.5μm [see Fig. 4(b)]. We attribute this displacement error primarily to the voltage-dependent differential resistance of the device causing incomplete subtraction of the laser voltage modulation by the compensation loop. This same effect also determines the practical current modulation amplitude to be 30mA in our system, which corresponds to a measurable displacement amplitude of 40μm. It is worth emphasizing, though, that with correct nonlinear compensation of the QCL voltage modulation (using a digital synthesizer, for example), the useful current modulation range could be extended up to the mode-hop-free tuning range of the laser under OF, which is 100mA in our case. Furthermore, the operating range of the electronic feedback loop in our system is expected to be AOLλ/2=3.6cm [13] for an open-loop gain AOL=4πLβkGALF/c=630, suggesting much greater displacement amplitudes could, in principle, be measured using our technique.

 figure: Fig. 4.

Fig. 4. (a) Displacement (blue, solid line) determined from the feedback control signal Vout, in response to two oscillation cycles of a target vibrating at 2 Hz with a peak-to-peak displacement of 22.5 μm (actual displacement shown by the red, dashed line). (b) Displacement error determined from the difference between the measured and actual displacements.

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In summary, we have demonstrated an active phase-nulling scheme for THz QCLs under OF, through electronic feedback control of the emission frequency. This scheme has been applied successfully to real-time measurement of the frequency tuning rate of a QCL, and offers significantly reduced experimental complexity compared to alternative measurement approaches. In addition, we have demonstrated an alternative modality in which the position of a moving target is replicated on the output voltage of our instrument in real-time and with a noise equivalent displacement of 0.2μm (λ/570). In this regard, it is worth noting that the speed of response to OF is fundamentally determined by elastic and inelastic scattering mechanisms that occur on picosecond time scales in THz QCLs, thereby enabling response bandwidths on the order of 10100GHz, in principle. As such, this scheme could be extended readily to high-frequency vibrometry applications, with the maximum frequency response being determined, in practice, by the loop filter bandwidth. This same approach could equally be applied to the surface profiling of targets; in this case, the output voltage would portray the surface morphology as the target is scanned laterally through the focussed beam. Finally, we note that the electronic feedback approach reported here would also be applicable to frequency-stabilization schemes for THz QCLs, for which frequency drifts can occur on the scale of several MHz (1 part in 105106) over time-scales of seconds, [15,17,24]. For example, according to Eq. (1), frequency stabilization to 1 part in 107 would be possible using our scheme with a 10-m external cavity stable to within 1 μm.

The authors acknowledge support from the EPSRC (UK), the ERC programme “TOSCA,” the Royal Society and the Wolfson Foundation, and the European Cooperation in Science and Technology (COST) Action BM1205. This research was supported under Australian Research Council’s Discovery Projects funding scheme (DP 120 103703). Y. L. L. acknowledges support under the Queensland Government’s Smart Futures Fellowships programme.

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Figures (4)

Fig. 1.
Fig. 1. Schematic diagram of the experimental system. A control signal V out is generated by a PI loop filter (transfer function A LF ) acting on the self-mixing voltage V SM . The current driver (transconductance G ) causes a corresponding perturbation to the QCL driving current Δ i , leading to active phase-nulling of V SM . The dashed box indicates the compensation loop used to cancel voltage modulation of the laser. LPF—low pass filter.
Fig. 2.
Fig. 2. (a) Change in cavity length Δ L . (b) Corresponding error signal V error measured without (red, dashed) and with (blue, solid) electronic feedback control of the QCL. (c) Corresponding feedback control signal generated by the PI filter.
Fig. 3.
Fig. 3. Frequency tuning Δ ν of the QCL arising from a current perturbation Δ i , as determined from the feedback control signal V out measured in response to a modulation of the external cavity length. A linear fit to the data (red, dashed line) yields a tuning rate k = 8.2 MHz / mA . Inset: relationship between driving current and Δ ν determined using a swept-frequency interferometric measurement (blue circles). A linear fit to this data (red, solid line) yields a tuning rate k = 8.5 MHz / mA .
Fig. 4.
Fig. 4. (a) Displacement (blue, solid line) determined from the feedback control signal V out , in response to two oscillation cycles of a target vibrating at 2 Hz with a peak-to-peak displacement of 22.5 μm (actual displacement shown by the red, dashed line). (b) Displacement error determined from the difference between the measured and actual displacements.

Equations (2)

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Δ ν ν 0 = Δ L L 0 .
Δ ν = k Δ i = k G V out ,
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