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Effects of Doppler Broadening and Unequal Pump Intensities in Saturated Degenerate Four-Wave Mixing Spectroscopy

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Abstract

Degenerate four-wave mixing (DFWM) is a technique that shows great promise for sensitive measurements of transient gas-phase species, and diagnostic applications of DFWM are being pursued actively at laboratories throughout the world. Applications of DFWM as a combustion diagnostic and as a tool for molecular spectroscopy are reviewed in a recent article by Farrow and Rakestraw (1992). However, significant questions remain regarding strategies for quantitative concentration measurements using DFWM.

© 1994 Optical Society of America

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