High-resolution Fourier transform measurements of line strengths in the 00<sup>0</sup>2-00<sup>0</sup>0 main isotopologue band of nitrous oxide

Viktor Werwein; Jens Brunzendorf; Gang Li; Anton Serdyukov; Olav Werhahn; Volker Ebert

doi:10.1364/AO.56.000E99

Applied Optics
Vol. 56,
Issue 11,
pp. E99-E105
(2017)
•https://doi.org/10.1364/AO.56.000E99

High-resolution Fourier transform measurements of line strengths in the 00⁰2-00⁰0 main isotopologue band of nitrous oxide

Viktor Werwein, Jens Brunzendorf, Gang Li, Anton Serdyukov, Olav Werhahn, and Volker Ebert

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Viktor Werwein, Jens Brunzendorf, Gang Li, Anton Serdyukov, Olav Werhahn, and Volker Ebert, "High-resolution Fourier transform measurements of line strengths in the 00⁰2-00⁰0 main isotopologue band of nitrous oxide," Appl. Opt. 56, E99-E105 (2017)

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Abstract

Nitrous oxide ( $N_{2} O$ ) is a key greenhouse gas and a major ozone-depleting anthropogenic pollutant monitored by the total carbon column observing network (TCCON) in the $00^{0} 2 - 00^{0} 0$ -band of its main isotopologue. Here, we present highly accurate line strengths for this window determined using Fourier transform infrared spectroscopy with pressure, temperature, and optical path length being metrologically traceable to the SI. The obtained results agree with previous studies within the given uncertainties. Depending on the respective rovibrational transition, the present uncertainties could be reduced by a factor of 5 to 83 in comparison to literature data.

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$J$	$ν_{0}$	$S$	$U (S)$	$Δ (S)$	$U (Δ (S))$	$Δ (S)$	$U (Δ (S))$	$Δ (S)$	$U (Δ (S))$
	HITRAN [20]	This Study		Toth Calculation [28]		Toth Measurement [27]		Daumont et al. [26]
1	${cm}^{- 1}$	$10^{- 22} {cm}^{- 1} / (mol. \cdot {cm}^{- 2})$	%	%	%	%	%	%	%
0	4418.20196	1.191	0.81	1.12	4.72	-	-	−0.47	5.04
1	4419.01234	2.376	0.47	0.86	4.66	−4.08	3.87	−0.66	4.99
2	4419.80888	3.527	0.36	1.00	4.66	−6.91	18.62	−0.50	4.99
3	4420.59159	4.633	0.31	1.18	4.66	2.71	6.17	−0.33	4.99
4	4421.36046	5.684	0.29	1.36	4.67	0.77	4.04	−0.14	5.00
5	4422.11549	6.695	0.27	1.09	4.66	0.00	6.01	−0.37	4.99
6	4422.85668	7.607	0.26	1.23	4.66	3.39	4.14	−0.22	5.00
7	4423.58401	8.450	0.25	1.15	4.66	0.71	4.04	−0.30	4.99
8	4424.29749	9.200	0.25	1.09	4.66	5.22	4.22	−0.32	4.99
9	4424.99711	9.842	0.25	1.13	4.66	−0.01	10.00	−0.26	4.99
10	4425.68287	10.377	0.24	1.28	4.67	1.06	6.07	−0.16	5.00
11	4426.35476	10.815	0.24	1.25	4.66	0.69	4.04	−0.14	5.00
12	4427.01278	11.180	0.24	0.98	4.65	0.29	4.02	−0.36	4.99
13	4427.65693	11.406	0.24	1.00	4.65	4.31	4.18	−0.32	4.99
14	4428.28720	11.548	0.24	0.97	4.65	3.04	4.13	−0.41	4.99
15	4428.90358	11.571	0.24	1.03	4.65	5.26	21.05	−0.27	4.99
16	4429.50609	11.521	0.24	0.94	4.65	1.52	8.13	−0.36	4.99
17	4430.09470	11.379	0.24	0.89	4.65	2.79	6.17	−0.34	4.99
18	4430.66942	11.163	0.24	0.87	4.65	2.97	4.13	−0.38	4.99
19	4431.23024	10.868	0.24	0.85	4.65	2.80	4.12	−0.35	4.99
20	4431.77717	10.534	0.24	0.63	4.64	2.61	4.11	−0.51	4.98
21	4432.31019	10.113	0.25	0.76	4.64	2.09	4.09	−0.43	4.98
22	4432.82930	9.671	0.25	0.66	4.64	−1.57	7.88	−0.47	4.98
23	4433.33450	9.190	0.25	0.60	4.63	−3.45	19.31	−0.52	4.98
24	4433.82578	8.681	0.25	0.57	4.63	3.61	4.15	-	-
25	4434.30315	8.153	0.26	0.53	4.63	1.42	6.09	−0.54	4.98
26	4434.76660	7.609	0.26	0.57	4.63	6.02	6.37	−0.47	4.98
27	4435.21612	7.079	0.27	0.39	4.63	2.56	6.16	−0.63	4.98
28	4435.65171	6.559	0.27	0.08	4.61	−1.61	5.91	−0.91	4.96
29	4436.07337	6.017	0.28	0.23	4.62	3.90	6.24	−0.73	4.97
30	4436.48109	5.496	0.29	0.30	4.62	2.73	4.12	−0.62	4.98
31	4436.87488	5.013	0.30	0.02	4.61	1.37	10.14	−0.88	4.97
32	4437.25472	4.533	0.32	0.10	4.62	3.84	8.31	−0.79	4.97
33	4437.62062	4.092	0.33	−0.14	4.61	−2.61	5.85	−0.99	4.96
34	4437.97257	3.675	0.35	−0.37	4.60	5.37	21.08	−1.19	4.95
35	4438.31056	3.264	0.38	0.01	4.62	−1.51	9.86	−0.79	4.97
36	4438.63461	2.905	0.40	−0.28	4.60	−2.40	5.87	−1.07	4.96
37	4438.94469	2.558	0.44	0.00	4.62	−3.03	5.83	−0.74	4.98
38	4439.24081	2.252	0.48	−0.12	4.62	1.03	6.08	−0.83	4.98
39	4439.52297	1.982	0.53	−0.74	4.60	1.76	8.16	−1.40	4.96
40	4439.79116	1.736	0.59	−1.33	4.58	−0.11	6.02	-	-

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Applied Optics