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Ultrafast nonadiabatic dynamics through an intermolecular conical intersection

Antonietta De Sio, Ephraim Sommer, Lynn Gross, Xuan Trung Nguyen, Duško Popović, Elena Mena-Osteritz, Peter Bäuerle, Thomas Frauenheim, Sergei Tretiak, and Christoph Lienau

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Abstract

Combining <10-fs two-dimensional electronic spectroscopy and atomistic nonadiabatic dynamics simulations, we track, for the first time, vibrational wavepacket motion through an intermolecular conical intersection governing the sub-100-fs energy transfer in photovoltaic molecular aggregates.

© 2020 The Author(s)

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