Abstract

The nonlinear absorption and ultrafast dynamics process of Au triangular nanoprisms were investigated by using broadband (ranging from 550 to 700 nm) nanosecond Z-scan measurements and femtosecond time-resolved transient absorption spectrum, respectively. We found that Au triangular nanoprisms exhibit saturation absorption (SA) at low excitation intensities. With the increase of incident intensity, a switch from SA to reverse saturation absorption (RSA) occurs. Photo-dynamics process was found to be a double-exponential energy relaxation with a fast and a slow decay component. Interestingly, when probe wavelength is away from the plasma resonance peak, the decay of relaxation also shows the modulation due to the vibration mode of the coherent excitation.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2018 (3)

S. Sareen, V. Mutreja, B. Pal, and S. Singh, “Synthesis of bimetallic Au-Ag alloyed mesocomposites and their catalytic activity for the reduction of nitroaromatics,” Appl. Surf. Sci. 435(30), 552–562 (2018).
[Crossref]

C. Zheng, J. X. Huang, L. Lei, W. Z. Chen, H. Y. Wang, and W. Li, “Nanosecond nonlinear optical and optical limiting properties of hollow gold nanocages,” Appl. Phys. B 124(1), 17 (2018).
[Crossref]

K. Wei, T. Jiang, Z. Xu, J. Zhou, J. You, Y. Tang, H. Li, R. Chen, X. Zheng, S. Wang, K. Yin, Z. Wang, J. Wang, and X. Cheng, “Ultrafast carrier transfer promoted by interlayer coulomb coupling in 2D/3D perovskite heterostructures,” Laser Photonics Rev. 12(10), 1800128 (2018).
[Crossref]

2017 (5)

A. Joplin, S. A. Hosseini Jebeli, E. Sung, N. Diemler, P. J. Straney, M. Yorulmaz, W. S. Chang, J. E. Millstone, and S. Link, “Correlated absorption and scattering spectroscopy of individual platinum-decorated gold nanorods reveals strong excitation enhancement in the nonplasmonic metal,” ACS Nano 11(12), 12346–12357 (2017).
[Crossref] [PubMed]

N. Liaros and J. T. Fourkas, “The characterization of absorptive nonlinearities,” Laser Photonics Rev. 11(5), 1700106 (2017).
[Crossref]

X. Cui, H. Li, M. Yuan, J. Yang, D. Xu, Z. Li, G. Yu, Y. Hou, and Z. Dong, “Facile preparation of fluffy N-doped carbon modified with Ag nanoparticles as a highly active and reusable catalyst for catalytic reduction of nitroarenes,” J. Colloid Interface Sci. 506(15), 524–531 (2017).
[Crossref] [PubMed]

P. Ferrari, S. Upadhyay, M. V. Shestakov, J. Vanbuel, B. D. Roo, Y. H. Kuang, M. D. Vece, V. V. Moshchalkov, J. Locquet, P. Lievens, and E. Janssens, “Wavelength-dependent nonlinear optical properties of Ag nanoparticles dispersed in a glass host,” J. Phys. Chem. C 121(49), 27580–27589 (2017).
[Crossref]

H. W. Dai, L. M. Zhang, Z. W. Wang, X. Wang, J. P. Zhang, H. M. Gong, J. Han, and Y. B. Han, “Linear and nonlinear optical properties of silver-coated gold nanorods,” J. Phys. Chem. C 121(22), 12358–12364 (2017).
[Crossref]

2016 (3)

2015 (5)

X. Zheng, Y. Zhang, R. Chen, X. Cheng, Z. Xu, and T. Jiang, “Z-scan measurement of the nonlinear refractive index of monolayer WS(2),” Opt. Express 23(12), 15616–15623 (2015).
[Crossref] [PubMed]

Z. Huang, X. Lei, Y. Liu, Z. Wang, X. Wang, Z. Wang, Q. Mao, and G. Meng, “Tapered optical fiber probe assembled with plasmonic nanostructures for surface-enhanced Raman scattering application,” ACS Appl. Mater. Interfaces 7(31), 17247–17254 (2015).
[Crossref] [PubMed]

J. Huang, Y. Zhu, C. Liu, Y. Zhao, Z. Liu, M. N. Hedhili, A. Fratalocchi, and Y. Han, “Fabricating a homogeneously alloyed AuAg shell on Au nanorods to achieve strong, stable, and tunable surface plasmon resonances,” Small 11(39), 5214–5221 (2015).
[Crossref] [PubMed]

H. Lunden, A. Liotta, D. Chateau, F. Lerouge, F. Chaput, S. Parola, C. Brannlund, Z. Ghadyani, M. Kildemo, M. Lindgren, and C. Lopes, “Dispersion and self-orientation of gold nanoparticles in sol-gel hybrid silica-optical transmission properties,” J. Mater. Chem. C Mater. Opt. Electron. Devices 3(5), 1026–1034 (2015).
[Crossref]

Y. Hua, K. Chandra, D. H. M. Dam, G. P. Wiederrecht, and T. W. Odom, “Shape-dependent nonlinear optical properties of anisotropic gold nanoparticles,” J. Phys. Chem. Lett. 6(24), 4904–4908 (2015).
[Crossref] [PubMed]

2013 (3)

Z. Zhang, J. Wang, and C. Chen, “Gold nanorods based platforms for light-mediated theranostics,” Theranostics 3(3), 223–238 (2013).
[Crossref] [PubMed]

Z. X. Li, Y. Yu, Z. Y. Chen, T. R. Liu, Z. K. Zhou, J. B. Han, J. T. Li, C. J. Jin, and X. H. Wang, “Ultrafast third-order optical nonlinearity in Au triangular nanoprism with strong dipole and quadrupole plasmon resonance,” J. Phys. Chem. C 117(39), 20127–20132 (2013).
[Crossref]

Z. Chen, H. Dai, J. Liu, H. Xu, Z. Li, Z. K. Zhou, and J. B. Han, “Dipole plasmon resonance induced large third-order optical nonlinearity of Au triangular nanoprism in infrared region,” Opt. Express 21(15), 17568–17575 (2013).
[Crossref] [PubMed]

2011 (3)

N. Liu, M. L. Tang, M. Hentschel, H. Giessen, and A. P. Alivisatos, “Nanoantenna-enhanced gas sensing in a single tailored nanofocus,” Nat. Mater. 10(8), 631–636 (2011).
[Crossref] [PubMed]

G. V. Hartland, “Optical studies of dynamics in noble metal nanostructures,” Chem. Rev. 111(6), 3858–3887 (2011).
[Crossref] [PubMed]

Y. Tsutsui, T. Hayakawa, G. Kawamura, and M. Nogami, “Tuned longitudinal surface plasmon resonance and third-order nonlinear optical properties of gold nanorods,” Nanotechnology 22(27), 275203 (2011).
[Crossref] [PubMed]

2010 (3)

D. Martín-Cano, L. Martín-Moreno, F. J. García-Vidal, and E. Moreno, “Resonance energy transfer and superradiance mediated by plasmonic nanowaveguides,” Nano Lett. 10(8), 3129–3134 (2010).
[Crossref] [PubMed]

J. Nelayah, M. Kociak, O. Stéphan, N. Geuquet, L. Henrard, F. J. García de Abajo, I. Pastoriza-Santos, L. M. Liz-Marzán, and C. Colliex, “Two-dimensional quasistatic stationary short range surface plasmons in flat nanoprisms,” Nano Lett. 10(3), 902–907 (2010).
[Crossref] [PubMed]

J. Li, S. Liu, Y. Liu, F. Zhou, and Z. Y. Li, “Anisotropic and enhanced absorptive nonlinearities in a macroscopic film induced by aligned gold nanorods,” Appl. Phys. Lett. 96(26), 263103 (2010).
[Crossref]

2009 (1)

2008 (5)

J. Merlein, M. Kahl, A. Zuschlag, A. Sell, A. Halm, J. Boneberg, P. Leiderer, A. Leitenstorfer, and R. Bratschitsch, “Nanomechanical control of an optical antenna,” Nat. Photonics 2(4), 230–233 (2008).
[Crossref]

L. Brus, “Noble metal nanocrystals: plasmon electron transfer photochemistry and single-molecule Raman spectroscopy,” Acc. Chem. Res. 41(12), 1742–1749 (2008).
[Crossref] [PubMed]

B. H. Staleva and G. V. Hartland, “Vibrational dynamics of silver nanocubes and nanowires studied by single-particle transient absorption spectroscopy,” Adv. Funct. Mater. 18(23), 3809–3817 (2008).
[Crossref]

H. Staleva and G. V. Hartland, “Transient absorption studies of single silver nanocubes,” J. Phys. Chem. C 112(20), 7535–7539 (2008).
[Crossref]

S. Kim, J. Jin, Y. J. Kim, I. Y. Park, Y. Kim, and S. W. Kim, “High-harmonic generation by resonant plasmon field enhancement,” Nature 453(7196), 757–760 (2008).
[Crossref] [PubMed]

2006 (3)

P. K. Jain, W. Qian, and M. A. El-Sayed, “Ultrafast electron relaxation dynamics in coupled metal nanoparticles in aggregates,” J. Phys. Chem. B 110(1), 136–142 (2006).
[Crossref] [PubMed]

M. Hu, H. Petrova, J. Chen, J. M. McLellan, A. R. Siekkinen, M. Marquez, X. Li, Y. Xia, and G. V. Hartland, “Ultrafast laser studies of the photothermal properties of gold nanocages,” J. Phys. Chem. B 110(4), 1520–1524 (2006).
[Crossref] [PubMed]

H. I. Elim, J. Yang, J. Y. Lee, J. Mi, and W. Ji, “Observation of saturable and reverse-saturable absorption at longitudinal surface plasmon resonance in gold nanorods,” Appl. Phys. Lett. 88(8), 083107 (2006).
[Crossref]

2005 (2)

Y. C. Gao, X. R. Zhang, Y. L. Li, H. F. Liu, Y. X. Wang, Q. Chang, W. Y. Jiao, and Y. L. Song, “Saturable absorption and reverse saturable absorption in platinum nanoparticles,” Opt. Commun. 251(4), 429–433 (2005).
[Crossref]

J. E. Millstone, S. Park, K. L. Shuford, L. Qin, G. C. Schatz, and C. A. Mirkin, “Observation of a quadrupole plasmon mode for a colloidal solution of gold nanoprisms,” J. Am. Chem. Soc. 127(15), 5312–5313 (2005).
[Crossref] [PubMed]

2004 (1)

G. V. Hartland, “Measurements of the material properties of metal nanoparticles by time-resolved spectroscopy,” Phys. Chem. Chem. Phys. 6(23), 5263–5274 (2004).
[Crossref]

2003 (1)

R. West, Y. Wang, and T. Goodson, “Nonlinear absorption properties in novel gold nanostructured topologies,” J. Phys. Chem. B 107(15), 3419–3426 (2003).
[Crossref]

2002 (1)

G. V. Hartland, “Coherent vibrational motion in metal particles: Determination of the vibrational amplitude and excitation mechanism,” J. Chem. Phys. 116(18), 8048–8055 (2002).
[Crossref]

2000 (2)

N. D. Fatti, F. Vallee, C. Flytzanis, Y. Hamanaka, and A. Nakamura, “Electron dynamics and surface plasmon resonance nonlinearities in metal nanoparticles,” Chem. Phys. 251(1), 215–226 (2000).
[Crossref]

J. H. Hodak, A. Henglein, and G. V. J. Hartland, “Photophysics of nanometer sized metal particles: electron− phonon coupling and coherent excitation of breathing vibrational modes,” J. Phys. Chem. B 104(43), 9954–9965 (2000).
[Crossref]

1999 (2)

G. V. Hartland, J. H. Hodak, and I. Martini, “Comment on “Optically induced damping of the surface plasmon resonance in gold colloids”,” Phys. Rev. Lett. 82(15), 3188 (1999).
[Crossref]

S. Link and M. A. El-Sayed, “Spectral properties and relaxation dynamics of surface plasmon electronic oscillations in gold and silver nanodots and nanorods,” J. Phys. Chem. B 103(40), 8410–8426 (1999).
[Crossref]

1998 (1)

J. H. Hodak, I. Martini, and G. V. Hartland, “Spectroscopy and dynamics of nanometer-sized noble metal particles,” J. Phys. Chem. B 102(36), 6958–6967 (1998).
[Crossref]

1996 (1)

T. S. Ahmadi, S. L. Logunov, and M. A. El-Sayed, “Picosecond dynamics of colloidal gold nanoparticles,” J. Phys. Chem. 100(20), 8053–8056 (1996).
[Crossref]

1994 (1)

J. Z. Zhang, R. H. O’Neil, and T. W. Roberti, “Femtosecond studies of photoinduced electron dynamics at the liquid-solid interface of aqueous CdS colloids,” J. Phys. Chem. 98(14), 3859–3864 (1994).
[Crossref]

1990 (1)

M. Sheik-Bahae, A. A. Said, T.-H. Wei, D. J. Hagan, and E. W. Van Stryland, “Sensitive measurement of optical nonlinearities using a single beam,” IEEE J. Quantum Electron. 26(4), 760–769 (1990).
[Crossref]

1983 (1)

G. L. Eesley, “Observation of nonequilibrium electron heating in copper,” Phys. Rev. Lett. 51(23), 2140–2143 (1983).
[Crossref]

Ahmadi, T. S.

T. S. Ahmadi, S. L. Logunov, and M. A. El-Sayed, “Picosecond dynamics of colloidal gold nanoparticles,” J. Phys. Chem. 100(20), 8053–8056 (1996).
[Crossref]

Alivisatos, A. P.

N. Liu, M. L. Tang, M. Hentschel, H. Giessen, and A. P. Alivisatos, “Nanoantenna-enhanced gas sensing in a single tailored nanofocus,” Nat. Mater. 10(8), 631–636 (2011).
[Crossref] [PubMed]

Almaguer-Valenzuela, S.

Austin, J.

Baldovino-Pantaleón, O.

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D. L. Kong, J. L. Xu, R. Z. Zhan, X. Y. Duan, and Z. K. Zhou, “Surface plasmon-enhanced third-order optical non-linearity of silver triangular nanoplate,” J. Mod. Opt. 63(21), 2396–2401 (2016).
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Figures (6)

Fig. 1
Fig. 1 (a) SEM image of Au triangular nanoprisms, (b) linear absorption spectra of Au triangular nanoprisms.
Fig. 2
Fig. 2 Normalized transmission of Au triangular nanoprisms position for open aperture Z-scan at different wavelengths (550 nm, 600 nm, 650 nm and 700 nm). (a) laser energy of 300 μJ (irradiance at focus of 3.6×1013 W/m2), (b) laser energy of 600 μJ (irradiance at focus of 7.2×1013 W/m2). The dots are experimental data while the solid lines are theoretical fit.
Fig. 3
Fig. 3 The dotted lines are theoretical fit Saturation strength I s and nonlinear absorption coefficient β of Au triangular nanoprisms vs. wavelength. (a) 3.6×1013 W/m2 ( I 0 ), (b) 7.2×1013 W/m2 ( I 0 ) and (c) 7.2×1013 W/m2 ( I 0 ). The solid lines are the linear absorption spectra.
Figures 4
Figures 4 (a) and (b) Time and wavelength resolved transient absorption data of Au triangular nanoprisms. (c) Transient absorption spectra for Au triangular nanoprisms at different delay times. (d) Dynamic traces of Au triangular nanoprisms at two wavelengths 530 nm and 700 nm, respectively (The dots are experimental data while the solid lines are theoretical fit generated).
Fig. 5
Fig. 5 (a) and (b). Normalized dynamics curves for Au triangular nanoprisms at different pump fluencies at two resonant peaks, respectively (The dots are experimental data while the solid lines are theoretical fit generated). The insert shows the decay constant versus ( τ 1 ) change plotted as a function of pump laser power.
Fig. 6
Fig. 6 Dynamic traces of Au triangular nanoprisms at 547 nm (The dashed line is experimental data while the solid line is theoretical fit generated). The inset shows a plot of vibrational frequencies, which is obtained by Fourier transforming the modulated portion of the data.

Tables (2)

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Table 1 Nonlinear Optical Parameters of Au triangular nanoprisms

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Table 2 Fitting results for the decay processes for Au triangular nanoprisms at different powers.

Equations (6)

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T(z)= m=0 [ β I 0 L eff (1+ z 2 / z 0 2 ) ] m (m+1) 3/2
α( I )= α 0 1+( I/ I s ) +βI
I= I 0 1+ z 2 / z 0 2
α( I 0 )= α 0 1+ I 0 (1+ z 2 / z 0 2 ) I s + β I 0 1+ z 2 / z 0 2
ΔT T = A 1 exp( t τ 1 )+ A 2 exp( t τ 2 )
S( t )=Acos( 2πt T +φ ) e t τ v + A 1 e t τ 1 + A 2 e t τ 2 +B

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