Mid-infrared (2.75–6.0-μm) second-harmonic generation in LiInS<sub>2</sub>

G. M. H. Knippels; A. F. G. van der Meer; A. M. MacLeod; A. Yelisseyev; L. Isaenko; S. Lobanov; I. Thénot; J.-J. Zondy

doi:10.1364/OL.26.000617

Optics Letters
Vol. 26,
Issue 9,
pp. 617-619
(2001)
•https://doi.org/10.1364/OL.26.000617

Mid-infrared (2.75–6.0-μm) second-harmonic generation in LiInS₂

G. M. H. Knippels, A. F. G. van der Meer, A. M. MacLeod, A. Yelisseyev, L. Isaenko, S. Lobanov, I. Thénot, and J.-J. Zondy

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G. M. H. Knippels, A. F. G. van der Meer, A. M. MacLeod, A. Yelisseyev, L. Isaenko, S. Lobanov, I. Thénot, and J.-J. Zondy, "Mid-infrared (2.75–6.0-μm) second-harmonic generation in LiInS₂," Opt. Lett. 26, 617-619 (2001)

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Abstract

Phase-matched second-harmonic generation is obtained in various ${LiInS}_{2}$ crystals by use of the tunable picosecond output of the free-electron laser for infrared experiments (FELIX) as the pump source in the mid-IR range from 2.75 to $6.0 μ m$ . Deviations from the phase-matching curve calculated from Boyd’s refractive-index data are observed. Furthermore, the optical damage threshold of the crystals has been measured to be $1.1 . J / {cm}^{2} (> 6 GW / {cm}^{2})$ at the $5 ‐ μ m$ wavelength. ${LiInS}_{2}$ holds great promise for parametric interaction in the $1 - 13 ‐ μ m$ range.

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Crystal Type, Color^a	Composition	$N_{Li} +$ $N_{In}$	$N_{Li + In} :$ $N_{S}$	$N_{Li} :$ $N_{In}$
As grown, yellow	${Li}_{0.96} {In}_{1.06} S_{1.98}$	2.02	1.01	0.90
Annealed, rose	${Li}_{0.86} {In}_{1.04} S_{1.98}$	1.90	0.95	0.83

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Optics Letters