Characterization of Push-Pull Polyenes of Increasing Size: Linear and Quadratic Polarizabilities in Solution

Alain Fort; Jacques Muller; Joel Azoulay; Marguerite Barzoukas; Valérie Alain; Mireille Blanchard-Desce

doi:10.1364/OTFA.1997.WC.4

Organic Thin Films for Photonics Applications
Technical Digest Series (Optica Publishing Group, 1997),
paper WC.4
•https://doi.org/10.1364/OTFA.1997.WC.4

Characterization of Push-Pull Polyenes of Increasing Size: Linear and Quadratic Polarizabilities in Solution

Alain Fort, Jacques Muller, Joel Azoulay, Marguerite Barzoukas, Valérie Alain, and Mireille Blanchard-Desce

Organic Thin Films for Photonic Applications 1997

Long Beach, California United States
15–17 October 1997
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A. Fort, J. Muller, J. Azoulay, M. Barzoukas, V. Alain, and M. Blanchard-Desce, "Characterization of Push-Pull Polyenes of Increasing Size: Linear and Quadratic Polarizabilities in Solution," in Organic Thin Films for Photonics Applications, Technical Digest Series (Optica Publishing Group, 1997), paper WC.4.

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Abstract

Push-pull molecules have been extensively studied for their properties in the field of quadratic nonlinear optics. Such molecules consist of electron-donor and electron acceptor substituents connected via a conjugation path. The partial intramolecular charge transfer (ICT) between these end groups can lead to large ground-state dipoles μ. Also, they can display huge static quadratic hyperpolarizabilities β(0) related to the occurence of the ICT transition between the ground and first-excited states [1].

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