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Optical-Environment-Dependent Lifetimes and Radiation Patterns of Luminescent Centers in Very Thin Films

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Abstract

The emission from luminescent centers located in a thin film (O) of thickness dO≪λ (where λ is the emission wavelength) is optical-environment-dependent: The raditive lifetimes depend not only on the refractive index nO of the film but also on the indices n1 and n2 of the adjacent media n1 and n2. The angular distributions of the emitted light differ drastically from the well-known multipole radiation patterns. From these electro-dynamical effects informations about the emitting centers can be obtained (determination of quantum efficiencies, multipolarity assignments, orientation of the emission dipoles).1,2

© 1984 Optical Society of America

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