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Long-Wave Mid-Infrared Time-Resolved Dual-Comb Spectroscopy of the Simplest Criegee Intermediate

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Abstract

A long-wave mid-infrared dual-comb spectrometer is constructed and employed to measure transient absorption spectra of the simplest Criegee intermediate (CH2OO) near 8-μm. With time-resolved dual-comb spectroscopy, reaction kinetics of CH2OO with SO2 are also studied.

© 2023 The Author(s)

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