Abstract

We demonstrate for the first time, to our knowledge, second harmonic optical phase conjugation, using the second spatial harmonics of a nonsinusoidal grating formed in a photorefractive material. The possibility of harmonic phase conjugation has been considered previously for artificial Kerr media.¹ We have applied the same idea to barium titanate, since the existence of the higher-order gratings in this material has been known to us for some time. In our experiment, two 1.06-µm cw Nd:YAG laser beams wrote a grating in a poled photorefractive barium titanate crystal. Then a second harmonic of the YAG at 0.532 µm read out the grating in a counterpropagating direction to one of the writing beams. In this geometry, the usual Bragg condition is not satisfied. The reflectivity of the 0.532-µm signal was rather weak, ~0.01%, with ~0.1-mW reading beam power. The buildup time was around 3 s, with loosely focused writing beams with 50-mW power in each beam. The same experiment with a SBN crystal showed no significant harmonic phase conjugation. Finally, we stress that this effect is different from the previously published result.²

© 1986 Optical Society of America