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Theoretical far-wing line shape and absorption for high-temperature CO2

Qiancheng Ma, Richard H. Tipping, Christian Boulet, and Jean-Pierre Bouanich

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Abstract

Theoretical results for the far-wing line shapes and corresponding absorption coefficients in the high-frequency wing of the ν 3 fundamental band of self-broadened CO2 are presented for a number of temperatures between 218 and 751 K. These first-principles calculations are made assuming binary collisions within the framework of a quasi-static theory with a more accurate interaction potential than in previous calculations. The theoretical results are compared with existing laboratory data and are in good agreement for all the temperatures considered.

© 1999 Optical Society of America

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