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Theory of Multiple-Light-Scattering Spectroscopy

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Abstract

We present an algorithm for determining the dielectric autocorrelation function of a disordered medium from angle resolved multiple light scattering measurements. Photons propagating in a disordered, multiple scattering medium are classified as being either ballistic, “snake-like” or diffusive, depending on the nature of their trajectory between source and detector. Considerable information about the nature of the scattering medium is contained in the early arriving snake-like photons whereas this information is smeared in the late-arriving diffusive photons. We derive from first principle a formal mathematical description which encompasses all three regimes of transport and relates the experimentally observed light intensity correlation functions to the ensemble averaged autocorrelation function B˜(x,y)ε*(x)ε(y)ens for a disordered medium with dielectric constant ε(x).

© 1994 Optical Society of America

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