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Coherent Control of a Single-Molecule Switch with Sub-Cycle Atomic Forces

Lukas Z. Kastner, Dominik Peller, Thomas Buchner, Carmen Roelcke, Florian Albrecht, Nikolaj Moll, Jascha Repp, and Rupert Huber

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Abstract

We introduce sub-cycle atomic-scale forces provided by near fields of a lightwave-driven scanning probe tip. Exerting these ultrafast forces to key atoms of a single-molecule switch allows us to coherently steer a select structural rotation that modulates the switching statistics by up to 39%.

© 2020 The Author(s)

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