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New approach to femtosecond spectroscopy in the near infrared

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Abstract

Generation of optical pulses of <100-fs duration and a subsequent amplification at kilohertz repetition rate has been shown to be a powerful technique for nonlinear optical investigations requiring simultaneously high excitation intensities (>1013W/cm2) and sensitive detection (transmission changes of <10−4). It is interesting to extend these techniques to the near-IR region (800-1100 nm). Recently, pulses of <100-fs duration have been produced in the near-IR region at 8601 and 805 nm.2 In the latter case, amplification of 805-nm pulses to microjoule energies has been demonstrated at 6-kHz repetition rate2 using a copper-vapor laser-pumped amplifier, which is similar to that which has been developed for the 625-nm CPM laser wavelength range.2 Continuum generation in ethylene glycol results in broadband white light which is now very intense in the 820-1100-nm region.

© 1987 Optical Society of America

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