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Mode-selective O-H stretching relaxation in a hydrogen bond studied by ultrafast vibrational spectroscopy

W. Werncke, V. Kozich, J. Dreyer, S. Ashihara, and T. Elsaesser

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Abstract

The 200 fs decay of O-H stretching population in an intramolecular hydrogen bond is governed by mode-selective excitation of fingerprint modes with a significant O-H bending character, followed by energy randomization within 10 ps.

© 2006 Optical Society of America

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