Abstract

Industrial fabrication of Mn-doped CdS/ZnS core/shell nanocrystals (NCs) was conducted using a one-pot method, and the NCs’ fluorescence peak could be varied from 564 to 616 nm by changing the Mn2+ doping process and ZnS shell thickness. The synthesis parameters were optimized to increase the NCs’ output, and ~10 g of NCs could be yielded in 1.5 L of solution. A reverse microemulsion method was used to encapsulate these CdS:Mn/ZnS NCs with SiO2 aerosols to improve their photostability in white-light-emitting diodes (WLEDs). A yield of ~3 × 106 1 W WLEDs was obtained by enveloping blue chips with CdS:Mn/ZnS@SiO2 NCs and YAG:Ce3+ is helpful to industrialization; the WLEDs’ color rendering index and luminous efficiency were 88 and 108 lm/W, respectively.

© 2015 Optical Society of America

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References

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    [Crossref]
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    [Crossref]
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    [Crossref] [PubMed]

2014 (4)

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

J. Yoon, Y. Kim, N. Kim, C. Jhun, S. Lee, Y. Kim, F. Zhu, and W. Kim, “Realization of high-performance blue organic light-emitting diodes using multi-emissive layers,” Chin. Opt. Lett. 12(1), 012302 (2014).
[Crossref]

J. W. Kim, N. H. Kim, J. A. Yoon, S. I. Yoo, J. S. Kang, and W. Y. Kim, “White phosphorescent organic light-emitting diodes using double emissive layer with three dopants for color stability,” Chin. Opt. Lett. 12(10), 102302 (2014).
[Crossref]

S. R. Alvarado, Y. Guo, T. P. A. Ruberu, E. Tavasoli, and J. Vela, “Inorganic chemistry solutions to semiconductor nanocrystal problems,” Coord. Chem. Rev. 263, 182–196 (2014).
[Crossref]

2013 (3)

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

B. P. Yang, X. C. Shen, H. C. Zhang, Y. P. Cui, and J. Y. Zhang, “Luminescent and Magnetic Properties in Semiconductor Nanocrystals with Radial-Position-Controlled Mn2+ Doping,” J. Phys. Chem. C 117(30), 15829–15834 (2013).
[Crossref]

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
[Crossref]

2012 (1)

X. Wang, X. Yan, W. Li, and K. Sun, “Doped quantum dots for white-light-emitting diodes without reabsorption of multiphase phosphors,” Adv. Mater. 24(20), 2742–2747 (2012).
[Crossref] [PubMed]

2011 (1)

P. Yang, M. Ando, and N. Murase, “Highly luminescent CdSe/CdxZn1-XS quantum dots coated with thickness-controlled SiO2 shell through silanization,” Langmuir 27(15), 9535–9540 (2011).
[Crossref] [PubMed]

2010 (4)

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
[Crossref]

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

J. M. Zhang, X. K. Zhang, and J. Y. Zhang, “Dependence of Microstructure and Luminescence on Shell Layers in Colloidal CdSe/CdS Core/Shell Nanocrystals,” J. Phys. Chem. C 114(9), 3904–3908 (2010).
[Crossref]

2009 (1)

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

2008 (2)

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “On Doping CdS/ZnS Core/Shell Nanocrystals with Mn,” J. Am. Chem. Soc. 130(46), 15649–15661 (2008).
[Crossref] [PubMed]

2007 (3)

Y. H. Yang, L. H. Jing, X. L. Yu, D. D. Yan, and M. Y. Gao, “Coating Aqueous Quantum Dots with Silica via Reverse Microemulsion Method: Toward Size-Controllable and Robust Fluorescent Nanoparticles,” Chem. Mater. 19(17), 4123–4128 (2007).
[Crossref]

S. Ithurria, P. Guyot-Sionnest, B. Mahler, and B. Dubertret, “Mn2+ as a Radial Pressure Gauge in Colloidal Core/Shell Nanocrystals,” Phys. Rev. Lett. 99(26), 265501 (2007).
[Crossref] [PubMed]

N. Pradhan and X. Peng, “Efficient and color-tunable Mn-doped ZnSe nanocrystal emitters: Control of optical performance via greener synthetic chemistry,” J. Am. Chem. Soc. 129(11), 3339–3347 (2007).
[Crossref] [PubMed]

2006 (2)

A. Ishizumi and Y. Kanemitsu, “Luminescence Spectra and Dynamics of Mn-Doped CdS Core/Shell Nanocrystals,” Adv. Mater. 18(8), 1083–1085 (2006).
[Crossref]

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “Radial-Position-Controlled Doping in CdS/ZnS Core/Shell Nanocrystals,” J. Am. Chem. Soc. 128(38), 12428–12429 (2006).
[Crossref] [PubMed]

2004 (2)

H. Yang, P. H. Holloway, G. Cunningham, and K. S. Schanze, “CdS:Mn nanocrystals passivated by ZnS: Synthesis and luminescent Properties,” J. Chem. Phys. 121(20), 10233–10240 (2004).
[Crossref] [PubMed]

Y. Chan, J. P. Zimmer, M. Stroh, J. S. Steckel, R. K. Jain, and M. G. Bawendi, “Incorporation of Luminescent Nanocrystals into Monodisperse Core-Shell Silica Microspheres,” Adv. Mater. 16(23–24), 2092–2097 (2004).
[Crossref]

2001 (1)

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

2000 (1)

J. F. Suyver, S. F. Wuister, J. J. Kelly, and A. Meijerink, “Luminescence of nanocrystalline ZnSe:Mn2+,” Phys. Chem. Chem. Phys. 2(23), 5445–5448 (2000).
[Crossref]

1994 (1)

R. N. Bhargava, D. Gallagher, X. Hong, and A. Nurmikko, “Optical Properties of Manganese-Doped Nanocrystals of ZnS,” Phys. Rev. Lett. 72(3), 416–419 (1994).
[Crossref] [PubMed]

Alvarado, S. R.

S. R. Alvarado, Y. Guo, T. P. A. Ruberu, E. Tavasoli, and J. Vela, “Inorganic chemistry solutions to semiconductor nanocrystal problems,” Coord. Chem. Rev. 263, 182–196 (2014).
[Crossref]

Ando, M.

P. Yang, M. Ando, and N. Murase, “Highly luminescent CdSe/CdxZn1-XS quantum dots coated with thickness-controlled SiO2 shell through silanization,” Langmuir 27(15), 9535–9540 (2011).
[Crossref] [PubMed]

Angerhofer, A.

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “On Doping CdS/ZnS Core/Shell Nanocrystals with Mn,” J. Am. Chem. Soc. 130(46), 15649–15661 (2008).
[Crossref] [PubMed]

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “Radial-Position-Controlled Doping in CdS/ZnS Core/Shell Nanocrystals,” J. Am. Chem. Soc. 128(38), 12428–12429 (2006).
[Crossref] [PubMed]

Bals, S.

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
[Crossref]

Bawendi, M. G.

Y. Chan, J. P. Zimmer, M. Stroh, J. S. Steckel, R. K. Jain, and M. G. Bawendi, “Incorporation of Luminescent Nanocrystals into Monodisperse Core-Shell Silica Microspheres,” Adv. Mater. 16(23–24), 2092–2097 (2004).
[Crossref]

Bhargava, R. N.

R. N. Bhargava, D. Gallagher, X. Hong, and A. Nurmikko, “Optical Properties of Manganese-Doped Nanocrystals of ZnS,” Phys. Rev. Lett. 72(3), 416–419 (1994).
[Crossref] [PubMed]

Bovin, J. O.

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

Brot, S.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Cao, Y. C.

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “On Doping CdS/ZnS Core/Shell Nanocrystals with Mn,” J. Am. Chem. Soc. 130(46), 15649–15661 (2008).
[Crossref] [PubMed]

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “Radial-Position-Controlled Doping in CdS/ZnS Core/Shell Nanocrystals,” J. Am. Chem. Soc. 128(38), 12428–12429 (2006).
[Crossref] [PubMed]

Chan, Y.

Y. Chan, J. P. Zimmer, M. Stroh, J. S. Steckel, R. K. Jain, and M. G. Bawendi, “Incorporation of Luminescent Nanocrystals into Monodisperse Core-Shell Silica Microspheres,” Adv. Mater. 16(23–24), 2092–2097 (2004).
[Crossref]

Chen, O.

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “On Doping CdS/ZnS Core/Shell Nanocrystals with Mn,” J. Am. Chem. Soc. 130(46), 15649–15661 (2008).
[Crossref] [PubMed]

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “Radial-Position-Controlled Doping in CdS/ZnS Core/Shell Nanocrystals,” J. Am. Chem. Soc. 128(38), 12428–12429 (2006).
[Crossref] [PubMed]

Chen, W.

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

Cherian, R.

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

Chowdhury, A.

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

Chu, H. R.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

Cui, J.

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

Cui, T.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

Cui, Y. P.

B. P. Yang, X. C. Shen, H. C. Zhang, Y. P. Cui, and J. Y. Zhang, “Luminescent and Magnetic Properties in Semiconductor Nanocrystals with Radial-Position-Controlled Mn2+ Doping,” J. Phys. Chem. C 117(30), 15829–15834 (2013).
[Crossref]

Cunningham, G.

H. Yang, P. H. Holloway, G. Cunningham, and K. S. Schanze, “CdS:Mn nanocrystals passivated by ZnS: Synthesis and luminescent Properties,” J. Chem. Phys. 121(20), 10233–10240 (2004).
[Crossref] [PubMed]

De, S.

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

de Mello Donega, C.

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
[Crossref]

Debnath, S.

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

Du, Z.

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

Dubertret, B.

S. Ithurria, P. Guyot-Sionnest, B. Mahler, and B. Dubertret, “Mn2+ as a Radial Pressure Gauge in Colloidal Core/Shell Nanocrystals,” Phys. Rev. Lett. 99(26), 265501 (2007).
[Crossref] [PubMed]

Fan, J. B.

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

Gallagher, D.

R. N. Bhargava, D. Gallagher, X. Hong, and A. Nurmikko, “Optical Properties of Manganese-Doped Nanocrystals of ZnS,” Phys. Rev. Lett. 72(3), 416–419 (1994).
[Crossref] [PubMed]

Gao, M. Y.

Y. H. Yang, L. H. Jing, X. L. Yu, D. D. Yan, and M. Y. Gao, “Coating Aqueous Quantum Dots with Silica via Reverse Microemulsion Method: Toward Size-Controllable and Robust Fluorescent Nanoparticles,” Chem. Mater. 19(17), 4123–4128 (2007).
[Crossref]

Gopal, A. V.

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

Gu, P. F.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

Gu, Z.

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

Guo, Y.

S. R. Alvarado, Y. Guo, T. P. A. Ruberu, E. Tavasoli, and J. Vela, “Inorganic chemistry solutions to semiconductor nanocrystal problems,” Coord. Chem. Rev. 263, 182–196 (2014).
[Crossref]

Guyot-Sionnest, P.

S. Ithurria, P. Guyot-Sionnest, B. Mahler, and B. Dubertret, “Mn2+ as a Radial Pressure Gauge in Colloidal Core/Shell Nanocrystals,” Phys. Rev. Lett. 99(26), 265501 (2007).
[Crossref] [PubMed]

Hazarika, A.

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

Holloway, P. H.

H. Yang, P. H. Holloway, G. Cunningham, and K. S. Schanze, “CdS:Mn nanocrystals passivated by ZnS: Synthesis and luminescent Properties,” J. Chem. Phys. 121(20), 10233–10240 (2004).
[Crossref] [PubMed]

Hong, X.

R. N. Bhargava, D. Gallagher, X. Hong, and A. Nurmikko, “Optical Properties of Manganese-Doped Nanocrystals of ZnS,” Phys. Rev. Lett. 72(3), 416–419 (1994).
[Crossref] [PubMed]

Hu, M. Z.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Huang, Y.

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

Ishizumi, A.

A. Ishizumi and Y. Kanemitsu, “Luminescence Spectra and Dynamics of Mn-Doped CdS Core/Shell Nanocrystals,” Adv. Mater. 18(8), 1083–1085 (2006).
[Crossref]

Ithurria, S.

S. Ithurria, P. Guyot-Sionnest, B. Mahler, and B. Dubertret, “Mn2+ as a Radial Pressure Gauge in Colloidal Core/Shell Nanocrystals,” Phys. Rev. Lett. 99(26), 265501 (2007).
[Crossref] [PubMed]

Jain, R. K.

Y. Chan, J. P. Zimmer, M. Stroh, J. S. Steckel, R. K. Jain, and M. G. Bawendi, “Incorporation of Luminescent Nanocrystals into Monodisperse Core-Shell Silica Microspheres,” Adv. Mater. 16(23–24), 2092–2097 (2004).
[Crossref]

Jana, N. R.

B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
[Crossref]

Jana, S.

B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
[Crossref]

Jhun, C.

Jing, L. H.

Y. H. Yang, L. H. Jing, X. L. Yu, D. D. Yan, and M. Y. Gao, “Coating Aqueous Quantum Dots with Silica via Reverse Microemulsion Method: Toward Size-Controllable and Robust Fluorescent Nanoparticles,” Chem. Mater. 19(17), 4123–4128 (2007).
[Crossref]

Kanemitsu, Y.

A. Ishizumi and Y. Kanemitsu, “Luminescence Spectra and Dynamics of Mn-Doped CdS Core/Shell Nanocrystals,” Adv. Mater. 18(8), 1083–1085 (2006).
[Crossref]

Kang, J. S.

Karan, N. S.

B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
[Crossref]

Ke, X.

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
[Crossref]

Kelly, J. J.

J. F. Suyver, S. F. Wuister, J. J. Kelly, and A. Meijerink, “Luminescence of nanocrystalline ZnSe:Mn2+,” Phys. Chem. Chem. Phys. 2(23), 5445–5448 (2000).
[Crossref]

Kim, J. W.

Kim, N.

Kim, N. H.

Kim, W.

Kim, W. Y.

Kim, Y.

Kingston, D.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Kotov, N. A.

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

Kuijper, J.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Layek, A.

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

Lee, S.

Leek, D. M.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Li, L. S.

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

Li, W.

X. Wang, X. Yan, W. Li, and K. Sun, “Doped quantum dots for white-light-emitting diodes without reabsorption of multiphase phosphors,” Adv. Mater. 24(20), 2742–2747 (2012).
[Crossref] [PubMed]

Li, X.

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

Liang, Z. W.

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

Lin, Y. J.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

Liu, J. H.

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

Lou, S.

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

Luo, S. L.

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

Mahadevan, P.

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

Mahler, B.

S. Ithurria, P. Guyot-Sionnest, B. Mahler, and B. Dubertret, “Mn2+ as a Radial Pressure Gauge in Colloidal Core/Shell Nanocrystals,” Phys. Rev. Lett. 99(26), 265501 (2007).
[Crossref] [PubMed]

Malm, J. O.

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

Meijerink, A.

J. F. Suyver, S. F. Wuister, J. J. Kelly, and A. Meijerink, “Luminescence of nanocrystalline ZnSe:Mn2+,” Phys. Chem. Chem. Phys. 2(23), 5445–5448 (2000).
[Crossref]

Mohan, A.

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

Murase, N.

P. Yang, M. Ando, and N. Murase, “Highly luminescent CdSe/CdxZn1-XS quantum dots coated with thickness-controlled SiO2 shell through silanization,” Langmuir 27(15), 9535–9540 (2011).
[Crossref] [PubMed]

Nag, A.

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

Niu, J. Z.

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

Nurmikko, A.

R. N. Bhargava, D. Gallagher, X. Hong, and A. Nurmikko, “Optical Properties of Manganese-Doped Nanocrystals of ZnS,” Phys. Rev. Lett. 72(3), 416–419 (1994).
[Crossref] [PubMed]

Ouyang, J.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Paria, S.

B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
[Crossref]

Peng, X.

N. Pradhan and X. Peng, “Efficient and color-tunable Mn-doped ZnSe nanocrystal emitters: Control of optical performance via greener synthetic chemistry,” J. Am. Chem. Soc. 129(11), 3339–3347 (2007).
[Crossref] [PubMed]

Pietra, F.

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
[Crossref]

Pradhan, N.

B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
[Crossref]

N. Pradhan and X. Peng, “Efficient and color-tunable Mn-doped ZnSe nanocrystal emitters: Control of optical performance via greener synthetic chemistry,” J. Am. Chem. Soc. 129(11), 3339–3347 (2007).
[Crossref] [PubMed]

Ripmeester, J. A.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Ruberu, T. P. A.

S. R. Alvarado, Y. Guo, T. P. A. Ruberu, E. Tavasoli, and J. Vela, “Inorganic chemistry solutions to semiconductor nanocrystal problems,” Coord. Chem. Rev. 263, 182–196 (2014).
[Crossref]

Sammynaiken, R.

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

Sarma, D. D.

A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
[Crossref] [PubMed]

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
[Crossref]

Schanze, K. S.

H. Yang, P. H. Holloway, G. Cunningham, and K. S. Schanze, “CdS:Mn nanocrystals passivated by ZnS: Synthesis and luminescent Properties,” J. Chem. Phys. 121(20), 10233–10240 (2004).
[Crossref] [PubMed]

Shen, H.

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

Shen, X. C.

B. P. Yang, X. C. Shen, H. C. Zhang, Y. P. Cui, and J. Y. Zhang, “Luminescent and Magnetic Properties in Semiconductor Nanocrystals with Radial-Position-Controlled Mn2+ Doping,” J. Phys. Chem. C 117(30), 15829–15834 (2013).
[Crossref]

Srivastava, B. B.

B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
[Crossref]

Steckel, J. S.

Y. Chan, J. P. Zimmer, M. Stroh, J. S. Steckel, R. K. Jain, and M. G. Bawendi, “Incorporation of Luminescent Nanocrystals into Monodisperse Core-Shell Silica Microspheres,” Adv. Mater. 16(23–24), 2092–2097 (2004).
[Crossref]

Stroh, M.

Y. Chan, J. P. Zimmer, M. Stroh, J. S. Steckel, R. K. Jain, and M. G. Bawendi, “Incorporation of Luminescent Nanocrystals into Monodisperse Core-Shell Silica Microspheres,” Adv. Mater. 16(23–24), 2092–2097 (2004).
[Crossref]

Sun, K.

X. Wang, X. Yan, W. Li, and K. Sun, “Doped quantum dots for white-light-emitting diodes without reabsorption of multiphase phosphors,” Adv. Mater. 24(20), 2742–2747 (2012).
[Crossref] [PubMed]

Suyver, J. F.

J. F. Suyver, S. F. Wuister, J. J. Kelly, and A. Meijerink, “Luminescence of nanocrystalline ZnSe:Mn2+,” Phys. Chem. Chem. Phys. 2(23), 5445–5448 (2000).
[Crossref]

Tavasoli, E.

S. R. Alvarado, Y. Guo, T. P. A. Ruberu, E. Tavasoli, and J. Vela, “Inorganic chemistry solutions to semiconductor nanocrystal problems,” Coord. Chem. Rev. 263, 182–196 (2014).
[Crossref]

van Dijk - Moes, R. J. A.

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
[Crossref]

Van Tendeloo, G.

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
[Crossref]

Vanmaekelbergh, D.

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
[Crossref]

Vela, J.

S. R. Alvarado, Y. Guo, T. P. A. Ruberu, E. Tavasoli, and J. Vela, “Inorganic chemistry solutions to semiconductor nanocrystal problems,” Coord. Chem. Rev. 263, 182–196 (2014).
[Crossref]

Vengurlekar, A. S.

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

Wallenberg, R.

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

Wang, H.

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

Wang, X.

X. Wang, X. Yan, W. Li, and K. Sun, “Doped quantum dots for white-light-emitting diodes without reabsorption of multiphase phosphors,” Adv. Mater. 24(20), 2742–2747 (2012).
[Crossref] [PubMed]

Wang, Y. D.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

Wu, X.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Wuister, S. F.

J. F. Suyver, S. F. Wuister, J. J. Kelly, and A. Meijerink, “Luminescence of nanocrystalline ZnSe:Mn2+,” Phys. Chem. Chem. Phys. 2(23), 5445–5448 (2000).
[Crossref]

Xu, W.

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

Xu, X. B.

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

Yan, D. D.

Y. H. Yang, L. H. Jing, X. L. Yu, D. D. Yan, and M. Y. Gao, “Coating Aqueous Quantum Dots with Silica via Reverse Microemulsion Method: Toward Size-Controllable and Robust Fluorescent Nanoparticles,” Chem. Mater. 19(17), 4123–4128 (2007).
[Crossref]

Yan, X.

X. Wang, X. Yan, W. Li, and K. Sun, “Doped quantum dots for white-light-emitting diodes without reabsorption of multiphase phosphors,” Adv. Mater. 24(20), 2742–2747 (2012).
[Crossref] [PubMed]

Yang, B. P.

B. P. Yang, X. C. Shen, H. C. Zhang, Y. P. Cui, and J. Y. Zhang, “Luminescent and Magnetic Properties in Semiconductor Nanocrystals with Radial-Position-Controlled Mn2+ Doping,” J. Phys. Chem. C 117(30), 15829–15834 (2013).
[Crossref]

Yang, H.

H. Yang, P. H. Holloway, G. Cunningham, and K. S. Schanze, “CdS:Mn nanocrystals passivated by ZnS: Synthesis and luminescent Properties,” J. Chem. Phys. 121(20), 10233–10240 (2004).
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Yang, P.

P. Yang, M. Ando, and N. Murase, “Highly luminescent CdSe/CdxZn1-XS quantum dots coated with thickness-controlled SiO2 shell through silanization,” Langmuir 27(15), 9535–9540 (2011).
[Crossref] [PubMed]

Yang, Y.

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “On Doping CdS/ZnS Core/Shell Nanocrystals with Mn,” J. Am. Chem. Soc. 130(46), 15649–15661 (2008).
[Crossref] [PubMed]

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “Radial-Position-Controlled Doping in CdS/ZnS Core/Shell Nanocrystals,” J. Am. Chem. Soc. 128(38), 12428–12429 (2006).
[Crossref] [PubMed]

Yang, Y. H.

Y. H. Yang, L. H. Jing, X. L. Yu, D. D. Yan, and M. Y. Gao, “Coating Aqueous Quantum Dots with Silica via Reverse Microemulsion Method: Toward Size-Controllable and Robust Fluorescent Nanoparticles,” Chem. Mater. 19(17), 4123–4128 (2007).
[Crossref]

Yoo, S. I.

Yoon, J.

Yoon, J. A.

Yu, K.

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

Yu, W. W.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

Yu, X. L.

Y. H. Yang, L. H. Jing, X. L. Yu, D. D. Yan, and M. Y. Gao, “Coating Aqueous Quantum Dots with Silica via Reverse Microemulsion Method: Toward Size-Controllable and Robust Fluorescent Nanoparticles,” Chem. Mater. 19(17), 4123–4128 (2007).
[Crossref]

Zhang, H. C.

B. P. Yang, X. C. Shen, H. C. Zhang, Y. P. Cui, and J. Y. Zhang, “Luminescent and Magnetic Properties in Semiconductor Nanocrystals with Radial-Position-Controlled Mn2+ Doping,” J. Phys. Chem. C 117(30), 15829–15834 (2013).
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Zhang, J. M.

J. M. Zhang, X. K. Zhang, and J. Y. Zhang, “Dependence of Microstructure and Luminescence on Shell Layers in Colloidal CdSe/CdS Core/Shell Nanocrystals,” J. Phys. Chem. C 114(9), 3904–3908 (2010).
[Crossref]

Zhang, J. Y.

B. P. Yang, X. C. Shen, H. C. Zhang, Y. P. Cui, and J. Y. Zhang, “Luminescent and Magnetic Properties in Semiconductor Nanocrystals with Radial-Position-Controlled Mn2+ Doping,” J. Phys. Chem. C 117(30), 15829–15834 (2013).
[Crossref]

J. M. Zhang, X. K. Zhang, and J. Y. Zhang, “Dependence of Microstructure and Luminescence on Shell Layers in Colloidal CdSe/CdS Core/Shell Nanocrystals,” J. Phys. Chem. C 114(9), 3904–3908 (2010).
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Zhang, K. B. Q. R.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
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Zhang, T. Q.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
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J. M. Zhang, X. K. Zhang, and J. Y. Zhang, “Dependence of Microstructure and Luminescence on Shell Layers in Colloidal CdSe/CdS Core/Shell Nanocrystals,” J. Phys. Chem. C 114(9), 3904–3908 (2010).
[Crossref]

Zhang, Y.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

Zhao, J.

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
[Crossref]

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
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J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
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Zhu, M. Q.

J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
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Zimmer, J. P.

Y. Chan, J. P. Zimmer, M. Stroh, J. S. Steckel, R. K. Jain, and M. G. Bawendi, “Incorporation of Luminescent Nanocrystals into Monodisperse Core-Shell Silica Microspheres,” Adv. Mater. 16(23–24), 2092–2097 (2004).
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W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
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Adv. Mater. (3)

A. Ishizumi and Y. Kanemitsu, “Luminescence Spectra and Dynamics of Mn-Doped CdS Core/Shell Nanocrystals,” Adv. Mater. 18(8), 1083–1085 (2006).
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Y. Chan, J. P. Zimmer, M. Stroh, J. S. Steckel, R. K. Jain, and M. G. Bawendi, “Incorporation of Luminescent Nanocrystals into Monodisperse Core-Shell Silica Microspheres,” Adv. Mater. 16(23–24), 2092–2097 (2004).
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X. Wang, X. Yan, W. Li, and K. Sun, “Doped quantum dots for white-light-emitting diodes without reabsorption of multiphase phosphors,” Adv. Mater. 24(20), 2742–2747 (2012).
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Chem. Mater. (2)

Y. H. Yang, L. H. Jing, X. L. Yu, D. D. Yan, and M. Y. Gao, “Coating Aqueous Quantum Dots with Silica via Reverse Microemulsion Method: Toward Size-Controllable and Robust Fluorescent Nanoparticles,” Chem. Mater. 19(17), 4123–4128 (2007).
[Crossref]

F. Pietra, R. J. A. van Dijk - Moes, X. Ke, S. Bals, G. Van Tendeloo, C. de Mello Donega, and D. Vanmaekelbergh, “Synthesis of highly luminescent silica-coated CdSe/CdS nanorods,” Chem. Mater. 25(17), 3427–3434 (2013).
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Chin. Opt. Lett. (2)

Coord. Chem. Rev. (1)

S. R. Alvarado, Y. Guo, T. P. A. Ruberu, E. Tavasoli, and J. Vela, “Inorganic chemistry solutions to semiconductor nanocrystal problems,” Coord. Chem. Rev. 263, 182–196 (2014).
[Crossref]

Dalton Trans. (1)

J. Z. Niu, H. Shen, C. Zhou, W. Xu, X. Li, H. Wang, S. Lou, Z. Du, and L. S. Li, “Controlled synthesis of high quality type-II/type-I CdS/ZnSe/ZnS core/shell1/shell2 nanocrystals,” Dalton Trans. 39(13), 3308–3314 (2010).
[Crossref] [PubMed]

J. Am. Chem. Soc. (3)

N. Pradhan and X. Peng, “Efficient and color-tunable Mn-doped ZnSe nanocrystal emitters: Control of optical performance via greener synthetic chemistry,” J. Am. Chem. Soc. 129(11), 3339–3347 (2007).
[Crossref] [PubMed]

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “On Doping CdS/ZnS Core/Shell Nanocrystals with Mn,” J. Am. Chem. Soc. 130(46), 15649–15661 (2008).
[Crossref] [PubMed]

Y. Yang, O. Chen, A. Angerhofer, and Y. C. Cao, “Radial-Position-Controlled Doping in CdS/ZnS Core/Shell Nanocrystals,” J. Am. Chem. Soc. 128(38), 12428–12429 (2006).
[Crossref] [PubMed]

J. Appl. Phys. (1)

W. Chen, R. Sammynaiken, Y. Huang, J. O. Malm, R. Wallenberg, J. O. Bovin, V. Zwiller, and N. A. Kotov, “Crystal field, phonon coupling and emission shift of Mn2+ in ZnS:Mn nanoparticles,” J. Appl. Phys. 89(2), 1120–1129 (2001).
[Crossref]

J. Chem. Phys. (1)

H. Yang, P. H. Holloway, G. Cunningham, and K. S. Schanze, “CdS:Mn nanocrystals passivated by ZnS: Synthesis and luminescent Properties,” J. Chem. Phys. 121(20), 10233–10240 (2004).
[Crossref] [PubMed]

J. Phys. Chem. C (4)

B. P. Yang, X. C. Shen, H. C. Zhang, Y. P. Cui, and J. Y. Zhang, “Luminescent and Magnetic Properties in Semiconductor Nanocrystals with Radial-Position-Controlled Mn2+ Doping,” J. Phys. Chem. C 117(30), 15829–15834 (2013).
[Crossref]

A. Nag, R. Cherian, P. Mahadevan, A. V. Gopal, A. Hazarika, A. Mohan, A. S. Vengurlekar, and D. D. Sarma, “Size-Dependent Tuning of Mn2+ d Emission in Mn2+-Doped CdS Nanocrystals: Bulk vs Surface,” J. Phys. Chem. C 114(43), 18323–18329 (2010).
[Crossref]

J. Ouyang, J. Kuijper, S. Brot, D. Kingston, X. Wu, D. M. Leek, M. Z. Hu, J. A. Ripmeester, and K. Yu, “Photoluminescent Colloidal CdS Nanocrystals with High Quality via Noninjection One-Pot Synthesis in 1-Octadecene,” J. Phys. Chem. C 113(18), 7579–7593 (2009).
[Crossref]

J. M. Zhang, X. K. Zhang, and J. Y. Zhang, “Dependence of Microstructure and Luminescence on Shell Layers in Colloidal CdSe/CdS Core/Shell Nanocrystals,” J. Phys. Chem. C 114(9), 3904–3908 (2010).
[Crossref]

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B. B. Srivastava, S. Jana, N. S. Karan, S. Paria, N. R. Jana, D. D. Sarma, and N. Pradhan, “Highly Luminescent Mn-Doped ZnS Nanocrystals: Gram-Scale Synthesis,” J. Phys. Chem. Lett. 1(9), 1454–1458 (2010).
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J. H. Liu, J. B. Fan, Z. Gu, J. Cui, X. B. Xu, Z. W. Liang, S. L. Luo, and M. Q. Zhu, “Green Chemistry for Large-Scale Synthesis of Semiconductor Quantum Dots,” Langmuir 24(10), 5241–5244 (2008).
[Crossref] [PubMed]

P. Yang, M. Ando, and N. Murase, “Highly luminescent CdSe/CdxZn1-XS quantum dots coated with thickness-controlled SiO2 shell through silanization,” Langmuir 27(15), 9535–9540 (2011).
[Crossref] [PubMed]

Particuology (1)

Y. J. Lin, Y. Zhang, J. Zhao, P. F. Gu, K. B. Q. R. Zhang, H. R. Chu, T. Q. Zhang, T. Cui, Y. D. Wang, J. Zhao, and W. W. Yu, “White-light-emitting diodes using GaN-excited CdSe/CdS/ZnS quantum dots,” Particuology 15, 90–93 (2014).
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A. Hazarika, A. Layek, S. De, A. Nag, S. Debnath, P. Mahadevan, A. Chowdhury, and D. D. Sarma, “Ultranarrow and Widely Tunable Mn2+-Induced Photoluminescence from Single Mn-Doped Nanocrystals of ZnS-CdS Alloys,” Phys. Rev. Lett. 110(26), 267401 (2013).
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Figures (7)

Fig. 1
Fig. 1 Concentration and size of the CdS:Mn cores obtained using different molar ratios of (a) SA to Cd and (b) S to Cd, and (c) different amounts of OAm. TEM (High-Resolution TEM) images of CdS:Mn “core” (d) with and (e) without an added mass of OAm.
Fig. 2
Fig. 2 (a) PL spectra of four samples I-IV. Inset: TEM and HRTEM images of sample II. The dependency of the emission wavelength on Mn doping concentration (b) and shell structure (c).
Fig. 3
Fig. 3 XRD patterns for the CdS:Mn core and NCs in samples I–IV. Vertical lines indicate zinc-blende CdS (bottom) and ZnS (top) bulk reflections.
Fig. 4
Fig. 4 Lifetime decay curves of four samples. All lifetime decays are within the millisecond scale.
Fig. 5
Fig. 5 EPR spectra of four Mn-doped samples.
Fig. 6
Fig. 6 TEM images of sample II (a) before and (b) after coating with silica. (c) Absorption (left) and PL spectra (right) of sample II NCs before and after coating with silica. (d) PL intensity trends under strong UV light (365 nm, 10 W/mm2) of sample II before and after coating with silica.
Fig. 7
Fig. 7 Electroluminescence (EL) spectra (left) and corresponding Commission Internationale de l’Éclairage (CIE) color coordinates of the WLED with CdS:Mn/ZnS@SiO2 and YAG:Ce3+ (λNCs = 610 nm) (right). Insets show the WLED before and after the application of a forward current of 350 mA.

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