Wavelength, intensity and chirp are used to control impulsive generation and detection of I3’ ground state vibrational coherences. Intensity harmonic switching, sub- 1/v2 dependence of second harmonic T*2(vib), and phase space mapping of vibrational coherences by chirped probing are demonstrated.

© 2000 Optical Society of America

PDF Article


You do not have subscription access to this journal. Citation lists with outbound citation links are available to subscribers only. You may subscribe either as an OSA member, or as an authorized user of your institution.

Contact your librarian or system administrator
Login to access OSA Member Subscription