Abstract

266 nm laser output in NaSr3Be3B3O9F4 crystal by the fourth harmonic generation process with a picosecond mode-locked Nd-based YAG laser has been done for the first time. When the input pumping energy was 870 μJ at 532 nm, a 280 μJ 266 nm UV laser was obtained and the corresponding conversion efficiency was 35.9%. Further investigations identified that NaSr3Be3B3O9F4 has a large acceptance angle width of 0.47 (mrad • cm), a small walk-off angle of 35.43 mrad and a large deff as 0.62 pm/V for the fourth harmonic generation. These results indicate that NSBBF is applicable for high-power 266 nm laser generation.

© 2017 Optical Society of America

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    [Crossref] [PubMed]
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    [Crossref]
  30. W. G. Zhang, H. W. Yu, H. P. Wu, and P. S. Halasyamani, “Phase-Matching in Nonlinear Optical Compounds: A Materials Perspective,” Chem. Mater. 29(7), 2655–2668 (2017).
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2017 (1)

W. G. Zhang, H. W. Yu, H. P. Wu, and P. S. Halasyamani, “Phase-Matching in Nonlinear Optical Compounds: A Materials Perspective,” Chem. Mater. 29(7), 2655–2668 (2017).
[Crossref]

2016 (1)

2015 (1)

X. S. Wang, L. J. Liu, X. Y. Wang, L. Bai, and C. T. Chen, “Growth and optical properties of the novel nonlinear optical crystal NaSr3Be3B3O9F4,” CrystEngComm 17(4), 925–929 (2015).
[Crossref]

2012 (1)

L. R. Wang, G. L. Wang, X. Zhang, L. J. Liu, X. Y. Wang, Y. Zhu, and C. T. Chen, “Generation of Ultraviolet Radiation at 266 nm with RbBe2BO3F2 Crystal,” Chin. Phys. Lett. 29(6), 064203 (2012).
[Crossref]

2011 (3)

J. Wang, Y. Yue, J. Yao, and Z. Hu, “Growth and characterization of Ba(Al,Ga)BO3F2 crystal,” J. Cryst. Growth 318(1), 962–965 (2011).
[Crossref]

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

X. Y. Wang, X. Yan, S. Y. Luo, and C. T. Chen, “Flux growth of large KBBF crystals by localized spontaneous nucleation,” J. Cryst. Growth 318(1), 610–612 (2011).
[Crossref]

2010 (1)

X. Yan, Q. Liu, H. Chen, X. Fu, M. Gong, and D. Wang, “35.1 W all-solid-state 355 nm ultraviolet laser,” Laser Phys. Lett. 7(8), 563–568 (2010).
[Crossref]

2009 (3)

E. S. Allee, H. Y. Pang, and N. Hodgson, “Q-switched diode-pumped Nd:YAG rod laser with output power of 420W at 532nm and 160W at 355nm,” Proc. SPIE 7193, 1–8 (2009).

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2-discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
[Crossref]

C. Chen, S. Luo, X. Wang, G. Wang, X. Wen, H. Wu, X. Zhang, and Z. Xu, “Deep UV nonlinear optical crystal: RbBe2(BO3)F2,” J. Opt. Soc. Am. B 26(8), 1519–1525 (2009).
[Crossref]

2008 (1)

D. Rytz, A. Gross, S. Vernay, and V. Wesemann, “YAl3(BO3)4: a novel NLO crystal for frequency conversion to UV wavelengths,” Proc. SPIE 6998, 699814 (2008).
[Crossref]

2007 (1)

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

2006 (2)

A. G. Al-Ama, E. L. Belokoneva, S. Y. Stefanovich, O. V. Dimitrova, and N. N. Mochenova, “Potassium bromo-borate K3[B6O10]Br—A new nonlinear optical material,” Crystallogr. Rep. 51(2), 225–230 (2006).
[Crossref]

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

2005 (1)

A. Görtler and C. Strowitzki, “Excimer Lasers – The powerful light source in the UV and VUV,” Laser Tech. J. 2(2), 46–50 (2005).
[Crossref]

2001 (2)

L. I. Isaenko, A. Dragomir, J. G. McInerney, and D. N. Nikogosyan, “Anisotropy of two-photon absorption in BBO at 264 nm,” Opt. Commun. 198(4-6), 433–438 (2001).
[Crossref]

D. Y. Tang, Y. N. Xia, B. C. Wu, and C. T. Chen, “Growth of a new UV nonlinear optical crystal: KBe2(BO3)F2,” J. Cryst. Growth 222(1-2), 125–129 (2001).
[Crossref]

2000 (1)

1998 (2)

N. Ye, W. Zeng, B. Wu, and C. Chen, “Two new nonlinear optical crystals: BaAl2B2O7 and K2Al2B2O7,” Proc. SPIE 3556, 21–23 (1998).
[Crossref]

Z. G. Hu, T. Higashiyama, M. Yoshimura, Y. K. Yap, Y. Mori, and T. Sasaki, “A New Nonlinear Optical Borate Crystal K2Al2B2O7 (KAB),” J. Appl. Phys. 37(Part 2, No. 10A), L1093–L1094 (1998).
[Crossref]

1995 (1)

T. Sasaki, Y. Mori, I. Kuroda, S. Nakajima, K. Yamaguchi, S. Watanabe, and S. Nakai, “Cesium Lithium Borate - a New Nonlinear-Optical Crystal,” Acta Crystallogr. C 51(11), 2222–2224 (1995).
[Crossref]

1993 (1)

Y. Wu, T. Sasaki, S. Nakai, A. Yokotani, H. Tang, and C. Chen, “CsB3O5: A new nonlinear optical crystal,” Appl. Phys. Lett. 62(21), 2614–2615 (1993).
[Crossref]

1989 (1)

1985 (1)

C. T. Chen, B. C. Wu, A. D. Jiang, and G. M. You, “A New-Type Ultraviolet SHG Crystal - Beta-BaB2O4,” Sci. Sin. [B] 28, 235–241 (1985).

1976 (1)

I. A. Baidina, V. V. Bakakin, L. R. Batsanova, N. A. Pal’chik, N. V. Podberezskaya, and L. P. Solov’eva, “X-ray structural study of borato-fluoroberyllates with the composition MBe2(BO3)F2 (M=Na, K, Rb, Cs),” J. Struct. Chem. 16(6), 963–965 (1976).
[Crossref]

Al-Ama, A. G.

A. G. Al-Ama, E. L. Belokoneva, S. Y. Stefanovich, O. V. Dimitrova, and N. N. Mochenova, “Potassium bromo-borate K3[B6O10]Br—A new nonlinear optical material,” Crystallogr. Rep. 51(2), 225–230 (2006).
[Crossref]

Allee, E. S.

E. S. Allee, H. Y. Pang, and N. Hodgson, “Q-switched diode-pumped Nd:YAG rod laser with output power of 420W at 532nm and 160W at 355nm,” Proc. SPIE 7193, 1–8 (2009).

Bai, L.

X. S. Wang, L. J. Liu, X. Y. Wang, L. Bai, and C. T. Chen, “Growth and optical properties of the novel nonlinear optical crystal NaSr3Be3B3O9F4,” CrystEngComm 17(4), 925–929 (2015).
[Crossref]

Baidina, I. A.

I. A. Baidina, V. V. Bakakin, L. R. Batsanova, N. A. Pal’chik, N. V. Podberezskaya, and L. P. Solov’eva, “X-ray structural study of borato-fluoroberyllates with the composition MBe2(BO3)F2 (M=Na, K, Rb, Cs),” J. Struct. Chem. 16(6), 963–965 (1976).
[Crossref]

Bakakin, V. V.

I. A. Baidina, V. V. Bakakin, L. R. Batsanova, N. A. Pal’chik, N. V. Podberezskaya, and L. P. Solov’eva, “X-ray structural study of borato-fluoroberyllates with the composition MBe2(BO3)F2 (M=Na, K, Rb, Cs),” J. Struct. Chem. 16(6), 963–965 (1976).
[Crossref]

Batsanova, L. R.

I. A. Baidina, V. V. Bakakin, L. R. Batsanova, N. A. Pal’chik, N. V. Podberezskaya, and L. P. Solov’eva, “X-ray structural study of borato-fluoroberyllates with the composition MBe2(BO3)F2 (M=Na, K, Rb, Cs),” J. Struct. Chem. 16(6), 963–965 (1976).
[Crossref]

Belokoneva, E. L.

A. G. Al-Ama, E. L. Belokoneva, S. Y. Stefanovich, O. V. Dimitrova, and N. N. Mochenova, “Potassium bromo-borate K3[B6O10]Br—A new nonlinear optical material,” Crystallogr. Rep. 51(2), 225–230 (2006).
[Crossref]

Bi, Y.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Bo, Y.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Chen, C.

B. Xu, Z. Hou, M. Xia, L. Liu, X. Wang, R. Li, and C. Chen, “High average power third harmonic generation at 355 nm with K3B6O10Br crystal,” Opt. Express 24(10), 10345–10351 (2016).
[Crossref] [PubMed]

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

C. Chen, S. Luo, X. Wang, G. Wang, X. Wen, H. Wu, X. Zhang, and Z. Xu, “Deep UV nonlinear optical crystal: RbBe2(BO3)F2,” J. Opt. Soc. Am. B 26(8), 1519–1525 (2009).
[Crossref]

N. Ye, W. Zeng, B. Wu, and C. Chen, “Two new nonlinear optical crystals: BaAl2B2O7 and K2Al2B2O7,” Proc. SPIE 3556, 21–23 (1998).
[Crossref]

Y. Wu, T. Sasaki, S. Nakai, A. Yokotani, H. Tang, and C. Chen, “CsB3O5: A new nonlinear optical crystal,” Appl. Phys. Lett. 62(21), 2614–2615 (1993).
[Crossref]

C. Chen, Y. Wu, A. Jiang, B. Wu, G. You, R. Li, and S. Lin, “New nonlinear-optical crystal: LiB3O5,” J. Opt. Soc. Am. B 6(4), 616–621 (1989).
[Crossref]

Chen, C. T.

X. S. Wang, L. J. Liu, X. Y. Wang, L. Bai, and C. T. Chen, “Growth and optical properties of the novel nonlinear optical crystal NaSr3Be3B3O9F4,” CrystEngComm 17(4), 925–929 (2015).
[Crossref]

L. R. Wang, G. L. Wang, X. Zhang, L. J. Liu, X. Y. Wang, Y. Zhu, and C. T. Chen, “Generation of Ultraviolet Radiation at 266 nm with RbBe2BO3F2 Crystal,” Chin. Phys. Lett. 29(6), 064203 (2012).
[Crossref]

X. Y. Wang, X. Yan, S. Y. Luo, and C. T. Chen, “Flux growth of large KBBF crystals by localized spontaneous nucleation,” J. Cryst. Growth 318(1), 610–612 (2011).
[Crossref]

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2-discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
[Crossref]

D. Y. Tang, Y. N. Xia, B. C. Wu, and C. T. Chen, “Growth of a new UV nonlinear optical crystal: KBe2(BO3)F2,” J. Cryst. Growth 222(1-2), 125–129 (2001).
[Crossref]

C. T. Chen, B. C. Wu, A. D. Jiang, and G. M. You, “A New-Type Ultraviolet SHG Crystal - Beta-BaB2O4,” Sci. Sin. [B] 28, 235–241 (1985).

Chen, H.

X. Yan, Q. Liu, H. Chen, X. Fu, M. Gong, and D. Wang, “35.1 W all-solid-state 355 nm ultraviolet laser,” Laser Phys. Lett. 7(8), 563–568 (2010).
[Crossref]

Cui, D.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Cui, D. F.

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Dimitrova, O. V.

A. G. Al-Ama, E. L. Belokoneva, S. Y. Stefanovich, O. V. Dimitrova, and N. N. Mochenova, “Potassium bromo-borate K3[B6O10]Br—A new nonlinear optical material,” Crystallogr. Rep. 51(2), 225–230 (2006).
[Crossref]

Dragomir, A.

L. I. Isaenko, A. Dragomir, J. G. McInerney, and D. N. Nikogosyan, “Anisotropy of two-photon absorption in BBO at 264 nm,” Opt. Commun. 198(4-6), 433–438 (2001).
[Crossref]

Dubietis, A.

Fu, X.

X. Yan, Q. Liu, H. Chen, X. Fu, M. Gong, and D. Wang, “35.1 W all-solid-state 355 nm ultraviolet laser,” Laser Phys. Lett. 7(8), 563–568 (2010).
[Crossref]

Geng, A.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Gong, M.

X. Yan, Q. Liu, H. Chen, X. Fu, M. Gong, and D. Wang, “35.1 W all-solid-state 355 nm ultraviolet laser,” Laser Phys. Lett. 7(8), 563–568 (2010).
[Crossref]

Görtler, A.

A. Görtler and C. Strowitzki, “Excimer Lasers – The powerful light source in the UV and VUV,” Laser Tech. J. 2(2), 46–50 (2005).
[Crossref]

Gross, A.

D. Rytz, A. Gross, S. Vernay, and V. Wesemann, “YAl3(BO3)4: a novel NLO crystal for frequency conversion to UV wavelengths,” Proc. SPIE 6998, 699814 (2008).
[Crossref]

Guo, L.

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Halasyamani, P. S.

W. G. Zhang, H. W. Yu, H. P. Wu, and P. S. Halasyamani, “Phase-Matching in Nonlinear Optical Compounds: A Materials Perspective,” Chem. Mater. 29(7), 2655–2668 (2017).
[Crossref]

He, R.

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

Higashiyama, T.

Z. G. Hu, T. Higashiyama, M. Yoshimura, Y. K. Yap, Y. Mori, and T. Sasaki, “A New Nonlinear Optical Borate Crystal K2Al2B2O7 (KAB),” J. Appl. Phys. 37(Part 2, No. 10A), L1093–L1094 (1998).
[Crossref]

Hodgson, N.

E. S. Allee, H. Y. Pang, and N. Hodgson, “Q-switched diode-pumped Nd:YAG rod laser with output power of 420W at 532nm and 160W at 355nm,” Proc. SPIE 7193, 1–8 (2009).

Hou, Z.

Hu, Z.

J. Wang, Y. Yue, J. Yao, and Z. Hu, “Growth and characterization of Ba(Al,Ga)BO3F2 crystal,” J. Cryst. Growth 318(1), 962–965 (2011).
[Crossref]

Hu, Z. G.

Z. G. Hu, T. Higashiyama, M. Yoshimura, Y. K. Yap, Y. Mori, and T. Sasaki, “A New Nonlinear Optical Borate Crystal K2Al2B2O7 (KAB),” J. Appl. Phys. 37(Part 2, No. 10A), L1093–L1094 (1998).
[Crossref]

Huang, H.

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

Huang, J. Y.

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Isaenko, L. I.

L. I. Isaenko, A. Dragomir, J. G. McInerney, and D. N. Nikogosyan, “Anisotropy of two-photon absorption in BBO at 264 nm,” Opt. Commun. 198(4-6), 433–438 (2001).
[Crossref]

Jiang, A.

Jiang, A. D.

C. T. Chen, B. C. Wu, A. D. Jiang, and G. M. You, “A New-Type Ultraviolet SHG Crystal - Beta-BaB2O4,” Sci. Sin. [B] 28, 235–241 (1985).

Kuroda, I.

T. Sasaki, Y. Mori, I. Kuroda, S. Nakajima, K. Yamaguchi, S. Watanabe, and S. Nakai, “Cesium Lithium Borate - a New Nonlinear-Optical Crystal,” Acta Crystallogr. C 51(11), 2222–2224 (1995).
[Crossref]

Li, H.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Li, R.

Lin, S.

Lin, Z.

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

Liu, L.

Liu, L. J.

X. S. Wang, L. J. Liu, X. Y. Wang, L. Bai, and C. T. Chen, “Growth and optical properties of the novel nonlinear optical crystal NaSr3Be3B3O9F4,” CrystEngComm 17(4), 925–929 (2015).
[Crossref]

L. R. Wang, G. L. Wang, X. Zhang, L. J. Liu, X. Y. Wang, Y. Zhu, and C. T. Chen, “Generation of Ultraviolet Radiation at 266 nm with RbBe2BO3F2 Crystal,” Chin. Phys. Lett. 29(6), 064203 (2012).
[Crossref]

Liu, Q.

X. Yan, Q. Liu, H. Chen, X. Fu, M. Gong, and D. Wang, “35.1 W all-solid-state 355 nm ultraviolet laser,” Laser Phys. Lett. 7(8), 563–568 (2010).
[Crossref]

Lu, L.

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Luo, S.

Luo, S. Y.

X. Y. Wang, X. Yan, S. Y. Luo, and C. T. Chen, “Flux growth of large KBBF crystals by localized spontaneous nucleation,” J. Cryst. Growth 318(1), 610–612 (2011).
[Crossref]

McInerney, J. G.

L. I. Isaenko, A. Dragomir, J. G. McInerney, and D. N. Nikogosyan, “Anisotropy of two-photon absorption in BBO at 264 nm,” Opt. Commun. 198(4-6), 433–438 (2001).
[Crossref]

Mochenova, N. N.

A. G. Al-Ama, E. L. Belokoneva, S. Y. Stefanovich, O. V. Dimitrova, and N. N. Mochenova, “Potassium bromo-borate K3[B6O10]Br—A new nonlinear optical material,” Crystallogr. Rep. 51(2), 225–230 (2006).
[Crossref]

Mori, Y.

Z. G. Hu, T. Higashiyama, M. Yoshimura, Y. K. Yap, Y. Mori, and T. Sasaki, “A New Nonlinear Optical Borate Crystal K2Al2B2O7 (KAB),” J. Appl. Phys. 37(Part 2, No. 10A), L1093–L1094 (1998).
[Crossref]

T. Sasaki, Y. Mori, I. Kuroda, S. Nakajima, K. Yamaguchi, S. Watanabe, and S. Nakai, “Cesium Lithium Borate - a New Nonlinear-Optical Crystal,” Acta Crystallogr. C 51(11), 2222–2224 (1995).
[Crossref]

Nakai, S.

T. Sasaki, Y. Mori, I. Kuroda, S. Nakajima, K. Yamaguchi, S. Watanabe, and S. Nakai, “Cesium Lithium Borate - a New Nonlinear-Optical Crystal,” Acta Crystallogr. C 51(11), 2222–2224 (1995).
[Crossref]

Y. Wu, T. Sasaki, S. Nakai, A. Yokotani, H. Tang, and C. Chen, “CsB3O5: A new nonlinear optical crystal,” Appl. Phys. Lett. 62(21), 2614–2615 (1993).
[Crossref]

Nakajima, S.

T. Sasaki, Y. Mori, I. Kuroda, S. Nakajima, K. Yamaguchi, S. Watanabe, and S. Nakai, “Cesium Lithium Borate - a New Nonlinear-Optical Crystal,” Acta Crystallogr. C 51(11), 2222–2224 (1995).
[Crossref]

Nikogosyan, D. N.

L. I. Isaenko, A. Dragomir, J. G. McInerney, and D. N. Nikogosyan, “Anisotropy of two-photon absorption in BBO at 264 nm,” Opt. Commun. 198(4-6), 433–438 (2001).
[Crossref]

Pal’chik, N. A.

I. A. Baidina, V. V. Bakakin, L. R. Batsanova, N. A. Pal’chik, N. V. Podberezskaya, and L. P. Solov’eva, “X-ray structural study of borato-fluoroberyllates with the composition MBe2(BO3)F2 (M=Na, K, Rb, Cs),” J. Struct. Chem. 16(6), 963–965 (1976).
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Pang, H. Y.

E. S. Allee, H. Y. Pang, and N. Hodgson, “Q-switched diode-pumped Nd:YAG rod laser with output power of 420W at 532nm and 160W at 355nm,” Proc. SPIE 7193, 1–8 (2009).

Podberezskaya, N. V.

I. A. Baidina, V. V. Bakakin, L. R. Batsanova, N. A. Pal’chik, N. V. Podberezskaya, and L. P. Solov’eva, “X-ray structural study of borato-fluoroberyllates with the composition MBe2(BO3)F2 (M=Na, K, Rb, Cs),” J. Struct. Chem. 16(6), 963–965 (1976).
[Crossref]

Rytz, D.

D. Rytz, A. Gross, S. Vernay, and V. Wesemann, “YAl3(BO3)4: a novel NLO crystal for frequency conversion to UV wavelengths,” Proc. SPIE 6998, 699814 (2008).
[Crossref]

Sasaki, T.

Z. G. Hu, T. Higashiyama, M. Yoshimura, Y. K. Yap, Y. Mori, and T. Sasaki, “A New Nonlinear Optical Borate Crystal K2Al2B2O7 (KAB),” J. Appl. Phys. 37(Part 2, No. 10A), L1093–L1094 (1998).
[Crossref]

T. Sasaki, Y. Mori, I. Kuroda, S. Nakajima, K. Yamaguchi, S. Watanabe, and S. Nakai, “Cesium Lithium Borate - a New Nonlinear-Optical Crystal,” Acta Crystallogr. C 51(11), 2222–2224 (1995).
[Crossref]

Y. Wu, T. Sasaki, S. Nakai, A. Yokotani, H. Tang, and C. Chen, “CsB3O5: A new nonlinear optical crystal,” Appl. Phys. Lett. 62(21), 2614–2615 (1993).
[Crossref]

Shen, D.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Shen, G.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Solov’eva, L. P.

I. A. Baidina, V. V. Bakakin, L. R. Batsanova, N. A. Pal’chik, N. V. Podberezskaya, and L. P. Solov’eva, “X-ray structural study of borato-fluoroberyllates with the composition MBe2(BO3)F2 (M=Na, K, Rb, Cs),” J. Struct. Chem. 16(6), 963–965 (1976).
[Crossref]

Stefanovich, S. Y.

A. G. Al-Ama, E. L. Belokoneva, S. Y. Stefanovich, O. V. Dimitrova, and N. N. Mochenova, “Potassium bromo-borate K3[B6O10]Br—A new nonlinear optical material,” Crystallogr. Rep. 51(2), 225–230 (2006).
[Crossref]

Strowitzki, C.

A. Görtler and C. Strowitzki, “Excimer Lasers – The powerful light source in the UV and VUV,” Laser Tech. J. 2(2), 46–50 (2005).
[Crossref]

Sun, Z.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Tamosauskas, G.

Tang, D. Y.

D. Y. Tang, Y. N. Xia, B. C. Wu, and C. T. Chen, “Growth of a new UV nonlinear optical crystal: KBe2(BO3)F2,” J. Cryst. Growth 222(1-2), 125–129 (2001).
[Crossref]

Tang, H.

Y. Wu, T. Sasaki, S. Nakai, A. Yokotani, H. Tang, and C. Chen, “CsB3O5: A new nonlinear optical crystal,” Appl. Phys. Lett. 62(21), 2614–2615 (1993).
[Crossref]

Valiulis, G.

Varanavicius, A.

Vernay, S.

D. Rytz, A. Gross, S. Vernay, and V. Wesemann, “YAl3(BO3)4: a novel NLO crystal for frequency conversion to UV wavelengths,” Proc. SPIE 6998, 699814 (2008).
[Crossref]

Wang, D.

X. Yan, Q. Liu, H. Chen, X. Fu, M. Gong, and D. Wang, “35.1 W all-solid-state 355 nm ultraviolet laser,” Laser Phys. Lett. 7(8), 563–568 (2010).
[Crossref]

Wang, G.

C. Chen, S. Luo, X. Wang, G. Wang, X. Wen, H. Wu, X. Zhang, and Z. Xu, “Deep UV nonlinear optical crystal: RbBe2(BO3)F2,” J. Opt. Soc. Am. B 26(8), 1519–1525 (2009).
[Crossref]

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Wang, G. L.

L. R. Wang, G. L. Wang, X. Zhang, L. J. Liu, X. Y. Wang, Y. Zhu, and C. T. Chen, “Generation of Ultraviolet Radiation at 266 nm with RbBe2BO3F2 Crystal,” Chin. Phys. Lett. 29(6), 064203 (2012).
[Crossref]

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2-discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
[Crossref]

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Wang, J.

J. Wang, Y. Yue, J. Yao, and Z. Hu, “Growth and characterization of Ba(Al,Ga)BO3F2 crystal,” J. Cryst. Growth 318(1), 962–965 (2011).
[Crossref]

Wang, L. R.

L. R. Wang, G. L. Wang, X. Zhang, L. J. Liu, X. Y. Wang, Y. Zhu, and C. T. Chen, “Generation of Ultraviolet Radiation at 266 nm with RbBe2BO3F2 Crystal,” Chin. Phys. Lett. 29(6), 064203 (2012).
[Crossref]

Wang, X.

B. Xu, Z. Hou, M. Xia, L. Liu, X. Wang, R. Li, and C. Chen, “High average power third harmonic generation at 355 nm with K3B6O10Br crystal,” Opt. Express 24(10), 10345–10351 (2016).
[Crossref] [PubMed]

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

C. Chen, S. Luo, X. Wang, G. Wang, X. Wen, H. Wu, X. Zhang, and Z. Xu, “Deep UV nonlinear optical crystal: RbBe2(BO3)F2,” J. Opt. Soc. Am. B 26(8), 1519–1525 (2009).
[Crossref]

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Wang, X. S.

X. S. Wang, L. J. Liu, X. Y. Wang, L. Bai, and C. T. Chen, “Growth and optical properties of the novel nonlinear optical crystal NaSr3Be3B3O9F4,” CrystEngComm 17(4), 925–929 (2015).
[Crossref]

Wang, X. Y.

X. S. Wang, L. J. Liu, X. Y. Wang, L. Bai, and C. T. Chen, “Growth and optical properties of the novel nonlinear optical crystal NaSr3Be3B3O9F4,” CrystEngComm 17(4), 925–929 (2015).
[Crossref]

L. R. Wang, G. L. Wang, X. Zhang, L. J. Liu, X. Y. Wang, Y. Zhu, and C. T. Chen, “Generation of Ultraviolet Radiation at 266 nm with RbBe2BO3F2 Crystal,” Chin. Phys. Lett. 29(6), 064203 (2012).
[Crossref]

X. Y. Wang, X. Yan, S. Y. Luo, and C. T. Chen, “Flux growth of large KBBF crystals by localized spontaneous nucleation,” J. Cryst. Growth 318(1), 610–612 (2011).
[Crossref]

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2-discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
[Crossref]

Watanabe, S.

T. Sasaki, Y. Mori, I. Kuroda, S. Nakajima, K. Yamaguchi, S. Watanabe, and S. Nakai, “Cesium Lithium Borate - a New Nonlinear-Optical Crystal,” Acta Crystallogr. C 51(11), 2222–2224 (1995).
[Crossref]

Wen, X.

Wesemann, V.

D. Rytz, A. Gross, S. Vernay, and V. Wesemann, “YAl3(BO3)4: a novel NLO crystal for frequency conversion to UV wavelengths,” Proc. SPIE 6998, 699814 (2008).
[Crossref]

Wu, B.

N. Ye, W. Zeng, B. Wu, and C. Chen, “Two new nonlinear optical crystals: BaAl2B2O7 and K2Al2B2O7,” Proc. SPIE 3556, 21–23 (1998).
[Crossref]

C. Chen, Y. Wu, A. Jiang, B. Wu, G. You, R. Li, and S. Lin, “New nonlinear-optical crystal: LiB3O5,” J. Opt. Soc. Am. B 6(4), 616–621 (1989).
[Crossref]

Wu, B. C.

D. Y. Tang, Y. N. Xia, B. C. Wu, and C. T. Chen, “Growth of a new UV nonlinear optical crystal: KBe2(BO3)F2,” J. Cryst. Growth 222(1-2), 125–129 (2001).
[Crossref]

C. T. Chen, B. C. Wu, A. D. Jiang, and G. M. You, “A New-Type Ultraviolet SHG Crystal - Beta-BaB2O4,” Sci. Sin. [B] 28, 235–241 (1985).

Wu, H.

Wu, H. P.

W. G. Zhang, H. W. Yu, H. P. Wu, and P. S. Halasyamani, “Phase-Matching in Nonlinear Optical Compounds: A Materials Perspective,” Chem. Mater. 29(7), 2655–2668 (2017).
[Crossref]

Wu, Y.

Y. Wu, T. Sasaki, S. Nakai, A. Yokotani, H. Tang, and C. Chen, “CsB3O5: A new nonlinear optical crystal,” Appl. Phys. Lett. 62(21), 2614–2615 (1993).
[Crossref]

C. Chen, Y. Wu, A. Jiang, B. Wu, G. You, R. Li, and S. Lin, “New nonlinear-optical crystal: LiB3O5,” J. Opt. Soc. Am. B 6(4), 616–621 (1989).
[Crossref]

Wu, Y. C.

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Xia, M.

Xia, Y. N.

D. Y. Tang, Y. N. Xia, B. C. Wu, and C. T. Chen, “Growth of a new UV nonlinear optical crystal: KBe2(BO3)F2,” J. Cryst. Growth 222(1-2), 125–129 (2001).
[Crossref]

Xu, B.

Xu, Z.

C. Chen, S. Luo, X. Wang, G. Wang, X. Wen, H. Wu, X. Zhang, and Z. Xu, “Deep UV nonlinear optical crystal: RbBe2(BO3)F2,” J. Opt. Soc. Am. B 26(8), 1519–1525 (2009).
[Crossref]

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Xu, Z. Y.

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2-discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
[Crossref]

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Yamaguchi, K.

T. Sasaki, Y. Mori, I. Kuroda, S. Nakajima, K. Yamaguchi, S. Watanabe, and S. Nakai, “Cesium Lithium Borate - a New Nonlinear-Optical Crystal,” Acta Crystallogr. C 51(11), 2222–2224 (1995).
[Crossref]

Yan, X.

X. Y. Wang, X. Yan, S. Y. Luo, and C. T. Chen, “Flux growth of large KBBF crystals by localized spontaneous nucleation,” J. Cryst. Growth 318(1), 610–612 (2011).
[Crossref]

X. Yan, Q. Liu, H. Chen, X. Fu, M. Gong, and D. Wang, “35.1 W all-solid-state 355 nm ultraviolet laser,” Laser Phys. Lett. 7(8), 563–568 (2010).
[Crossref]

Yao, J.

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

J. Wang, Y. Yue, J. Yao, and Z. Hu, “Growth and characterization of Ba(Al,Ga)BO3F2 crystal,” J. Cryst. Growth 318(1), 962–965 (2011).
[Crossref]

Yao, W.

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

Yap, Y. K.

Z. G. Hu, T. Higashiyama, M. Yoshimura, Y. K. Yap, Y. Mori, and T. Sasaki, “A New Nonlinear Optical Borate Crystal K2Al2B2O7 (KAB),” J. Appl. Phys. 37(Part 2, No. 10A), L1093–L1094 (1998).
[Crossref]

Ye, N.

N. Ye, W. Zeng, B. Wu, and C. Chen, “Two new nonlinear optical crystals: BaAl2B2O7 and K2Al2B2O7,” Proc. SPIE 3556, 21–23 (1998).
[Crossref]

Yokotani, A.

Y. Wu, T. Sasaki, S. Nakai, A. Yokotani, H. Tang, and C. Chen, “CsB3O5: A new nonlinear optical crystal,” Appl. Phys. Lett. 62(21), 2614–2615 (1993).
[Crossref]

Yoshimura, M.

Z. G. Hu, T. Higashiyama, M. Yoshimura, Y. K. Yap, Y. Mori, and T. Sasaki, “A New Nonlinear Optical Borate Crystal K2Al2B2O7 (KAB),” J. Appl. Phys. 37(Part 2, No. 10A), L1093–L1094 (1998).
[Crossref]

You, G.

You, G. M.

C. T. Chen, B. C. Wu, A. D. Jiang, and G. M. You, “A New-Type Ultraviolet SHG Crystal - Beta-BaB2O4,” Sci. Sin. [B] 28, 235–241 (1985).

Yu, H. W.

W. G. Zhang, H. W. Yu, H. P. Wu, and P. S. Halasyamani, “Phase-Matching in Nonlinear Optical Compounds: A Materials Perspective,” Chem. Mater. 29(7), 2655–2668 (2017).
[Crossref]

Yuan, X.

G. Wang, A. Geng, Y. Bo, H. Li, Z. Sun, Y. Bi, D. Cui, Z. Xu, X. Yuan, X. Wang, G. Shen, and D. Shen, “28.4 W 266 nm ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser,” Opt. Commun. 259(2), 820–822 (2006).
[Crossref]

Yue, Y.

J. Wang, Y. Yue, J. Yao, and Z. Hu, “Growth and characterization of Ba(Al,Ga)BO3F2 crystal,” J. Cryst. Growth 318(1), 962–965 (2011).
[Crossref]

Zeng, W.

N. Ye, W. Zeng, B. Wu, and C. Chen, “Two new nonlinear optical crystals: BaAl2B2O7 and K2Al2B2O7,” Proc. SPIE 3556, 21–23 (1998).
[Crossref]

Zhai, N.

H. Huang, J. Yao, Z. Lin, X. Wang, R. He, W. Yao, N. Zhai, and C. Chen, “NaSr3Be3B3O9F4: A Promising Deep-Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F](10-) Anionic Group,” Angew. Chem. Int. Ed. Engl. 50(39), 9141–9144 (2011).
[Crossref] [PubMed]

Zhang, H. B.

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Zhang, J. Y.

L. Guo, G. L. Wang, H. B. Zhang, D. F. Cui, Y. C. Wu, L. Lu, J. Y. Zhang, J. Y. Huang, and Z. Y. Xu, “High-power picoseconds 355 nm laser by third harmonic generation based on CsB3O5 crystal,” Appl. Phys. B 88(2), 197–200 (2007).
[Crossref]

Zhang, W. G.

W. G. Zhang, H. W. Yu, H. P. Wu, and P. S. Halasyamani, “Phase-Matching in Nonlinear Optical Compounds: A Materials Perspective,” Chem. Mater. 29(7), 2655–2668 (2017).
[Crossref]

Zhang, X.

L. R. Wang, G. L. Wang, X. Zhang, L. J. Liu, X. Y. Wang, Y. Zhu, and C. T. Chen, “Generation of Ultraviolet Radiation at 266 nm with RbBe2BO3F2 Crystal,” Chin. Phys. Lett. 29(6), 064203 (2012).
[Crossref]

C. Chen, S. Luo, X. Wang, G. Wang, X. Wen, H. Wu, X. Zhang, and Z. Xu, “Deep UV nonlinear optical crystal: RbBe2(BO3)F2,” J. Opt. Soc. Am. B 26(8), 1519–1525 (2009).
[Crossref]

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Figures (5)

Fig. 1
Fig. 1 (a)Photograph of this as-grown NSBBF crystal; (b) Photograph of polished NSBBF crystal; (c) Photograph of output 266 nm laser spot; (d) Experimental settings for 266nm laser light generation.
Fig. 2
Fig. 2 Rocking curve of the cut and polished NSBBF crystal plate.
Fig. 3
Fig. 3 Output energy at 266 nm versus input energy at 532 nm (red line), and the corresponding conversion efficiency of NSBBF crystal from 532 nm to 266 nm (blue line).
Fig. 4
Fig. 4 Experimental setup for the measurements of acceptance angle of NSBBF crystal for 266 nm laser output.
Fig. 5
Fig. 5 Fixed curve of experimental records and experimental records for the 266 nm output power versus rotated angles.

Tables (1)

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Table 1 NLO Characteristics of NSBBF and Several Commonly used NLO Crystals for 266nm Generation

Equations (7)

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n e 2 =2.35176+0.0095831/( λ 2 0.015857)0.010554× λ 2 n o 2 =2.52763+0.013118/( λ 2 0.013828)0.011574× λ 2
θ PM =arcsin [ n e 2 (2ω) n o 2 (ω) n o 2 (2ω) n o 2 (ω) n o 2 (2ω) n e 2 (2ω) ] 1/2
d eff = d 31 sinθ d 22 cosθsin3φ TypeI
ρ=arctan{ 1 2 n o 2 (ω)[ n e -2 (2ω) n o -2 (2ω)]sin(2 θ PM ) }
  I 2ω   { sin( lΔk/2 ) lΔk/2 } 2
Δ θ int l= lΔk λ ω 2π n o 3 (ω)[ n e 2 (2ω) n o 2 (2ω)]sin(2 θ PM )
η= I 2ω I ω [ 1- ( n ω o -1 n ω o +1 ) 2 ] -1 [ 1- ( n 2ω e ( θ )-1 n 2ω e ( θ )+1 ) 2 ] -1

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