Extended analyses of Se vii and Se viii

Th. A. M. VanKleef; Y. N. Joshi

doi:10.1364/JOSAB.1.000271

Journal of the Optical Society of America B
Vol. 1,
Issue 2,
pp. 271-278
(1984)
•https://doi.org/10.1364/JOSAB.1.000271

Extended analyses of Se vii and Se viii

Th. A. M. VanKleef and Y. N. Joshi

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Th. A. M. VanKleef and Y. N. Joshi, "Extended analyses of Se vii and Se viii," J. Opt. Soc. Am. B 1, 271-278 (1984)

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Abstract

The spectrum of selenium was photographed in the 400–1200-Å wavelength region on a variety of spectrographs by using a triggered spark source. Seventeen of the eighteen levels of the 3d⁹4d configuration of Se vii have been established. The revision of the J = 1 levels of the 3d⁹5p and 3d⁹nf (n = 4–7) configurations has led to a revised value of the ionization limit of Se vii as 3d⁹²D_5/2 = 1 252 800 ± 100 cm⁻¹ (155.3 eV). In Se viii all levels of the 3d⁸4s configuration and missing levels of the 3d⁸4p configuration have been determined. Several levels of the 3d⁸4p configuration have also been revised. The parametric calculations support both analyses. Sixty-four additional lines have been classified in Se vii, and seventy-four additional lines have been classified in Se viii.

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Parameter	LSF	HF	LSF/HF
E_av	759 778 ± 86	754 788	1.007
F²(3d4d)	27 269 ± 427	26 019	1.048
F⁴(3d4d)	14 021 ± 344	11 507	1.218
G⁰(3d4d)^a	5 905	9 085	0.65
G²(3d4d)	10 225 ± 516	9 966	1.026
G⁴(3d4d)	6 862 ± 990	7 432	0.923
ζ₃_d	2 745 ±41	2 792	0.983
ζ₄_d	340 ± 41	303	1.122
β^b	0
T^b	0
α₁^b	0
α₂	19.1 ± 7.2
σ^c	133

	3d84s			3d84p

Parameter	LSF	HF	LSF/HF	LSF^a	HF	LSF/HF
E_av	555 287 ± 117	563 174	0.986	691 684 ± 247	690 979	1.001
F²(3d3d)	150 994 ± 116	170 346	0.886	152 878 ± 238	170 487	0.897
F⁴(3d3d)	96 453 ± 295	107 864	0.894	101 474 ± 602	107 962	0.940
F²(3d4p)	–	–	–	39 670 ± 168	40 322	0.984
G¹(3d4p)	–	–	–	12 517 ± 99	13 356	0.937
G²(3d4s)	15 501 ± 48	15 485	1.001	–	–	–
G³(3d4p)	–	–	–	12 543 ± 346	12 837	0.977
ζ₃_d	3 013 ± 13	2 956	1.019	2 979 ± 28	2 959	1.007
ζ₄_p	–	–	–	5 430 ± 48	4 753	1.142
β	−479 ± 30	–	–	−728 ± 62	–	–
T^b	−8.9	–	–	−8.9	–	–
α₁	89.6 db 2.8	–	–	15.9 ± 9.4	–	–
α₂	–	–	–	33.8 ± 6.6	–	–
σ^c	40	–	–	125	–	–

Designation	J	Level Value (cm⁻¹)	Δ^a	Composition^b
³S	1	745 828.3	−110	93% + 6%³P + 1% ¹P
³G	5	754 490.8	71	100%
	4	754 676.1	56	63% + 36%¹G + 1% ³F
	3	758 457.0	−2	65% + 20%¹F + 11%³F + 5% ³D
3P	2	755 169.9	−20	73% + 26%³D + 1% ³F
	1	759 860.9	9	54% + 38%¹P + 7% ³S + 1% ³D
	0	758 571.1	39	100%
³D	3	757 339.0	106	87% + 10% ³F + 2% ³G
	2	759 492.4	70	48% + 22%¹D + 19%³P + 11% ³F
	1	762 938.6	236	79% + 12% ³P + 9% ¹P
3F	4	763 857.0	12	52% + 26% ¹G + 22%³G
	3	767 345.9	−153	54% + 38% ¹F + 8%³D
	2	767 567.2	−87	57% + 42% ¹D + 1%³P
¹P	1	755 062.8	−116	51% + 28% ³P + 20%³D
¹G	4	759 756.1	−65	38% + 47% ³F + 15% ³G
¹F	3	762 598.8	−110	42% + 33%³G + 25%³F
¹D	2	765 888.2	58	36% + 31%³F + 25%³D + 7%³P
¹S	0	(806 135)^c		100%

Intensity^a	λ (Å)	σ (cm⁻¹)	Classification		Δ(cm⁻¹)^b
10	502.436	199 030.2	$3 d^{9} 4 p {{}^{3}F}_{2}^{\circ}$	3d⁹4d³F₂	−0.6
9	502.554	198 983.6	${{}^{3}F}_{3}^{\circ}$	¹F₃	0.3
32	503.430	198 637.2	${{}^{3}P}_{2}^{\circ}$	³D₃	0.2
30	508.988	196 468.2	${{}^{3}P}_{2}^{\circ}$	³P₂	0.3
2	509.266	196 361.1	${{}^{3}P}_{2}^{\circ}$	¹P₁	0.3
35^c	510.884	195 739.0	${{}^{3}F}_{4}^{\circ}$	³F₄	0.0
12	513.237	194 841.8	${{}^{3}F}_{3}^{\circ}$	³G₃	0.3
16	514.878	194 220.6	${{}^{3}P}_{1}^{\circ}$	³P₁	0.3
9	515.303	194 060.6	${{}^{3}F}_{2}^{\circ}$	¹F₃	−1.7
16	515.861	193 850.7	${{}^{3}P}_{1}^{\circ}$	³D₂	−1.7
7	516.200	193 723.3	${{}^{3}F}_{3}^{\circ}$	³D₃	−0.2
5	517.704	193 160.4	${{}^{3}P}_{0}^{\circ}$	³D₁	−1.2
6	518.319	192 931.4	${{}^{3}P}_{1}^{\circ}$	³P₀	0.0
2	521.397	191 792.4	${{}^{1}F}_{3}^{\circ}$	³F₃	−1.0
24	521.817	191 638.0	${{}^{3}F}_{4}^{\circ}$	¹G₄	−0.1
2	522.046	191 554.0	${{}^{3}F}_{3}^{\circ}$	³P₂	−0.4
53	523.393	191 061.1	${{}^{3}F}_{3}^{\circ}$	³G₄	0.5
2	523.682	190 955.7	${{}^{3}F}_{2}^{\circ}$	³D₂	−0.2
Se ii^d	526.081	190 084.5	${{}^{3}P}_{0}^{\circ}$	³P₁	0.6
41	526.536	189 920.6	${{}^{3}F}_{2}^{\circ}$	³G₃	0.1
2	527.924	189 421.2	${{}^{3}P}_{1}^{\circ}$	¹P₁	0.4
26	528.274	189 295.8	${{}^{1}P}_{1}^{\circ}$	³F₂	0.5
52^e	528.483	189 220.7	${{}^{3}F}_{4}^{\circ}$	³D₃	−0.3
25	529.166	188 976.7	${{}^{3}D}_{3}^{\circ}$	³F₃	0.8
39	533.363	187 489.7	${{}^{1}D}_{2}^{\circ}$	¹F₃	1.4
43	534.396	187 127.2	${{}^{3}P}_{2}^{\circ}$	³S₁	0.8
9	536.023	186 559.0	${{}^{3}F}_{4}^{\circ}$	³G₄	−0.1
62	536.559	186 372.8	${{}^{3}F}_{4}^{\circ}$	³G₅	0.0
54	539.121	185 487.0	${{}^{3}D}_{3}^{\circ}$	³F₁	0.0
10	541.083	184 814.4	${{}^{3}D}_{2}^{\circ}$	³F₂	0.1
6	541.513	184 667.8	${{}^{1}P}_{1}^{\circ}$	³D₁	1.2
42	541.732	184 593.2	${{}^{3}D}_{2}^{\circ}$	³P₃	0.3
44	542.290	184 403.3	${{}^{3}D}_{1}^{\circ}$	¹D₂	0.1
35	542.351	184 382.6	${{}^{1}D}_{2}^{\circ}$	³D₂	0.7
62	542.876	184 203.6	${{}^{1}F}_{3}^{\circ}$	¹G₄	0.0
16	545.417	183 346.1	${{}^{1}D}_{2}^{\circ}$	³G₃	−0.4
7	546.045	183 135.1	${{}^{3}D}_{2}^{\circ}$	¹D₂	−0.1
44	550.096	181 786.4	${{}^{1}F}_{3}^{\circ}$	³D₃	−0.1
7	550.697	181 588.1	${{}^{1}P}_{1}^{\circ}$	³P₁	−0.8
9	551.105	181 453.6	${{}^{3}D}_{1}^{\circ}$	³D₁	0.0
29	554.977	180 187.5	${{}^{3}P}_{1}^{\circ}$	³S₁	−0.8
10	555.699	179 951.4	${{}^{1}D}_{2}^{\circ}$	¹P₁	1.1
5	556.738	179 617.7	${{}^{1}F}_{3}^{\circ}$	³P₂	0.3
2	558.275	179 123.2	${{}^{1}F}_{3}^{\circ}$	³G₄	−0.4
18	558.754	178 969.6	${{}^{3}D}_{3}^{\circ}$	³D₃	0.6
2	560.613	178 376.2	${{}^{3}D}_{1}^{\circ}$	³P₁	0.3
2	564.627	177 108.1	${{}^{3}D}_{2}^{\circ}$	³P₁	0.2
10	565.611	176 799.8	³D₃	³P₂	−0.1
10	565.642	176 790.2	${{}^{1}P}_{1}^{\circ}$	¹P₁	−0.6
2	565.802	176 740.4	${{}^{3}D}_{2}^{\circ}$	³D₂	1.0
23	576.103	173 578.0	${{}^{3}D}_{1}^{\circ}$	¹P₁	0.2

λ (Å)	Intensity	σ (cm⁻¹)	Upper Level
112.832	1	886 275	$3 d^{9} 5 p {{}^{3}P}_{1}^{\circ}$
112.030	65	892 616	$5 p {{}^{1}P}_{1}^{\circ}$
111.817	66	894 316	$5 p {{}^{3}D}_{1}^{\circ}$
110.512	30	904 879	$4 f {{}^{3}P}_{1}^{\circ}$
109.945	60	909 544	$4 f {{}^{3}D}_{1}^{\circ}$
108.962	80	917 749	$4 f {{}^{1}P}_{1}^{\circ}$
97.063	5	1 030 264	$5 f {{}^{3}P}_{1}^{\circ}$
96.762	40	1 033 466	$5 f {{}^{3}D}_{1}^{\circ}$
96.071	50	1 040 901	$5 f {{}^{1}P}_{1}^{\circ}$
90.832	10	1 100 929	$6 f {{}^{3}D}_{1}^{\circ}$
90.253	12	1 108 002	$6 f {{}^{1}P}_{1}^{\circ}$
87.590	2	1 141 687	$7 f {{}^{3}D}_{1}^{\circ}$
87.074	3	1 148 442	$7 f {{}^{1}P}_{1}^{\circ}$

Configuration	Designation	Level (cm⁻¹)	Comment
3d⁹5p	${{}^{3}P}_{1}^{\circ}$	886 280	^a
	${{}^{1}P}_{1}^{\circ}$	892 620	^a
	${{}^{3}D}_{1}^{\circ}$	894 320	^b
3d⁹4f	${{}^{3}P}_{1}^{\circ}$	904 880	^b
	${{}^{3}D}_{1}^{\circ}$	909 540	^b, ^d
	${{}^{1}P}_{1}^{\circ}$	917 750	^b, ^d
3d⁹5f	${{}^{3}P}_{1}^{\circ}$	1 030 260	^a
	${{}^{3}D}_{1}^{\circ}$	1 033 470	^c, ^d
	${{}^{1}P}_{1}^{\circ}$	1 040 900	^c, ^d
3d⁹6f	${{}^{3}D}_{1}^{\circ}$	1 100 930	^c, ^d
	${{}^{1}P}_{1}^{\circ}$	1 108 000	^c, ^d
3d⁹7f	³D₁	1141 690	^c, ^d
	${{}^{1}P}_{1}^{\circ}$	1 148 440	^c, ^d

Configuration	Designation	J	Level Value (cm⁻¹)	Δ^a	Composition^b
3d⁸4s	(³F)⁴F	9/2	525 659.1	8.6	100%
		7/2	529 307.0	10.5	87% + 12%(³F)²F + 1%(¹G)²G
		5/2	533 147.1	8.2	96% + 3%(³F)²F + 1%(¹D)²D
		3/2	535 368.9	24.4	95% + 5%(¹D)²D
	(³F)²F	7/2	537 429.3	−56.5	87% + 12%(³F)⁴F + 1%(¹G)²G
		5/2	542 929.5	5.7	89% + 8%(¹D)²D + 2%(³F)⁴F
	(³P)⁴P	5/2	553 937.8	12.9	52% + 40%(¹D)²D + 6%(³F)²F
		3/2	561 128.6	−18.5	84% + 15%(¹D)²D + 1%(³P)²P
		1/2	561 200.0	−32.0	99% + 1%(¹S)²S
	(¹D)²D	5/2	562 261.3	−4.2	50% + 47%(³P)⁴P + 2%(³F)²F
		3/2	555 686.8	3.4	70% + 16%(³P)⁴P + 10%(³P)²P
	(³P)²P	3/2	568 958.0	−42.8	89% + 10%(¹D)²D + 1%(³P)⁴P
		1/2	570 361.0	80.5	99% + 1%(¹S)²S
	(1G)²G	9/2	573 518.5	−13.8	100%
		7/2	573 581.0	14.0	99% + 1%(³P)²F
	(¹S)²S	1/2	628 180.1	−0.2	99% + 1%(³P)⁴P
3d⁸4p	(³F)⁴D	7/2	655 301.0	−159.6	84% + 8%(³F)⁴F + 4%(³P)⁴D
		5/2	661 777.6	−97.0	81% + 10%(³P)⁴P + 7%(³P)⁴D
		3/2	666 638.4	−5.5	81% + 9%(³P)⁴D + 9%(³F)⁴F
		1/2	669 527.3	−48.7	85% + 12%(³P)⁴D + 2%(¹D)²P
	(³F)⁴G	11/2	665 589.8	15.2	100%
		9/2	660 547.0	−72.4	48% + 30%(³F)²G + 21%(³F)⁴P
		7/2	665 040.0	−0.6	72% + 14%(³F)⁴F + 11%(³P)²G
	(³F)⁴F	9/2	670 130.5	59.7	75% + 19%(³P)²G + 5%(³F)⁴G
	(³F)²G	9/2	674 002.5	−27.3	50% + 47%(³P)⁴G + 3%(³F)⁴F
	(³P)⁴P	1/2	687 338.6	95.1	90% + 5%(¹D)²P + 3%(³P)²P
	(¹D)²P	3/2	698 872.4^c	−21.4	29% + 26%(¹D)²D + 20%(³P)⁴D
	(³P)⁴D	3/2	700 567.6^c	95.4	49% + 28%(¹D)²P + 8%(¹D)²D
	(¹G)²H	11/2	709 504.3	−54.2	100%
		9/2	702 828.6	−67.2	96% + 4%(¹G)²G
	(³P)⁴S	3/2	714 289.3	10.9	95% + 2%(³P)⁴P + 1%(¹D)²P
	(¹G)²G	9/2	722 842.6	−19.6	96% + 3%(¹G)²H + 1%(³P)⁴F
		7/2	721 815.0	45.6	94% + 5%(¹G)²F + 1%(¹D)²F

λ (Å)	σ (cm⁻¹)	I^a	Char.^b	Even Level	Odd Level
138.540	721 815.3	12	1	3d^{9 2}D_5/2	(¹G)4p²G_7/2
141.350	707 466.0	4	1	3d^{9 2}D_3/2	(³P)4p²D_5/2
152.602	655 301.0	2	1	3d^{9 2}D_5/2	(³F)4p⁴D_7/2
652.907	153 161.1	43	6	(³P)4s⁴P_3/2	(³P)4p⁴S_3/2
653.215	153 088.9	24	1	(³P)4s⁴P_1/2	(³P)4p⁴S_3/2
657.773	152 028.2	50	6	(¹D)4s²D_5/2	(³P)4p⁴S_3/2
669.119	149 450.3	18	0	(³F)4s²P_7/2	(³P)4p⁴P_5/2
669.684	149 324.1	49	6	(¹G)4s²G_9/2	(¹G)4p²G_9/2
671.358	148 951.9	16	6	(³P)4s⁴P_5/2	(³P)4p⁴D_7/2
674.609	148 234.0	40	6	(¹G)4s²G_7/2	(¹G)4p²G_7/2
682.499	146 520.3	14	6	(¹D)4s²D_5/2	(¹G)4p²P_7/2
687.608	145 431.7	70	4	(³P)4s²P_3/2	(³P)4p²S_1/2
691.100	144 696.9	8	6	(³F)4s⁴P_7/2	(³F)4p²G_9/2
692.178	144 471.4	62	1	(³P)4s⁴P_9/2	(³F)4p⁴P_9/2
696.843	143 504.3	2	6	(³F)4s⁴P_5/2	(³F)4p²D_5/2
698.793	143 103.8	15	0	(¹S)4s²S_1/2	(¹S)4p²P_3/2
700.655	142 723.7	27	0	(³F)4s⁴P_7/2	(³P)4p²P_7/2
708.881	141 067.3	25	0	(³P)4s⁴P_5/2	(¹D)4p²F_7/2
709.687	140 907.2	12	1	(³P)4s²P_1/2	(³P)4p²P_1/2
710.109	140 823.5	33	0	(³F)4s⁴F_7/2	(³P)4p⁴P_9/2
711.050	140 637.0	72	1	(¹D)4s²D_5/2	(³P)4p⁴D_7/2
713.000	140 252.4	2	5	(³P)4s⁴P_5/2	(³F)4p⁴P_5/2
713.194	140 214.3	32	6D	(³P)4s²P_7/2	(³F)4p²F_7/2
			D	(³P)4s⁴P_3/2	(³P)4p⁴D_5/2
714.165	140 023.6	37	0	(³P)4s²P_5/2	(³F)4p²P_5/2
714.640	139 930.6	63	6	(³P)4s⁴P_9/2	(³F)4p⁴G1_1/2
717.527	139 367.6	41	1	(³P)4s⁴P_1/2	(³P)4p⁴D_3/2
717.810	139 312.6	14	0	(³P)4s²P_1/2	(³P)4p²D_3/2
718.273	139 222.8	43	6	(³P)4s²F_7/2	(³P)4p²D_5/2
718.780	139 124.7	34	7	(³P)4s⁴P_1/2	(³P)4p⁴D_1/2
720.030	138 883.2	20	0	(³F)4s⁴F_5/2	(³F)4p²F_7/2
721.736	138 554.9	23	6	(¹G)4s²G_7/2	(¹G)4p²F_5/2
721.928	138 518.0	22	6	(³P)4s²P_3/2	(³P)4p²D_5/2
726.005	137 740.2	8	0	(³F)4s²F_5/2	(³P)4p⁴F_3/2
729.927	137 000.1	14	0	(³F)4s⁴F_3/2	(³F)4p²D_3/2
			M	(³P)4s⁴P_5/2	(¹D)4p²F_5/2
730.532	136 886.6	4	1	(³P)4s²P_3/2	(³P)4p²P_3/2
732.215	136 571.9	56	0	(³F)4s²F_7/2	(³F)4p²G_9/2
733.514	136 330.0	49	0	(³F)4s²F_5/2	(³F)4p²G_7/2
735.371	135 985.8	72	6	(¹G)4s²G_9/2	(¹G)4p²H1_1/2
736.722	135 736.4	44	0	(³F)4s⁴F_7/2	(³F)4p⁴G_7/2
737.209	135 646.7	77	4B	(¹S)4s²S_1/2	(¹S)4p²P_1/2
739.371	135 250.1	28	0D	(¹D)4s²D_3/2	(¹D)4p²F_5/2
			D	(¹G)4s²G_9/2	(¹G)4p²P_7/2
741.059	134 942.1	13	1	(¹D)4s²D_5/2	(¹D)4p²D_5/2
741.356	134 887.9	46	6	(³F)4s⁴F_9/2	(³F)4p⁴G_9/2
742.938	134 600.7	3	0	(³F)4s²F_1/2	(³F)4p²F_7/2
743.449	134 508.2	27	0D	(³F)4s⁴F_5/2	(³F)4p⁴G_5/2
			D	(³P)4s⁴P_3/2	(¹D)4p²P_1/2
745.388	134 158.3	25	0	(³F)4s⁴F_3/2	(³F)4p⁴D_1/2
748.395	133 619.3	2	5	(³P)4s⁴P_3/2	(¹D)4p²D_3/2
749.112	133 491.3	14	0	(³F)4s⁴F_5/2	(³F)4p⁴D_3/2
752.127	132 956.3	40	0	(³P)4s⁴P_5/2	(³P)4p⁴P_5/2
753.360	132 738.6	2	5	(¹D)4s²D_5/2	(¹D)4p²P_7/2
753.578	132 700.3	6	5	(³F)4s²F_7/2	(³F)4p⁴F_9/2
754.885	132 470.6	60	0	(³F)4s⁴F_7/2	(³F)4p⁴D_5/2
755.375	132 384.6	13	5	(³P)4s²P_3/2	(³P)4p⁴D_5/2
756.001	132 275.0	36	0	(³F)4s⁴F_3/2	(³P)4p⁴G_5/2
757.485	132 015.8	19	0	(³P)4s⁴P_5/2	(³P)4p⁴P_3/2
758.191	131 892.9	47	0	(³F)4s⁴F_5/2	(³P)4p⁴G_7/2
759.559	131 655.3	74	7	(¹D)4s²D_3/2	(³P)4p⁴P_1/2
761.984	131 236.4	69	0	(³F)4s⁴F_1/2	(³P)4p⁴G_9/2
769.449	129 963.1	4	6	(³P)4s²P_1/2	(³P)4p⁴D_1/2
771.355	129 641.9	60	0	(³F)4s⁴F_9/2	(³F)4p⁴D_7/2
772.946	129 375.1	24	0	(¹G)4s²G_9/2	(³P)4p⁴D_7/2
773.289	129 317.8	2	1	(¹G)4s²G_9/2	(¹G)4p²H_9/2
			M	(¹G)4s²G_7/2	(³P)4p⁴D_7/2
773.709	129 247.6	48	1	(¹G)4s²G_7/2	(¹G)4p²H_9/2
777.235	128 661.2	15	7	(¹D)4s²D_5/2	(¹D)4p²P_5/2
779.819	128 234.9	10	0	(³P)4s²P_3/2	(¹Z)4p²D_5/2
783.669	127 604.9	66	1	(³F)4s²F_7/2	(³P)4p⁴G_7/2
792.328	126 210.4	5	1	(³P)4s⁴P_3/2	(³P)4p⁴P_1/2
801.557	124 757.2	9	1	(³P)4s⁴P_1/2	(³P)4p⁴P_3/2
808.426	123 697.1	31	7	(¹D)4s²D_5/2	(³P)4p⁴P_3/2
812.225	123 118.6	9	0	(³P)4s²F_7/2	(³P)4p⁴G_9/2
818.609	122 158.5	77	1	(³F)4s⁴F_5/2	(³P)4p⁴D_7/2
818.937	122 109.5	79	1	(³P)4s²F_5/2	(³F)4p⁴G_7/2
846.752	118 098.3	5	1	(³P)4s⁴P_5/2	(³F)4p²P_7/2
852.087	117 358.9	78	8	(¹G)4s²G_7/2	(¹D)4p²P_5/2

Abstract

Cited By

Figures (2)

Tables (8)

Equations (3)

Journal of the Optical Society of America B