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Ultrafast Dephasing of Resorufin in D-Ethanol Glass from 1.8 - 35 K Studied by Incoherent Photon-Echo

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Abstract

Optical dephasing studies of organic glasses and polymers provide the valuable information about an amorphous system’s dynamics. In the recent years hole-burning and two-pulse picosecond photon-echo were widely used for these purposes. These methods have different characteristic times: minutes and more - for hole-burning, picoseconds - for two-pulse picosecond photon-echo. As a result, in the case of amorphous systems, data obtained by using of these methods correspond to different time scales and are not equivalent [1]. The comparison between the results obtained by these different methods can provide additional information about a dynamical processes in amorphous systems (for example, about spectral diffusion).

© 1991 Optical Society of America

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