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Tracking Ultrafast Charge Separation in a PBI-based Biomimetic Complex for Oxygen Evolution

Margherita Maiuri, Mattia Russo, Luca Moretti, Vasilis Petropoulos, Francesco Rigodanza, Andrea Sartorel, Maurizio Prato, Giulio Cerullo, and Marcella Bonchio

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Abstract

Multidimensional spectroscopies reveal a two-step process in a biomimetic supracomplex for oxygen evolution. A sub-ps charge-separation within the light-sensitizer moiety is followed by hole transfer from the catalyst counterpart, forming productive charges.

© 2020 The Author(s)

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