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Polarization Sensitive Femtosecond Mid-Infrared Spectrometer Using Chirped-Pulse Upconversion

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Abstract

Polarization sensitive femtosecond mid-infrared spectrometer is developed based on chirped-pulse upconversion. Polarization and frequency dependence of the pump pulse on the vibrational coupling between the CO stretching modes of a metal carbonyl complex reveals the appearance of Raman-active vibrations due to a slight decrease in the molecular symmetry.

© 2018 The Author(s)

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