Abstract

While many solid-state emitters can be optically excited non-resonantly, resonant excitation is necessary for many quantum information protocols as it often maximizes the non-classicality of the emitted light. Here, we study the resonance fluorescence in a solid-state system—a quantum dot—with the addition of weak, non-resonant light. In the inelastic scattering regime, changes in the resonance fluorescence intensity and linewidth are linked to both the non-resonant and resonant laser powers. Details of the intensity change indicate that charge-carrier loss from the quantum dot is resonant laser. As we enter the Mollow triplet regime, this resonant laser loss term rate is approximately 1/50  ns1. This work further clarifies resonance fluorescence in solid-state systems and will aid in the further improvement of solid-state non-classical light sources.

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    [Crossref]

2018 (1)

A. Reigue, A. Lemaître, C. G. Carbonell, C. Ulysse, K. Merghem, S. Guilet, R. Hostein, and V. Voliotis, “Resonance fluorescence revival in a voltage-controlled semiconductor quantum dot,” Appl. Phys. Lett. 112, 073103 (2018).
[Crossref]

2017 (2)

P. Senellart, G. Solomon, and A. White, “High-performance semiconductor quantum-dot single-photon sources,” Nat. Nanotechnol. 12, 1026–1039 (2017).
[Crossref]

T. Thomay, S. V. Polyakov, O. Gazzano, E. Goldschmidt, V. Loo, and G. S. Solomon, “Simultaneous, full characterization of a single-photon state using semiconductor quantum-dot light,” Phys. Rev. X 7, 041036 (2017).
[Crossref]

2016 (11)

A. Thoma, P. Schnauber, M. Gschrey, M. Seifried, J. Wolters, J.-H. Schulze, A. Strittmatter, S. Rodt, A. Carmele, A. Knorr, T. Heindel, and S. Reitzenstein, “Exploring dephasing of a solid-state quantum emitter via time- and temperature-dependent Hong-Ou-Mandel experiments,” Phys. Rev. Lett. 116, 033601 (2016).
[Crossref]

J. C. Loredo, N. A. Zakaria, N. Somaschi, C. Anton, L. de Santis, V. Giesz, T. Grange, M. A. Broome, O. Gazzano, G. Coppola, I. Sagnes, A. Lemaitre, A. Auffeves, P. Senellart, M. P. Almeida, and A. G. White, “Scalable performance in solid-state single-photon sources,” Optica 3, 433–440 (2016).
[Crossref]

H. Wang, Z.-C. Duan, Y.-H. Li, S. Chen, J.-P. Li, Y.-M. He, M.-C. Chen, Y. He, X. Ding, C.-Z. Peng, C. Schneider, M. Kamp, S. Höfling, C.-Y. Lu, and J.-W. Pan, “Near-transform-limited single photons from an efficient solid-state quantum emitter,” Phys. Rev. Lett. 116, 213601 (2016).
[Crossref]

C. Xiong, X. Zhang, Z. Liu, M. J. Collins, A. Mahendra, L. G. Helt, M. J. Steel, D.-Y. Choi, C. J. Chae, P. H. W. Leong, and B. J. Eggleton, “Active temporal multiplexing of indistinguishable heralded single photons,” Nat. Commun. 7, 10853 (2016).
[Crossref]

D. Chen, G. R. Lander, K. S. Krowpman, G. S. Solomon, and E. B. Flagg, “Characterization of the local charge environment of a single quantum dot via resonance fluorescence,” Phys. Rev. B 93, 115307 (2016).
[Crossref]

O. Gazzano and G. S. Solomon, “Toward optical quantum information processing with quantum dots coupled to microstructures [Invited],” J. Opt. Soc. Am. B 33, C160–C175 (2016).
[Crossref]

N. Somaschi, V. Giesz, L. De Santis, J. C. Loredo, M. P. Almeida, G. Hornecker, S. L. Portalupi, T. Grange, C. Antón, J. Demory, C. Gómez, I. Sagnes, N. D. Lanzillotti-Kimura, A. Lemaítre, A. Auffeves, A. G. White, L. Lanco, and P. Senellart, “Near-optimal single-photon sources in the solid state,” Nat. Photonics 10, 340–345 (2016).
[Crossref]

T. Huber, A. Predojević, G. S. Solomon, and G. Weihs, “Effects of photo-neutralization on the emission properties of quantum dots,” Opt. Express 24, 21794–21801 (2016).
[Crossref]

A. Kurzmann, A. Ludwig, A. D. Wieck, A. Lorke, and M. Geller, “Auger recombination in self-assembled quantum dots: quenching and broadening of the charged exciton transition,” Nano Lett. 16, 3367–3372 (2016).
[Crossref]

A. Kurzmann, B. Merkel, P. A. Labud, A. Ludwig, A. D. Wieck, A. Lorke, and M. Geller, “Optical blocking of electron tunneling into a single self-assembled quantum dot,” Phys. Rev. Lett. 117, 1–5 (2016).
[Crossref]

X. Ding, Y. He, Z.-C. Duan, N. Gregersen, M.-C. Chen, S. Unsleber, S. Maier, C. Schneider, M. Kamp, S. Höfling, C.-Y. Lu, and J.-W. Pan, “On-demand single photons with high extraction efficiency and near-unity indistinguishability from a resonantly driven quantum dot in a micropillar,” Phys. Rev. Lett. 116, 020401 (2016).
[Crossref]

2015 (3)

J. Carolan, C. Harrold, C. Sparrow, E. Martin-Lopez, N. J. Russell, J. W. Silverstone, P. J. Shadbolt, N. Matsuda, M. Oguma, M. Itoh, G. D. Marshall, M. G. Thompson, J. C. F. Matthews, T. Hashimoto, J. L. O’Brien, and A. Laing, “Universal linear optics,” Science 349, 711–716 (2015).
[Crossref]

T. Huber, A. Predojević, D. Föger, G. Solomon, and G. Weihs, “Optimal excitation conditions for indistinguishable photons from quantum dots,” New J. Phys. 17, 123025 (2015).
[Crossref]

A. V. Kuhlmann, J. H. Prechtel, J. Houel, A. Ludwig, D. Reuter, A. D. Wieck, and R. J. Warburton, “Transform-limited single photons from a single quantum dot,” Nat. Commun. 6, 8204 (2015).
[Crossref]

2014 (1)

H. Jayakumar, A. Predojević, T. Kauten, T. Huber, G. S. Solomon, and G. Weihs, “Time-bin entangled photons from a quantum dot,” Nat. Commun. 5, 4251 (2014).
[Crossref]

2013 (5)

M. A. Broome, A. Fedrizzi, S. Rahimi-Keshari, J. Dove, S. Aaronson, T. C. Ralph, and A. G. White, “Photonic Boson sampling in a tunable circuit,” Science 339, 794–798 (2013).
[Crossref]

Y.-M. He, Y. He, Y.-J. Wei, D. Wu, M. Atatüre, C. Schneider, S. Höfling, M. Kamp, C.-Y. Lu, and J.-W. Pan, “On-demand semiconductor single-photon source with near-unity indistinguishability,” Nat. Nanotechnol. 8, 213–217 (2013).
[Crossref]

O. Gazzano, S. Michaelis de Vasconcellos, C. Arnold, A. Nowak, E. Galopin, I. Sagnes, L. Lanco, A. Lemaître, and P. Senellart, “Bright solid-state sources of indistinguishable single photons,” Nat. Commun. 4, 1425 (2013).
[Crossref]

A. Ulhaq, S. Weiler, C. Roy, S. M. Ulrich, M. Jetter, S. Hughes, and P. Michler, “Detuning-dependent Mollow triplet of a coherently-driven single quantum dot,” Opt. Express 21, 4382–4395 (2013).
[Crossref]

H. S. Nguyen, G. Sallen, M. Abbarchi, R. Ferreira, C. Voisin, P. Roussignol, G. Cassabois, and C. Diederichs, “Photoneutralization and slow capture of carriers in quantum dots probed by resonant excitation spectroscopy,” Phys. Rev. B 87, 115305 (2013).
[Crossref]

2012 (4)

J. Houel, A. V. Kuhlmann, L. Greuter, F. Xue, M. Poggio, B. D. Gerardot, P. A. Dalgarno, A. Badolato, P. M. Petroff, A. Ludwig, D. Reuter, A. D. Wieck, and R. J. Warburton, “Probing single-charge fluctuations at a GaAs/AlAs interface using laser spectroscopy on a nearby InGaAs quantum dot,” Phys. Rev. Lett. 108, 107401 (2012).
[Crossref]

H. S. Nguyen, G. Sallen, C. Voisin, P. Roussignol, C. Diederichs, and G. Cassabois, “Optically gated resonant emission of single quantum dots,” Phys. Rev. Lett. 108, 057401 (2012).
[Crossref]

J. Yin, J.-G. Ren, H. Lu, Y. Cao, H.-L. Yong, Y.-P. Wu, C. Liu, S.-K. Liao, F. Zhou, Y. Jiang, X.-D. Cai, P. Xu, G.-S. Pan, J.-J. Jia, Y.-M. Huang, H. Yin, J.-Y. Wang, Y.-A. Chen, C.-Z. Peng, and J.-W. Pan, “Quantum teleportation and entanglement distribution over 100-kilometre free-space channels,” Nature 488, 185–188 (2012).
[Crossref]

E. B. Flagg, S. V. Polyakov, T. Thomay, and G. S. Solomon, “Dynamics of nonclassical light from a single solid-state quantum emitter,” Phys. Rev. Lett. 109, 163601 (2012).
[Crossref]

2011 (1)

L. Robledo, L. Childress, H. Bernien, B. Hensen, P. F. A. Alkemade, and R. Hanson, “High-fidelity projective read-out of a solid-state spin quantum register,” Nature 477, 574–578 (2011).
[Crossref]

2010 (3)

M. Metcalfe, S. M. Carr, A. Muller, G. S. Solomon, and J. Lawall, “Resolved sideband emission of InAs/GaAs quantum dots strained by surface acoustic waves,” Phys. Rev. Lett. 105, 037401 (2010).
[Crossref]

E. Flagg, A. Muller, S. Polyakov, A. Ling, A. Migdall, and G. Solomon, “Interference of single photons from two separate semiconductor quantum dots,” Phys. Rev. Lett. 104, 137401 (2010).
[Crossref]

R. B. Patel, A. J. Bennett, I. Farrer, C. A. Nicoll, D. A. Ritchie, and A. J. Shields, “Two-photon interference of the emission from electrically tunable remote quantum dots,” Nat. Photonics 4, 632–635 (2010).
[Crossref]

2009 (1)

E. B. Flagg, A. Muller, J. W. Robertson, S. Founta, D. G. Deppe, M. Xiao, W. Ma, G. J. Salamo, and C. K. Shih, “Resonantly driven coherent oscillations in a solid-state quantum emitter,” Nat. Phys. 5, 203–207 (2009).
[Crossref]

2008 (1)

A. Muller, W. Fang, J. Lawall, and G. S. Solomon, “Emission spectrum of a dressed exciton-biexciton complex in a semiconductor quantum dot,” Phys. Rev. Lett. 101, 027401 (2008).
[Crossref]

2007 (1)

A. Muller, E. B. Flagg, P. Bianucci, X. Y. Wang, D. G. Deppe, W. Ma, J. Zhang, G. J. Salamo, M. Xiao, and C. K. Shih, “Resonance fluorescence from a coherently driven semiconductor quantum dot in a cavity,” Phys. Rev. Lett. 99, 187402 (2007).
[Crossref]

2006 (1)

A. Berthelot, I. Favero, G. Cassabois, C. Voisin, C. Delalande, P. Roussignol, R. Ferreira, and J. M. Gérard, “Unconventional motional narrowing in the optical spectrum of a semiconductor quantum dot,” Nat. Phys. 2, 759–764 (2006).
[Crossref]

2004 (2)

J. J. Finley, M. Sabathil, P. Vogl, G. Abstreiter, R. Oulton, A. I. Tartakovskii, D. J. Mowbray, M. S. Skolnick, S. L. Liew, A. G. Cullis, and M. Hopkinson, “Quantum-confined Stark shifts of charged exciton complexes in quantum dots,” Phys. Rev. B 70, 201308 (2004).
[Crossref]

A. Kiraz, M. Atatüre, and A. Imamoğlu, “Quantum-dot single-photon sources: prospects for applications in linear optics quantum-information processing,” Phys. Rev. A 69, 1–10 (2004).
[Crossref]

2001 (1)

E. Knill, R. Laflamme, and G. J. Milburn, “A scheme for efficient quantum computation with linear optics,” Nature 409, 46–52 (2001).
[Crossref]

1998 (1)

H. Benisty, H. De Neve, and C. Weisbuch, “Impact of planar microcavity effects on light extraction-Part I: basic concepts and analytical trends,” IEEE J. Quantum Electron. 34, 1612–1631 (1998).
[Crossref]

1997 (1)

J. I. Cirac, P. Zoller, H. J. Kimble, and H. Mabuchi, “Quantum state transfer and entanglement distribution among distant nodes in a quantum network,” Phys. Rev. Lett. 78, 3221–3224 (1997).
[Crossref]

1988 (1)

Y. H. Shih and C. O. Alley, “New type of Einstein-Podolsky-Rosen-Bohm experiment using pairs of light quanta produced by optical parametric down conversion,” Phys. Rev. Lett. 61, 2921–2924 (1988).
[Crossref]

1985 (1)

J. L. Bjorkstam, J. Listerud, M. Villa, and C. I. Massara, “Motional narrowing of a Gaussian NMR line,” J. Magn. Reson. 65, 383–394 (1985).
[Crossref]

1969 (1)

B. Mollow, “Power spectrum of light scattered by two-level systems,” Phys. Rev. 188, 1969–1975 (1969).
[Crossref]

Aaronson, S.

M. A. Broome, A. Fedrizzi, S. Rahimi-Keshari, J. Dove, S. Aaronson, T. C. Ralph, and A. G. White, “Photonic Boson sampling in a tunable circuit,” Science 339, 794–798 (2013).
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Figures (4)

Fig. 1.
Fig. 1. Schematic of the experiment. A single-mode (SM) optical fiber is glued to the cleaved edge of the sample to resonantly excite a QD embedded between two distributed Bragg reflectors (DBR). The light is collected from the sample top surface using a fiber-coupled microscope objective. The weak, 633 nm laser is sent to the sample using the same objective. The Fabry–Pérot filter is bypassed in the resonance fluorescence spectroscopy scans. BS: beam splitter; SPAD: single photon avalanche photodiode.
Fig. 2.
Fig. 2. Characterizing the linewidth. (a), (b) Theoretical fluorescence maps of emission from a QD transition with (a) inhomogeneous or (b) homogeneous broadening. The shape of the intensity distribution in the diagonal ωph=ωL is Gaussian in the inhomogeneous case and Lorentzian in the homogeneous case, as indicated by the white dotted lines. (c) Experimental fluorescence map obtained by sweeping the frequency of a laser ωL and of a Fabry–Pérot filter ωph around the QD frequency, ω0. (d) Shaded curves: resonance fluorescence spectra obtained for different laser frequencies, as indicated by dotted lines in (c). The red dots indicate the resonance fluorescence maximum for each laser frequency. The envelope intensity is Gaussian (black line).
Fig. 3.
Fig. 3. Enhanced intensity and resonant-laser induced loss. (a) Autocorrelation measurements performed under CW resonant excitation and for different Rabi frequencies (i.e., resonant laser powers). (b) Integrated intensity as a function of HeNe power and for several resonant laser powers (red circles: Ωr=0.23  GHz, green squares: Ωr=0.30  GHz, blue diamonds: Ωr=0.47  GHz, violet triangles: Ωr=0.65  GHz). The solid lines represent the simulation; see text for details. The data with Ωr=0.47  GHz (blue diamonds) has an increase of integrated brightness of 17 with respect to its lowest value. The four curves were offset by 5000 counts each for clarity. The HeNe spot size is approximately 1 μm in diameter. (c) Resonance fluorescence excitation spectroscopy of a QD transition for two above-band 633 nm laser powers (red dots: 1.3 nW; blue dots: 40 nW). The intensity is not normalized to show the strong brightness improvement by a factor of 30. (d) Plot of the resonant-laser-induced loss term, obtained by fitting the data with the Monte Carlo simulation, as a function of the Rabi frequency ΩR.
Fig. 4.
Fig. 4. Inhomogeneous linewidth narrowing. (a) Inhomogeneous linewidth of the resonance fluorescence spectra as a function of HeNe power for several resonant laser powers (red circles: Ωr=0.23  GHz, green squares: Ωr=0.30  GHz, blue diamonds: Ωr=0.47  GHz, violet triangles: Ωr=0.65  GHz). The QD inhomogeneous linewidth decreases with increased HeNe power. The decrease is slower for higher resonant laser powers. The solid lines represent exponential fits. (b) Resonance fluorescence spectrum of a QD transition for two above-band 633 nm laser powers (red dots: 1.3 nW; blue dots: 100 nW). The intensity is normalized to show the inhomogeneous linewidth narrowing.

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