Abstract
We report comparisons of coherent anti-Stokes Raman spectroscopy (CARS) measurements using single-axial-and multiaxial-mode Nd:YAG lasers. Our results demonstrate the validity of a recently proposed convolution expression for unresolved CARS spectra. The results also support the use of a relative delay of several coherence lengths between pump-beam paths for reducing the effects of pump-field statistics on the CARS spectral profile.
© 1985 Optical Society of America
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