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Pulse Width Induced Crossover of Nonlinear Optical Response in Magnetically Active NiSe2

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Abstract

We demonstrated dominant antiferromagnetic NiSe2 and investigated third-order optical nonlinearities by the Z-scan technique. Pulse-width induced crossover results in excited-state and sequential two-photon absorption, and can be used potentially in advanced optics and photonics devices.

© 2022 The Author(s)

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