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Nonlinear Absorption Spectroscopy of a Bis(Porphyrin)-Substituted Squaraine

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Abstract

The nonlinear absorption mechanisms of a bis(porphyrin)-substituted squaraine have been studied with femtosecond, picosecond, and nanosecond pulsewidths. The two-photon absorption is ~10× larger than those of the constituents and is explained by intra-molecular charge transfer.

© 2009 Optical Society of America

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