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Controlling the coherent response of arbitrarily shaped plasmonic nanoparticles

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Abstract

We utilize an ultra-broadband pulse-shaper to control the coherent electronic motion in arbitrarily shaped nanoparticles, steering the third-order nonlinear response from destructive to constructive interference. Our results outperform the transform-limited case by a 200% enhancement.

© 2023 The Author(s)

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