Abstract

Here, we report the energy transfer in (PEA)2PbI4/MAPbBr3 perovskite heterostructures. Under two-photon excitation, the photoluminescence (PL) emission of the (PEA)2PbI4 flake is nearly completely quenched, while that of the MAPbBr3 microplate is greatly increased (6.5 folds higher) in the heterostructure. The opposite variation character of the PL emissions is attributed to the radiative energy transfer from the (PEA)2PbI4 flake to the MAPbBr3 microplate. The radiative energy transfer occurs on an ultrafast timescale with a high efficiency (~100%). In addition, a strongly thickness- and wavelength-dependent interlayer interaction is observed under one-photon excitation. This work advocates great promise for revealing the interlayer interaction of perovskite heterostructures and developing high-performance optoelectronic devices.

© 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2018 (12)

W. Liu, Y.-N. Zhu, M. Liu, B. Wen, S. Fang, H. Teng, M. Lei, L.-M. Liu, and Z. Wei, “Optical properties and applications for MoS2-Sb2Te3-MoS2 heterostructure materials,” Photon. Res. 6(3), 220–227 (2018).
[Crossref]

Q. Fang, Q. Shang, L. Zhao, R. Wang, Z. Zhang, P. Yang, X. Sui, X. Qiu, X. Liu, Q. Zhang, and Y. Zhang, “Ultrafast charge transfer in perovskite nanowire/2D transition metal dichalcogenide heterostructures,” J. Phys. Chem. Lett. 9(7), 1655–1662 (2018).
[Crossref] [PubMed]

A. Borgia, M. B. Borgia, K. Bugge, V. M. Kissling, P. O. Heidarsson, C. B. Fernandes, A. Sottini, A. Soranno, K. J. Buholzer, D. Nettels, B. B. Kragelund, R. B. Best, and B. Schuler, “Extreme disorder in an ultrahigh-affinity protein complex,” Nature 555(7694), 61–66 (2018).
[Crossref] [PubMed]

W. Huang, P. Cheng, Y. M. Yang, G. Li, and Y. Yang, “High-performance organic bulk-heterojunction solar cells based on multiple-donor or multiple-acceptor components,” Adv. Mater. 30(8), 1705706 (2018).
[Crossref] [PubMed]

H. Li, X. Zheng, Y. Liu, Z. Zhang, and T. Jiang, “Ultrafast interfacial energy transfer and interlayer excitons in the monolayer WS2/CsPbBr3 quantum dot heterostructure,” Nanoscale 10(4), 1650–1659 (2018).
[Crossref] [PubMed]

D. Gui, L. Ji, A. Muhammad, W. Li, W. Cai, Y. Li, X. Li, X. Wu, and P. Lu, “Jahn–Teller effect on framework flexibility of hybrid organic–inorganic perovskites,” J. Phys. Chem. Lett. 9(4), 751–755 (2018).
[Crossref] [PubMed]

X. Yang, X. Zhang, J. Deng, Z. Chu, Q. Jiang, J. Meng, P. Wang, L. Zhang, Z. Yin, and J. You, “Efficient green light-emitting diodes based on quasi-two-dimensional composition and phase engineered perovskite with surface passivation,” Nat. Commun. 9(1), 570 (2018).
[Crossref] [PubMed]

G. Jia, Z.-J. Shi, Y.-D. Xia, Q. Wei, Y.-H. Chen, G.-C. Xing, and W. Huang, “Super air stable quasi-2D organic-inorganic hybrid perovskites for visible light-emitting diodes,” Opt. Express 26(2), A66–A74 (2018).
[Crossref] [PubMed]

C. Ran, J. Xi, W. Gao, F. Yuan, T. Lei, B. Jiao, X. Hou, and Z. Wu, “Bilateral interface engineering toward efficient 2D–3D bulk heterojunction tin halide lead-free perovskite solar cells,” ACS Energy Lett. 3(3), 713–721 (2018).
[Crossref]

S. Luo, X. Ma, H. Xie, M. Li, Y. Zhou, W. Cao, and P. Lu, “Controlling nonsequential double ionization of Ne with parallel-polarized two-color laser pulses,” Opt. Express 26(10), 13666–13676 (2018).
[Crossref] [PubMed]

W. Liu, X. Li, Y. Song, C. Zhang, X. Han, H. Long, B. Wang, K. Wang, and P. Lu, “Cooperative enhancement of two-photon-absorption-induced photoluminescence from a 2D perovskite-microsphere hybrid dielectric structure,” Adv. Funct. Mater. 2018, 1707550 (2018).

H. Tsai, R. Asadpour, J.-C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
[Crossref] [PubMed]

2017 (15)

Y. Fang, H. Wei, Q. Dong, and J. Huang, “Quantification of re-absorption and re-emission processes to determine photon recycling efficiency in perovskite single crystals,” Nat. Commun. 8, 14417 (2017).
[Crossref] [PubMed]

Y. M. Kang, B. W. Li, and Z. Y. Fang, “Radiative energy transfer from MoS2 excitons to surface plasmons,” J. Opt. 19, 124009 (2017).

Y. Liu, H. Li, X. Zheng, X. Cheng, and T. Jiang, “Giant photoluminescence enhancement in monolayer WS2 by energy transfer from CsPbBr3 quantum dots,” Opt. Mater. Express 7(4), 1327 (2017).
[Crossref]

C. D. LaBoda, A. R. Lebeck, and C. L. Dwyer, “An optically modulated self-Assembled resonance energy transfer pass gate,” Nano Lett. 17(6), 3775–3781 (2017).
[Crossref] [PubMed]

W. Li, Z. Wang, F. Deschler, S. Gao, R. H. Friend, and A. K. Cheetham, “Chemically diverse and multifunctional hybrid organic-inorganic perovskites,” Nat. Rev. Mat. 2(3), 16099 (2017).
[Crossref]

D. Ma, Y. Fu, L. Dang, J. Zhai, I. A. Guzei, and S. Jin, “Single-crystal microplates of two-dimensional organic–inorganic lead halide layered perovskites for optoelectronics,” Nano Res. 10(6), 2117–2129 (2017).
[Crossref]

H. Lu, H. Zhang, S. Yuan, J. Wang, Y. Zhan, and L. Zheng, “An optical dynamic study of MAPbBr3 single crystals passivated with MAPbCl3/I3-MAPbBr3 heterojunctions,” Phys. Chem. Chem. Phys. 19(6), 4516–4521 (2017).
[Crossref] [PubMed]

W. Liu, J. Xing, J. Zhao, X. Wen, K. Wang, P. Lu, and Q. Xiong, “Giant two-photon absorption and its saturation in 2D organic-inorganic perovskite,” Adv. Opt. Mater. 5(7), 1601045 (2017).
[Crossref] [PubMed]

F. Ledee, G. Trippe-Allard, H. Diab, P. Audebert, D. Garrot, J.-S. Lauret, and E. Deleporte, “Fast growth of monocrystalline thin films of 2D layered hybrid perovskite,” CrystEngComm 19(19), 2598–2602 (2017).
[Crossref]

C. Wang and E. A. Weiss, “Accelerating FRET between near-infrared emitting quantum dots using a molecular J-aggregate as an exciton bridge,” Nano Lett. 17(9), 5666–5671 (2017).
[Crossref] [PubMed]

W. Xu, W. Liu, J. F. Schmidt, W. Zhao, X. Lu, T. Raab, C. Diederichs, W. Gao, D. V. Seletskiy, and Q. Xiong, “Correlated fluorescence blinking in two-dimensional semiconductor heterostructures,” Nature 541(7635), 62–67 (2017).
[Crossref] [PubMed]

P. K. Nayak, Y. Horbatenko, S. Ahn, G. Kim, J. U. Lee, K. Y. Ma, A. R. Jang, H. Lim, D. Kim, S. Ryu, H. Cheong, N. Park, and H. S. Shin, “Probing evolution of twist-angle-dependent interlayer excitons in MoSe2/WSe2 van der Waals heterostructures,” ACS Nano 11(4), 4041–4050 (2017).
[Crossref] [PubMed]

F. Ceballos, M. G. Ju, S. D. Lane, X. C. Zeng, and H. Zhao, “Highly efficient and anomalous charge transfer in van der Waals trilayer semiconductors,” Nano Lett. 17(3), 1623–1628 (2017).
[Crossref] [PubMed]

A. Raja, A. Chaves, J. Yu, G. Arefe, H. M. Hill, A. F. Rigosi, T. C. Berkelbach, P. Nagler, C. Schüller, T. Korn, C. Nuckolls, J. Hone, L. E. Brus, T. F. Heinz, D. R. Reichman, and A. Chernikov, “Coulomb engineering of the bandgap and excitons in two-dimensional materials,” Nat. Commun. 8, 15251 (2017).
[Crossref] [PubMed]

S. Bettis Homan, V. K. Sangwan, I. Balla, H. Bergeron, E. A. Weiss, and M. C. Hersam, “Ultrafast exciton dissociation and long-lived charge separation in a photovoltaic pentacene-MoS2 van der Waals heterojunction,” Nano Lett. 17(1), 164–169 (2017).
[Crossref] [PubMed]

2016 (6)

A. Boulesbaa, K. Wang, M. Mahjouri-Samani, M. Tian, A. A. Puretzky, I. Ivanov, C. M. Rouleau, K. Xiao, B. G. Sumpter, and D. B. Geohegan, “Ultrafast charge transfer and hybrid exciton formation in 2D/0D heterostructures,” J. Am. Chem. Soc. 138(44), 14713–14719 (2016).
[Crossref] [PubMed]

X. Li, S. Lin, X. Lin, Z. Xu, P. Wang, S. Zhang, H. Zhong, W. Xu, Z. Wu, and W. Fang, “Graphene/h-BN/GaAs sandwich diode as solar cell and photodetector,” Opt. Express 24(1), 134–145 (2016).
[Crossref] [PubMed]

D. Kozawa, A. Carvalho, I. Verzhbitskiy, F. Giustiniano, Y. Miyauchi, S. Mouri, A. H. Castro Neto, K. Matsuda, and G. Eda, “Evidence for fast interlayer energy transfer in MoSe2/WS2 heterostructures,” Nano Lett. 16(7), 4087–4093 (2016).
[Crossref] [PubMed]

D. M. Jang, D. H. Kim, K. Park, J. Park, J. W. Lee, and J. K. Song, “Ultrasound synthesis of lead halide perovskite nanocrystals,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(45), 10625–10629 (2016).
[Crossref]

J. Liu, Y. Xue, Z. Wang, Z. Q. Xu, C. Zheng, B. Weber, J. Song, Y. Wang, Y. Lu, Y. Zhang, and Q. Bao, “Two-dimensional CH3NH3PbI3 perovskite: synthesis and optoelectronic application,” ACS Nano 10(3), 3536–3542 (2016).
[Crossref] [PubMed]

S. Brittman and E. C. Garnett, “Measuring n and k at the microscale in single crystals of CH3NH3PbBr3 perovskite,” J. Phys. Chem. C 120(1), 616–620 (2016).
[Crossref]

2015 (6)

J. T. Li, S. K. Cushing, F. K. Meng, T. R. Senty, A. D. Bristow, and N. Q. Wu, “Plasmon-induced resonance energy transfer for solar energy conversion,” Nat. Photonics 9(9), 601–607 (2015).
[Crossref]

D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
[Crossref] [PubMed]

Q. Liao, K. Hu, H. Zhang, X. Wang, J. Yao, and H. Fu, “Perovskite microdisk microlasers self-assembled from solution,” Adv. Mater. 27(22), 3405–3410 (2015).
[Crossref] [PubMed]

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
[Crossref] [PubMed]

Y. Lee, J. Kwon, E. Hwang, C. H. Ra, W. J. Yoo, J. H. Ahn, J. H. Park, and J. H. Cho, “High-performance perovskite-graphene hybrid photodetector,” Adv. Mater. 27(1), 41–46 (2015).
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Z. Wu, X. Li, H. Zhong, S. Zhang, P. Wang, T. H. Kim, S. S. Kwak, C. Liu, H. Chen, S.-W. Kim, and S. Lin, “Graphene/h-BN/ZnO van der Waals tunneling heterostructure based ultraviolet photodetector,” Opt. Express 23(15), 18864–18871 (2015).
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2014 (1)

F. T. Rabouw, S. A. den Hartog, T. Senden, and A. Meijerink, “Photonic effects on the Förster resonance energy transfer efficiency,” Nat. Commun. 5(1), 3610 (2014).
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2013 (1)

L. Wang, I. Meric, P. Y. Huang, Q. Gao, Y. Gao, H. Tran, T. Taniguchi, K. Watanabe, L. M. Campos, D. A. Muller, J. Guo, P. Kim, J. Hone, K. L. Shepard, and C. R. Dean, “One-dimensional electrical contact to a two-dimensional material,” Science 342(6158), 614–617 (2013).
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2010 (1)

S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
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2009 (1)

A. A. Lutich, G. Jiang, A. S. Susha, A. L. Rogach, F. D. Stefani, and J. Feldmann, “Energy transfer versus charge separation in type-II hybrid organic-inorganic nanocomposites,” Nano Lett. 9(7), 2636–2640 (2009).
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Adinolfi, V.

D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
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Ahn, J. H.

Y. Lee, J. Kwon, E. Hwang, C. H. Ra, W. J. Yoo, J. H. Ahn, J. H. Park, and J. H. Cho, “High-performance perovskite-graphene hybrid photodetector,” Adv. Mater. 27(1), 41–46 (2015).
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Ahn, S.

P. K. Nayak, Y. Horbatenko, S. Ahn, G. Kim, J. U. Lee, K. Y. Ma, A. R. Jang, H. Lim, D. Kim, S. Ryu, H. Cheong, N. Park, and H. S. Shin, “Probing evolution of twist-angle-dependent interlayer excitons in MoSe2/WSe2 van der Waals heterostructures,” ACS Nano 11(4), 4041–4050 (2017).
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Ajayan, P. M.

H. Tsai, R. Asadpour, J.-C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Al Choueiry, A.

S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
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H. Tsai, R. Asadpour, J.-C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Alarousu, E.

D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
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Arefe, G.

A. Raja, A. Chaves, J. Yu, G. Arefe, H. M. Hill, A. F. Rigosi, T. C. Berkelbach, P. Nagler, C. Schüller, T. Korn, C. Nuckolls, J. Hone, L. E. Brus, T. F. Heinz, D. R. Reichman, and A. Chernikov, “Coulomb engineering of the bandgap and excitons in two-dimensional materials,” Nat. Commun. 8, 15251 (2017).
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H. Tsai, R. Asadpour, J.-C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Audebert, P.

F. Ledee, G. Trippe-Allard, H. Diab, P. Audebert, D. Garrot, J.-S. Lauret, and E. Deleporte, “Fast growth of monocrystalline thin films of 2D layered hybrid perovskite,” CrystEngComm 19(19), 2598–2602 (2017).
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S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
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D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
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A. Raja, A. Chaves, J. Yu, G. Arefe, H. M. Hill, A. F. Rigosi, T. C. Berkelbach, P. Nagler, C. Schüller, T. Korn, C. Nuckolls, J. Hone, L. E. Brus, T. F. Heinz, D. R. Reichman, and A. Chernikov, “Coulomb engineering of the bandgap and excitons in two-dimensional materials,” Nat. Commun. 8, 15251 (2017).
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A. Borgia, M. B. Borgia, K. Bugge, V. M. Kissling, P. O. Heidarsson, C. B. Fernandes, A. Sottini, A. Soranno, K. J. Buholzer, D. Nettels, B. B. Kragelund, R. B. Best, and B. Schuler, “Extreme disorder in an ultrahigh-affinity protein complex,” Nature 555(7694), 61–66 (2018).
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S. Bettis Homan, V. K. Sangwan, I. Balla, H. Bergeron, E. A. Weiss, and M. C. Hersam, “Ultrafast exciton dissociation and long-lived charge separation in a photovoltaic pentacene-MoS2 van der Waals heterojunction,” Nano Lett. 17(1), 164–169 (2017).
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H. Tsai, R. Asadpour, J.-C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Boissiere, C.

S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
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A. Borgia, M. B. Borgia, K. Bugge, V. M. Kissling, P. O. Heidarsson, C. B. Fernandes, A. Sottini, A. Soranno, K. J. Buholzer, D. Nettels, B. B. Kragelund, R. B. Best, and B. Schuler, “Extreme disorder in an ultrahigh-affinity protein complex,” Nature 555(7694), 61–66 (2018).
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A. Borgia, M. B. Borgia, K. Bugge, V. M. Kissling, P. O. Heidarsson, C. B. Fernandes, A. Sottini, A. Soranno, K. J. Buholzer, D. Nettels, B. B. Kragelund, R. B. Best, and B. Schuler, “Extreme disorder in an ultrahigh-affinity protein complex,” Nature 555(7694), 61–66 (2018).
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A. Boulesbaa, K. Wang, M. Mahjouri-Samani, M. Tian, A. A. Puretzky, I. Ivanov, C. M. Rouleau, K. Xiao, B. G. Sumpter, and D. B. Geohegan, “Ultrafast charge transfer and hybrid exciton formation in 2D/0D heterostructures,” J. Am. Chem. Soc. 138(44), 14713–14719 (2016).
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S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
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J. T. Li, S. K. Cushing, F. K. Meng, T. R. Senty, A. D. Bristow, and N. Q. Wu, “Plasmon-induced resonance energy transfer for solar energy conversion,” Nat. Photonics 9(9), 601–607 (2015).
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S. Brittman and E. C. Garnett, “Measuring n and k at the microscale in single crystals of CH3NH3PbBr3 perovskite,” J. Phys. Chem. C 120(1), 616–620 (2016).
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A. Raja, A. Chaves, J. Yu, G. Arefe, H. M. Hill, A. F. Rigosi, T. C. Berkelbach, P. Nagler, C. Schüller, T. Korn, C. Nuckolls, J. Hone, L. E. Brus, T. F. Heinz, D. R. Reichman, and A. Chernikov, “Coulomb engineering of the bandgap and excitons in two-dimensional materials,” Nat. Commun. 8, 15251 (2017).
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Bugge, K.

A. Borgia, M. B. Borgia, K. Bugge, V. M. Kissling, P. O. Heidarsson, C. B. Fernandes, A. Sottini, A. Soranno, K. J. Buholzer, D. Nettels, B. B. Kragelund, R. B. Best, and B. Schuler, “Extreme disorder in an ultrahigh-affinity protein complex,” Nature 555(7694), 61–66 (2018).
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Buholzer, K. J.

A. Borgia, M. B. Borgia, K. Bugge, V. M. Kissling, P. O. Heidarsson, C. B. Fernandes, A. Sottini, A. Soranno, K. J. Buholzer, D. Nettels, B. B. Kragelund, R. B. Best, and B. Schuler, “Extreme disorder in an ultrahigh-affinity protein complex,” Nature 555(7694), 61–66 (2018).
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Buin, A.

D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
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Cai, W.

D. Gui, L. Ji, A. Muhammad, W. Li, W. Cai, Y. Li, X. Li, X. Wu, and P. Lu, “Jahn–Teller effect on framework flexibility of hybrid organic–inorganic perovskites,” J. Phys. Chem. Lett. 9(4), 751–755 (2018).
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Campos, L. M.

L. Wang, I. Meric, P. Y. Huang, Q. Gao, Y. Gao, H. Tran, T. Taniguchi, K. Watanabe, L. M. Campos, D. A. Muller, J. Guo, P. Kim, J. Hone, K. L. Shepard, and C. R. Dean, “One-dimensional electrical contact to a two-dimensional material,” Science 342(6158), 614–617 (2013).
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Cao, W.

Carvalho, A.

D. Kozawa, A. Carvalho, I. Verzhbitskiy, F. Giustiniano, Y. Miyauchi, S. Mouri, A. H. Castro Neto, K. Matsuda, and G. Eda, “Evidence for fast interlayer energy transfer in MoSe2/WS2 heterostructures,” Nano Lett. 16(7), 4087–4093 (2016).
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Castro Neto, A. H.

D. Kozawa, A. Carvalho, I. Verzhbitskiy, F. Giustiniano, Y. Miyauchi, S. Mouri, A. H. Castro Neto, K. Matsuda, and G. Eda, “Evidence for fast interlayer energy transfer in MoSe2/WS2 heterostructures,” Nano Lett. 16(7), 4087–4093 (2016).
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F. Ceballos, M. G. Ju, S. D. Lane, X. C. Zeng, and H. Zhao, “Highly efficient and anomalous charge transfer in van der Waals trilayer semiconductors,” Nano Lett. 17(3), 1623–1628 (2017).
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A. Raja, A. Chaves, J. Yu, G. Arefe, H. M. Hill, A. F. Rigosi, T. C. Berkelbach, P. Nagler, C. Schüller, T. Korn, C. Nuckolls, J. Hone, L. E. Brus, T. F. Heinz, D. R. Reichman, and A. Chernikov, “Coulomb engineering of the bandgap and excitons in two-dimensional materials,” Nat. Commun. 8, 15251 (2017).
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W. Li, Z. Wang, F. Deschler, S. Gao, R. H. Friend, and A. K. Cheetham, “Chemically diverse and multifunctional hybrid organic-inorganic perovskites,” Nat. Rev. Mat. 2(3), 16099 (2017).
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H. Tsai, R. Asadpour, J.-C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
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Cheng, P.

W. Huang, P. Cheng, Y. M. Yang, G. Li, and Y. Yang, “High-performance organic bulk-heterojunction solar cells based on multiple-donor or multiple-acceptor components,” Adv. Mater. 30(8), 1705706 (2018).
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P. K. Nayak, Y. Horbatenko, S. Ahn, G. Kim, J. U. Lee, K. Y. Ma, A. R. Jang, H. Lim, D. Kim, S. Ryu, H. Cheong, N. Park, and H. S. Shin, “Probing evolution of twist-angle-dependent interlayer excitons in MoSe2/WSe2 van der Waals heterostructures,” ACS Nano 11(4), 4041–4050 (2017).
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A. Raja, A. Chaves, J. Yu, G. Arefe, H. M. Hill, A. F. Rigosi, T. C. Berkelbach, P. Nagler, C. Schüller, T. Korn, C. Nuckolls, J. Hone, L. E. Brus, T. F. Heinz, D. R. Reichman, and A. Chernikov, “Coulomb engineering of the bandgap and excitons in two-dimensional materials,” Nat. Commun. 8, 15251 (2017).
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Y. Lee, J. Kwon, E. Hwang, C. H. Ra, W. J. Yoo, J. H. Ahn, J. H. Park, and J. H. Cho, “High-performance perovskite-graphene hybrid photodetector,” Adv. Mater. 27(1), 41–46 (2015).
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X. Yang, X. Zhang, J. Deng, Z. Chu, Q. Jiang, J. Meng, P. Wang, L. Zhang, Z. Yin, and J. You, “Efficient green light-emitting diodes based on quasi-two-dimensional composition and phase engineered perovskite with surface passivation,” Nat. Commun. 9(1), 570 (2018).
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S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
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D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
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J. T. Li, S. K. Cushing, F. K. Meng, T. R. Senty, A. D. Bristow, and N. Q. Wu, “Plasmon-induced resonance energy transfer for solar energy conversion,” Nat. Photonics 9(9), 601–607 (2015).
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D. Ma, Y. Fu, L. Dang, J. Zhai, I. A. Guzei, and S. Jin, “Single-crystal microplates of two-dimensional organic–inorganic lead halide layered perovskites for optoelectronics,” Nano Res. 10(6), 2117–2129 (2017).
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F. Ledee, G. Trippe-Allard, H. Diab, P. Audebert, D. Garrot, J.-S. Lauret, and E. Deleporte, “Fast growth of monocrystalline thin films of 2D layered hybrid perovskite,” CrystEngComm 19(19), 2598–2602 (2017).
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F. T. Rabouw, S. A. den Hartog, T. Senden, and A. Meijerink, “Photonic effects on the Förster resonance energy transfer efficiency,” Nat. Commun. 5(1), 3610 (2014).
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Deng, J.

X. Yang, X. Zhang, J. Deng, Z. Chu, Q. Jiang, J. Meng, P. Wang, L. Zhang, Z. Yin, and J. You, “Efficient green light-emitting diodes based on quasi-two-dimensional composition and phase engineered perovskite with surface passivation,” Nat. Commun. 9(1), 570 (2018).
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W. Li, Z. Wang, F. Deschler, S. Gao, R. H. Friend, and A. K. Cheetham, “Chemically diverse and multifunctional hybrid organic-inorganic perovskites,” Nat. Rev. Mat. 2(3), 16099 (2017).
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F. Ledee, G. Trippe-Allard, H. Diab, P. Audebert, D. Garrot, J.-S. Lauret, and E. Deleporte, “Fast growth of monocrystalline thin films of 2D layered hybrid perovskite,” CrystEngComm 19(19), 2598–2602 (2017).
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H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
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Y. Fang, H. Wei, Q. Dong, and J. Huang, “Quantification of re-absorption and re-emission processes to determine photon recycling efficiency in perovskite single crystals,” Nat. Commun. 8, 14417 (2017).
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H. Tsai, R. Asadpour, J.-C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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C. Ran, J. Xi, W. Gao, F. Yuan, T. Lei, B. Jiao, X. Hou, and Z. Wu, “Bilateral interface engineering toward efficient 2D–3D bulk heterojunction tin halide lead-free perovskite solar cells,” ACS Energy Lett. 3(3), 713–721 (2018).
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H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
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H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
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D. Ma, Y. Fu, L. Dang, J. Zhai, I. A. Guzei, and S. Jin, “Single-crystal microplates of two-dimensional organic–inorganic lead halide layered perovskites for optoelectronics,” Nano Res. 10(6), 2117–2129 (2017).
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C. Ran, J. Xi, W. Gao, F. Yuan, T. Lei, B. Jiao, X. Hou, and Z. Wu, “Bilateral interface engineering toward efficient 2D–3D bulk heterojunction tin halide lead-free perovskite solar cells,” ACS Energy Lett. 3(3), 713–721 (2018).
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Q. Liao, K. Hu, H. Zhang, X. Wang, J. Yao, and H. Fu, “Perovskite microdisk microlasers self-assembled from solution,” Adv. Mater. 27(22), 3405–3410 (2015).
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Y. Fang, H. Wei, Q. Dong, and J. Huang, “Quantification of re-absorption and re-emission processes to determine photon recycling efficiency in perovskite single crystals,” Nat. Commun. 8, 14417 (2017).
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P. K. Nayak, Y. Horbatenko, S. Ahn, G. Kim, J. U. Lee, K. Y. Ma, A. R. Jang, H. Lim, D. Kim, S. Ryu, H. Cheong, N. Park, and H. S. Shin, “Probing evolution of twist-angle-dependent interlayer excitons in MoSe2/WSe2 van der Waals heterostructures,” ACS Nano 11(4), 4041–4050 (2017).
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D. M. Jang, D. H. Kim, K. Park, J. Park, J. W. Lee, and J. K. Song, “Ultrasound synthesis of lead halide perovskite nanocrystals,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(45), 10625–10629 (2016).
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D. Gui, L. Ji, A. Muhammad, W. Li, W. Cai, Y. Li, X. Li, X. Wu, and P. Lu, “Jahn–Teller effect on framework flexibility of hybrid organic–inorganic perovskites,” J. Phys. Chem. Lett. 9(4), 751–755 (2018).
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Jiang, G.

A. A. Lutich, G. Jiang, A. S. Susha, A. L. Rogach, F. D. Stefani, and J. Feldmann, “Energy transfer versus charge separation in type-II hybrid organic-inorganic nanocomposites,” Nano Lett. 9(7), 2636–2640 (2009).
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X. Yang, X. Zhang, J. Deng, Z. Chu, Q. Jiang, J. Meng, P. Wang, L. Zhang, Z. Yin, and J. You, “Efficient green light-emitting diodes based on quasi-two-dimensional composition and phase engineered perovskite with surface passivation,” Nat. Commun. 9(1), 570 (2018).
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C. Ran, J. Xi, W. Gao, F. Yuan, T. Lei, B. Jiao, X. Hou, and Z. Wu, “Bilateral interface engineering toward efficient 2D–3D bulk heterojunction tin halide lead-free perovskite solar cells,” ACS Energy Lett. 3(3), 713–721 (2018).
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D. Ma, Y. Fu, L. Dang, J. Zhai, I. A. Guzei, and S. Jin, “Single-crystal microplates of two-dimensional organic–inorganic lead halide layered perovskites for optoelectronics,” Nano Res. 10(6), 2117–2129 (2017).
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H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
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F. Ceballos, M. G. Ju, S. D. Lane, X. C. Zeng, and H. Zhao, “Highly efficient and anomalous charge transfer in van der Waals trilayer semiconductors,” Nano Lett. 17(3), 1623–1628 (2017).
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H. Tsai, R. Asadpour, J.-C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Y. M. Kang, B. W. Li, and Z. Y. Fang, “Radiative energy transfer from MoS2 excitons to surface plasmons,” J. Opt. 19, 124009 (2017).

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D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
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P. K. Nayak, Y. Horbatenko, S. Ahn, G. Kim, J. U. Lee, K. Y. Ma, A. R. Jang, H. Lim, D. Kim, S. Ryu, H. Cheong, N. Park, and H. S. Shin, “Probing evolution of twist-angle-dependent interlayer excitons in MoSe2/WSe2 van der Waals heterostructures,” ACS Nano 11(4), 4041–4050 (2017).
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D. M. Jang, D. H. Kim, K. Park, J. Park, J. W. Lee, and J. K. Song, “Ultrasound synthesis of lead halide perovskite nanocrystals,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(45), 10625–10629 (2016).
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P. K. Nayak, Y. Horbatenko, S. Ahn, G. Kim, J. U. Lee, K. Y. Ma, A. R. Jang, H. Lim, D. Kim, S. Ryu, H. Cheong, N. Park, and H. S. Shin, “Probing evolution of twist-angle-dependent interlayer excitons in MoSe2/WSe2 van der Waals heterostructures,” ACS Nano 11(4), 4041–4050 (2017).
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L. Wang, I. Meric, P. Y. Huang, Q. Gao, Y. Gao, H. Tran, T. Taniguchi, K. Watanabe, L. M. Campos, D. A. Muller, J. Guo, P. Kim, J. Hone, K. L. Shepard, and C. R. Dean, “One-dimensional electrical contact to a two-dimensional material,” Science 342(6158), 614–617 (2013).
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Kim, S.-W.

Kim, T. H.

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A. Borgia, M. B. Borgia, K. Bugge, V. M. Kissling, P. O. Heidarsson, C. B. Fernandes, A. Sottini, A. Soranno, K. J. Buholzer, D. Nettels, B. B. Kragelund, R. B. Best, and B. Schuler, “Extreme disorder in an ultrahigh-affinity protein complex,” Nature 555(7694), 61–66 (2018).
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A. Raja, A. Chaves, J. Yu, G. Arefe, H. M. Hill, A. F. Rigosi, T. C. Berkelbach, P. Nagler, C. Schüller, T. Korn, C. Nuckolls, J. Hone, L. E. Brus, T. F. Heinz, D. R. Reichman, and A. Chernikov, “Coulomb engineering of the bandgap and excitons in two-dimensional materials,” Nat. Commun. 8, 15251 (2017).
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Kozawa, D.

D. Kozawa, A. Carvalho, I. Verzhbitskiy, F. Giustiniano, Y. Miyauchi, S. Mouri, A. H. Castro Neto, K. Matsuda, and G. Eda, “Evidence for fast interlayer energy transfer in MoSe2/WS2 heterostructures,” Nano Lett. 16(7), 4087–4093 (2016).
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A. Borgia, M. B. Borgia, K. Bugge, V. M. Kissling, P. O. Heidarsson, C. B. Fernandes, A. Sottini, A. Soranno, K. J. Buholzer, D. Nettels, B. B. Kragelund, R. B. Best, and B. Schuler, “Extreme disorder in an ultrahigh-affinity protein complex,” Nature 555(7694), 61–66 (2018).
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Kwon, J.

Y. Lee, J. Kwon, E. Hwang, C. H. Ra, W. J. Yoo, J. H. Ahn, J. H. Park, and J. H. Cho, “High-performance perovskite-graphene hybrid photodetector,” Adv. Mater. 27(1), 41–46 (2015).
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F. Ceballos, M. G. Ju, S. D. Lane, X. C. Zeng, and H. Zhao, “Highly efficient and anomalous charge transfer in van der Waals trilayer semiconductors,” Nano Lett. 17(3), 1623–1628 (2017).
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S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
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F. Ledee, G. Trippe-Allard, H. Diab, P. Audebert, D. Garrot, J.-S. Lauret, and E. Deleporte, “Fast growth of monocrystalline thin films of 2D layered hybrid perovskite,” CrystEngComm 19(19), 2598–2602 (2017).
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C. D. LaBoda, A. R. Lebeck, and C. L. Dwyer, “An optically modulated self-Assembled resonance energy transfer pass gate,” Nano Lett. 17(6), 3775–3781 (2017).
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P. K. Nayak, Y. Horbatenko, S. Ahn, G. Kim, J. U. Lee, K. Y. Ma, A. R. Jang, H. Lim, D. Kim, S. Ryu, H. Cheong, N. Park, and H. S. Shin, “Probing evolution of twist-angle-dependent interlayer excitons in MoSe2/WSe2 van der Waals heterostructures,” ACS Nano 11(4), 4041–4050 (2017).
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Lee, J. W.

D. M. Jang, D. H. Kim, K. Park, J. Park, J. W. Lee, and J. K. Song, “Ultrasound synthesis of lead halide perovskite nanocrystals,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(45), 10625–10629 (2016).
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H. Lu, H. Zhang, S. Yuan, J. Wang, Y. Zhan, and L. Zheng, “An optical dynamic study of MAPbBr3 single crystals passivated with MAPbCl3/I3-MAPbBr3 heterojunctions,” Phys. Chem. Chem. Phys. 19(6), 4516–4521 (2017).
[Crossref] [PubMed]

Q. Liao, K. Hu, H. Zhang, X. Wang, J. Yao, and H. Fu, “Perovskite microdisk microlasers self-assembled from solution,” Adv. Mater. 27(22), 3405–3410 (2015).
[Crossref] [PubMed]

Zhang, L.

X. Yang, X. Zhang, J. Deng, Z. Chu, Q. Jiang, J. Meng, P. Wang, L. Zhang, Z. Yin, and J. You, “Efficient green light-emitting diodes based on quasi-two-dimensional composition and phase engineered perovskite with surface passivation,” Nat. Commun. 9(1), 570 (2018).
[Crossref] [PubMed]

Zhang, Q.

Q. Fang, Q. Shang, L. Zhao, R. Wang, Z. Zhang, P. Yang, X. Sui, X. Qiu, X. Liu, Q. Zhang, and Y. Zhang, “Ultrafast charge transfer in perovskite nanowire/2D transition metal dichalcogenide heterostructures,” J. Phys. Chem. Lett. 9(7), 1655–1662 (2018).
[Crossref] [PubMed]

Zhang, S.

Zhang, S. J.

S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
[Crossref]

Zhang, X.

X. Yang, X. Zhang, J. Deng, Z. Chu, Q. Jiang, J. Meng, P. Wang, L. Zhang, Z. Yin, and J. You, “Efficient green light-emitting diodes based on quasi-two-dimensional composition and phase engineered perovskite with surface passivation,” Nat. Commun. 9(1), 570 (2018).
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D. Shi, V. Adinolfi, R. Comin, M. Yuan, E. Alarousu, A. Buin, Y. Chen, S. Hoogland, A. Rothenberger, K. Katsiev, Y. Losovyj, X. Zhang, P. A. Dowben, O. F. Mohammed, E. H. Sargent, and O. M. Bakr, “Solar cells. Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals,” Science 347(6221), 519–522 (2015).
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Zhang, Y.

Q. Fang, Q. Shang, L. Zhao, R. Wang, Z. Zhang, P. Yang, X. Sui, X. Qiu, X. Liu, Q. Zhang, and Y. Zhang, “Ultrafast charge transfer in perovskite nanowire/2D transition metal dichalcogenide heterostructures,” J. Phys. Chem. Lett. 9(7), 1655–1662 (2018).
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J. Liu, Y. Xue, Z. Wang, Z. Q. Xu, C. Zheng, B. Weber, J. Song, Y. Wang, Y. Lu, Y. Zhang, and Q. Bao, “Two-dimensional CH3NH3PbI3 perovskite: synthesis and optoelectronic application,” ACS Nano 10(3), 3536–3542 (2016).
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Zhang, Z.

Q. Fang, Q. Shang, L. Zhao, R. Wang, Z. Zhang, P. Yang, X. Sui, X. Qiu, X. Liu, Q. Zhang, and Y. Zhang, “Ultrafast charge transfer in perovskite nanowire/2D transition metal dichalcogenide heterostructures,” J. Phys. Chem. Lett. 9(7), 1655–1662 (2018).
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H. Li, X. Zheng, Y. Liu, Z. Zhang, and T. Jiang, “Ultrafast interfacial energy transfer and interlayer excitons in the monolayer WS2/CsPbBr3 quantum dot heterostructure,” Nanoscale 10(4), 1650–1659 (2018).
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Zhao, H.

F. Ceballos, M. G. Ju, S. D. Lane, X. C. Zeng, and H. Zhao, “Highly efficient and anomalous charge transfer in van der Waals trilayer semiconductors,” Nano Lett. 17(3), 1623–1628 (2017).
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Zhao, J.

W. Liu, J. Xing, J. Zhao, X. Wen, K. Wang, P. Lu, and Q. Xiong, “Giant two-photon absorption and its saturation in 2D organic-inorganic perovskite,” Adv. Opt. Mater. 5(7), 1601045 (2017).
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Zhao, L.

Q. Fang, Q. Shang, L. Zhao, R. Wang, Z. Zhang, P. Yang, X. Sui, X. Qiu, X. Liu, Q. Zhang, and Y. Zhang, “Ultrafast charge transfer in perovskite nanowire/2D transition metal dichalcogenide heterostructures,” J. Phys. Chem. Lett. 9(7), 1655–1662 (2018).
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Zhao, W.

W. Xu, W. Liu, J. F. Schmidt, W. Zhao, X. Lu, T. Raab, C. Diederichs, W. Gao, D. V. Seletskiy, and Q. Xiong, “Correlated fluorescence blinking in two-dimensional semiconductor heterostructures,” Nature 541(7635), 62–67 (2017).
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Zheng, C.

J. Liu, Y. Xue, Z. Wang, Z. Q. Xu, C. Zheng, B. Weber, J. Song, Y. Wang, Y. Lu, Y. Zhang, and Q. Bao, “Two-dimensional CH3NH3PbI3 perovskite: synthesis and optoelectronic application,” ACS Nano 10(3), 3536–3542 (2016).
[Crossref] [PubMed]

Zheng, L.

H. Lu, H. Zhang, S. Yuan, J. Wang, Y. Zhan, and L. Zheng, “An optical dynamic study of MAPbBr3 single crystals passivated with MAPbCl3/I3-MAPbBr3 heterojunctions,” Phys. Chem. Chem. Phys. 19(6), 4516–4521 (2017).
[Crossref] [PubMed]

Zheng, X.

H. Li, X. Zheng, Y. Liu, Z. Zhang, and T. Jiang, “Ultrafast interfacial energy transfer and interlayer excitons in the monolayer WS2/CsPbBr3 quantum dot heterostructure,” Nanoscale 10(4), 1650–1659 (2018).
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Y. Liu, H. Li, X. Zheng, X. Cheng, and T. Jiang, “Giant photoluminescence enhancement in monolayer WS2 by energy transfer from CsPbBr3 quantum dots,” Opt. Mater. Express 7(4), 1327 (2017).
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Zhou, Y.

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H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
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Zhu, X. Y.

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
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Zhu, Y.-N.

ACS Energy Lett. (1)

C. Ran, J. Xi, W. Gao, F. Yuan, T. Lei, B. Jiao, X. Hou, and Z. Wu, “Bilateral interface engineering toward efficient 2D–3D bulk heterojunction tin halide lead-free perovskite solar cells,” ACS Energy Lett. 3(3), 713–721 (2018).
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ACS Nano (2)

J. Liu, Y. Xue, Z. Wang, Z. Q. Xu, C. Zheng, B. Weber, J. Song, Y. Wang, Y. Lu, Y. Zhang, and Q. Bao, “Two-dimensional CH3NH3PbI3 perovskite: synthesis and optoelectronic application,” ACS Nano 10(3), 3536–3542 (2016).
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P. K. Nayak, Y. Horbatenko, S. Ahn, G. Kim, J. U. Lee, K. Y. Ma, A. R. Jang, H. Lim, D. Kim, S. Ryu, H. Cheong, N. Park, and H. S. Shin, “Probing evolution of twist-angle-dependent interlayer excitons in MoSe2/WSe2 van der Waals heterostructures,” ACS Nano 11(4), 4041–4050 (2017).
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Adv. Funct. Mater. (1)

W. Liu, X. Li, Y. Song, C. Zhang, X. Han, H. Long, B. Wang, K. Wang, and P. Lu, “Cooperative enhancement of two-photon-absorption-induced photoluminescence from a 2D perovskite-microsphere hybrid dielectric structure,” Adv. Funct. Mater. 2018, 1707550 (2018).

Adv. Mater. (3)

W. Huang, P. Cheng, Y. M. Yang, G. Li, and Y. Yang, “High-performance organic bulk-heterojunction solar cells based on multiple-donor or multiple-acceptor components,” Adv. Mater. 30(8), 1705706 (2018).
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Q. Liao, K. Hu, H. Zhang, X. Wang, J. Yao, and H. Fu, “Perovskite microdisk microlasers self-assembled from solution,” Adv. Mater. 27(22), 3405–3410 (2015).
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Adv. Opt. Mater. (1)

W. Liu, J. Xing, J. Zhao, X. Wen, K. Wang, P. Lu, and Q. Xiong, “Giant two-photon absorption and its saturation in 2D organic-inorganic perovskite,” Adv. Opt. Mater. 5(7), 1601045 (2017).
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CrystEngComm (1)

F. Ledee, G. Trippe-Allard, H. Diab, P. Audebert, D. Garrot, J.-S. Lauret, and E. Deleporte, “Fast growth of monocrystalline thin films of 2D layered hybrid perovskite,” CrystEngComm 19(19), 2598–2602 (2017).
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J. Am. Chem. Soc. (1)

A. Boulesbaa, K. Wang, M. Mahjouri-Samani, M. Tian, A. A. Puretzky, I. Ivanov, C. M. Rouleau, K. Xiao, B. G. Sumpter, and D. B. Geohegan, “Ultrafast charge transfer and hybrid exciton formation in 2D/0D heterostructures,” J. Am. Chem. Soc. 138(44), 14713–14719 (2016).
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D. M. Jang, D. H. Kim, K. Park, J. Park, J. W. Lee, and J. K. Song, “Ultrasound synthesis of lead halide perovskite nanocrystals,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(45), 10625–10629 (2016).
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Y. M. Kang, B. W. Li, and Z. Y. Fang, “Radiative energy transfer from MoS2 excitons to surface plasmons,” J. Opt. 19, 124009 (2017).

J. Phys. Chem. C (1)

S. Brittman and E. C. Garnett, “Measuring n and k at the microscale in single crystals of CH3NH3PbBr3 perovskite,” J. Phys. Chem. C 120(1), 616–620 (2016).
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D. Gui, L. Ji, A. Muhammad, W. Li, W. Cai, Y. Li, X. Li, X. Wu, and P. Lu, “Jahn–Teller effect on framework flexibility of hybrid organic–inorganic perovskites,” J. Phys. Chem. Lett. 9(4), 751–755 (2018).
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Q. Fang, Q. Shang, L. Zhao, R. Wang, Z. Zhang, P. Yang, X. Sui, X. Qiu, X. Liu, Q. Zhang, and Y. Zhang, “Ultrafast charge transfer in perovskite nanowire/2D transition metal dichalcogenide heterostructures,” J. Phys. Chem. Lett. 9(7), 1655–1662 (2018).
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Materials (Basel) (1)

S. J. Zhang, P. Audebert, Y. Wei, A. Al Choueiry, G. Lanty, A. Brehier, L. Galmiche, G. Clavier, C. Boissiere, J. S. Lauret, and E. Deleporte, “Preparations and characterizations of luminescent two dimensional organic-inorganic perovskite semiconductors,” Materials (Basel) 3(5), 3385–3406 (2010).
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Nano Lett. (6)

C. D. LaBoda, A. R. Lebeck, and C. L. Dwyer, “An optically modulated self-Assembled resonance energy transfer pass gate,” Nano Lett. 17(6), 3775–3781 (2017).
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D. Kozawa, A. Carvalho, I. Verzhbitskiy, F. Giustiniano, Y. Miyauchi, S. Mouri, A. H. Castro Neto, K. Matsuda, and G. Eda, “Evidence for fast interlayer energy transfer in MoSe2/WS2 heterostructures,” Nano Lett. 16(7), 4087–4093 (2016).
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C. Wang and E. A. Weiss, “Accelerating FRET between near-infrared emitting quantum dots using a molecular J-aggregate as an exciton bridge,” Nano Lett. 17(9), 5666–5671 (2017).
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F. Ceballos, M. G. Ju, S. D. Lane, X. C. Zeng, and H. Zhao, “Highly efficient and anomalous charge transfer in van der Waals trilayer semiconductors,” Nano Lett. 17(3), 1623–1628 (2017).
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D. Ma, Y. Fu, L. Dang, J. Zhai, I. A. Guzei, and S. Jin, “Single-crystal microplates of two-dimensional organic–inorganic lead halide layered perovskites for optoelectronics,” Nano Res. 10(6), 2117–2129 (2017).
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Nanoscale (1)

H. Li, X. Zheng, Y. Liu, Z. Zhang, and T. Jiang, “Ultrafast interfacial energy transfer and interlayer excitons in the monolayer WS2/CsPbBr3 quantum dot heterostructure,” Nanoscale 10(4), 1650–1659 (2018).
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Nat. Commun. (4)

A. Raja, A. Chaves, J. Yu, G. Arefe, H. M. Hill, A. F. Rigosi, T. C. Berkelbach, P. Nagler, C. Schüller, T. Korn, C. Nuckolls, J. Hone, L. E. Brus, T. F. Heinz, D. R. Reichman, and A. Chernikov, “Coulomb engineering of the bandgap and excitons in two-dimensional materials,” Nat. Commun. 8, 15251 (2017).
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X. Yang, X. Zhang, J. Deng, Z. Chu, Q. Jiang, J. Meng, P. Wang, L. Zhang, Z. Yin, and J. You, “Efficient green light-emitting diodes based on quasi-two-dimensional composition and phase engineered perovskite with surface passivation,” Nat. Commun. 9(1), 570 (2018).
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Nat. Mater. (1)

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
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Nat. Photonics (1)

J. T. Li, S. K. Cushing, F. K. Meng, T. R. Senty, A. D. Bristow, and N. Q. Wu, “Plasmon-induced resonance energy transfer for solar energy conversion,” Nat. Photonics 9(9), 601–607 (2015).
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W. Li, Z. Wang, F. Deschler, S. Gao, R. H. Friend, and A. K. Cheetham, “Chemically diverse and multifunctional hybrid organic-inorganic perovskites,” Nat. Rev. Mat. 2(3), 16099 (2017).
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Nature (2)

W. Xu, W. Liu, J. F. Schmidt, W. Zhao, X. Lu, T. Raab, C. Diederichs, W. Gao, D. V. Seletskiy, and Q. Xiong, “Correlated fluorescence blinking in two-dimensional semiconductor heterostructures,” Nature 541(7635), 62–67 (2017).
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Photon. Res. (1)

Phys. Chem. Chem. Phys. (1)

H. Lu, H. Zhang, S. Yuan, J. Wang, Y. Zhan, and L. Zheng, “An optical dynamic study of MAPbBr3 single crystals passivated with MAPbCl3/I3-MAPbBr3 heterojunctions,” Phys. Chem. Chem. Phys. 19(6), 4516–4521 (2017).
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Science (3)

L. Wang, I. Meric, P. Y. Huang, Q. Gao, Y. Gao, H. Tran, T. Taniguchi, K. Watanabe, L. M. Campos, D. A. Muller, J. Guo, P. Kim, J. Hone, K. L. Shepard, and C. R. Dean, “One-dimensional electrical contact to a two-dimensional material,” Science 342(6158), 614–617 (2013).
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Figures (5)

Fig. 1
Fig. 1 Optical microscope images of (a) a mechanically exfoliated (PEA)2PbI4 flake and (b) a MAPbBr3 microplate. (c) XRD patterns of the prepared (PEA)2PbI4 (up panel) and MAPbBr3 (bottom panel) monocrystallines, respectively. (d) Optical microscope image of a prepared perovskite heterostructure. (e) Normalized absorption spectrum of MAPbBr3 (red curve) and PL spectrum of (PEA)2PbI4 (green curve), respectively.
Fig. 2
Fig. 2 (a) Schematic of an inverted-confocal-microscope configuration used for optical measurements. (b) Two-photon-absorption-induced PL (TPL) spectra of the MAPbBr3 microplate, the (PEA)2PbI4 flake and the perovskite heterostructure (H) under forward excitation. (c) Integrated PL mapping of the perovskite heterostructure under forward excitation. (d) TPL spectra of the MAPbBr3 microplate, the (PEA)2PbI4 flake and the perovskite heterostructure (H) under backward excitation.
Fig. 3
Fig. 3 (a) Schematic of energy transfer from the excited (PEA)2PbI4 flake to the MAPbBr3 microplate. (b) Schematic of band alignment of (PEA)2PbI4 and MAPbBr3, showing a type-II band alignment. TPL spectra of the individual components and the heterostructures (c) separated by a 5-nm-thick dielectric layer (H1), (d) separated by a 10-nm-thick dielectric layer (H2), and (e) separated by a 400-μm-thick dielectric layer (H3), respectively, under forward excitation.
Fig. 4
Fig. 4 (a) Time-resolved PL decay traces and the corresponding fitted results for the MAPbBr3 microplate (black), the (PEA)2PbI4 flake (green) and the perovskite heterostructure (H) (red), respectively. (b) Enlarged PL decay traces shown in (a).
Fig. 5
Fig. 5 (a) PL spectra and (b) decay traces for the individual perovskite components and heterostructure (H) respectively, under forward excitation at 400 nm. The thickness of the MAPbBr3 microplate (> 1 μm) is much larger than the penetration depth of the laser beam (163 nm). (c) PL spectra for the individual perovskite components and heterostructure (H) with a 215-nm-thick MAPbBr3 microplate, under forward excitation at 400 nm. (d) PL spectra for the individual perovskite components and heterostructure (H) with a 420-nm-thick MAPbBr3 microplate, under forward excitation at 473 nm.

Equations (2)

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1 τ D = 1 τ D 0 + k T
Φ T =1 τ D τ D 0 = k T τ D 0 1+ k T τ D 0 1.

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